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Register a new userContacting single bundles of carbon nanotubes with alternating electric fields
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Single bundles of carbon nanotubes have been selectively deposited from suspensions onto sub-micron electrodes with alternating electric fields. We explore the resulting contacts using several solvents and delineate the differences between Au and Ag as electrode materials. Alignment of the bundles between electrodes occurs at frequencies above 1 kHz. Control over the number of trapped bundles is achieved by choosing an electrode material which interacts strongly with the chemical functional groups of the carbon nanotubes, with superior contacts being formed with Ag electrodes.
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We report measurements of the temperature and gate voltage dependence for individual bundles (ropes) of single-walled nanotubes. When the conductance is less than about e^2/h at room temperature, it is found to decrease as an approximate power law of temperature down to the region where Coulomb blockade sets in. The power-law exponents are consistent with those expected for electron tunneling into a Luttinger liquid. When the conductance is greater than e^2/h at room temperature, it changes much more slowly at high temperatures, but eventually develops very large fluctuations as a function of gate voltage when sufficiently cold. We discuss the interpretation of these results in terms of transport through a Luttinger liquid.
Helical modes, conducting opposite spins in opposite directions, are shown to exist in metallic armchair nanotubes in an all-electric setup. This is a consequence of the interplay between spin-orbit interaction and strong electric fields. The helical regime can also be obtained in chiral metallic nanotubes by applying an additional magnetic field. In particular, it is possible to obtain helical modes at one of the two Dirac points only, while the other one remains gapped. Starting from a tight-binding model we derive the effective low-energy Hamiltonian and the resulting spectrum.
Smoothly varying lattice strain in graphene affects the Dirac carriers through a synthetic gauge field. When the lattice strain is time dependent, as in connection with phononic excitations, the gauge field becomes time dependent and the synthetic vector potential is also associated with an electric field. We show that this synthetic electric field has observable consequences. Joule heating associated with the currents driven by the synthetic electric field dominates the intrinsic damping, caused by the electron-phonon interaction, of many acoustic phonon modes of graphene and metallic carbon nanotubes when including the effects of disorder and Coulomb interactions. Several important consequences follow from the observation that by time-reversal symmetry, the synthetic electric field associated with the vector potential has opposite signs for the two valleys. First, this implies that the synthetic electric field drives charge-neutral valley currents and is therefore unaffected by screening. This frequently makes the effects of the synthetic vector potential more relevant than a competing effect of the scalar deformation potential which has a much larger bare coupling constant. Second, valley currents decay by electron-electron scattering (valley Coulomb drag) which causes interesting temperature dependence of the damping rates. While our theory pertains first and foremost to metallic systems such as doped graphene and metallic carbon nanotubes, the underlying mechanisms should also be relevant for semiconducting carbon nanotubes when they are doped.
Using molecular dynamics simulations, we investigate systematically the water permeation properties across the single-walled carbon nanotube (SWCNT) in the presence of the terahertz electric field (TEF). With the TEF normal to the nanotube, the fracture of the hydrogen bonds results in the giant peak of net fluxes across the SWCNT with a three-fold enhancement centered around 14THz. The phenomenon is attributed to the resonant mechanisms, characterized by librational, rotational, and rotation-induced responses of in-tube polar water molecules to the TEF. For the TEF along the symmetry axis of the nanotube, the vortical modes for resonances and consequently the enhancement of net fluxes are greatly suppressed by the alignment of polar water along the symmetry axis, which characterizes the quasi one-dimensional feature of the SWCNT nicely. The resonances of water molecules in the TEF can have potential applications in the high-flux device designs used for various purposes.
The radial thermal expansion (ar) of bundles of single-walled carbon nanotubes saturated with 4He impurities to the molar concentration 9.4% has been investigated in the interval 2.5-9.5 K using the dilatometric method. In the interval 2.1-3.7 K (ar) is negative and is several times higher than the negative (ar) for pure nanotube bundles. This most likely points to 4He atom tunneling between different positions in the nanotube bundle system. The excess expansion was reduced with decreasing 4He concentration.
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