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Nonequilibrium Antiferromagnetic State in the Heavy Electron Compound URu_2Si_2

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 Added by Makoto Yokoyama
 Publication date 2002
  fields Physics
and research's language is English




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We have investigated the nature of the antiferromagnetic (AF) phase induced by uniaxial stress sigma in URu2Si2, by performing elastic neutron scattering measurements up to 0.4 GPa. We have found that the AF Bragg-peak intensity shows a clear hysteresis loop with sigma under the zero-stress cooling condition. The result strongly suggests that the sigma-induced AF phase is metastable and separated from the coexisting hidden ordered phase by a first-order phase transition. We also present the analyses of the crystalline strain effects, and suggest that the c/a ratio plays an important role in the competition between these two phases.



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We have performed the elastic neutron scattering experiments under uniaxial stress sigma along the tetragonal [100], [110] and [001] directions for URu2Si2. For sigma // [100] and [110], the antiferromagnetic moment mu_o is strongly enhanced from 0.02 mu_B (sigma=0) to 0.22 mu_B (sigma=2.5 kbar) at 1.5 K. The rate of increase dmu_o/dsigma is roughly estimated to be ~ 0.1 mu_B/kbar, which is much larger than that for the hydrostatic pressure (~ 0.025 mu_B/kbar). Above 2.5 kbar, mu_o shows a tendency to saturate similar to the behavior in the hydrostatic pressure. For sigma // [001], on the other hand, mu_o shows only a slight increase to 0.028 mu_B (sigma = 4.6 kbar) with a rate of ~ 0.002 mu_B/kbar. The observed anisotropy suggests that the competition between the hidden order and the antiferromagnetic state in URu2Si2 is strongly coupled with the tetragonal four-fold symmetry and the c/a ratio, or both.
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The effect of pressure on the unique electronic state of the antiferromagnetic (AF) compound EuCu2Ge2 has been measured in a wide temperature range from 10 mK to 300 K by electrical resistivity measurements up to 10 GPa. The Neel temperature of TN = 15 K at ambient pressure increases monotonically with increasing pressure and becomes a maximum of TN = 27 K at 6.2 GPa but suddenly drops to zero at Pc = 6.5 GPa, suggesting the quantum critical point (QCP) of the valence transition of Eu from a nearly divalent state to that with trivalent weight. The rhomag0 and A values obtained from the low-temperature electrical resistivity based on the Fermi liquid relation of rhomag = rhomag0 + AT^2 exhibit huge and sharp peaks around Pc. The exponent n obtained from the power law dependence rhomag = rhomag0 + BT^n is clearly less than 1.5 at P = Pc = 6. 5 GPa, which is expected at the AF-QCP. These results indicate that Pc coincides with Pv, corresponding to the quantum criticality of the valence transition pressure Pv. The electronic specific heat coefficient, estimated from the generalized Kadowaki-Woods relation, is about 510 mJ/mol K^2 around Pc, suggesting the formation of a heavy-fermion state.
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