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Glauber slow dynamics of the magnetization in a molecular Ising chain

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 Added by Roberta Sessoli
 Publication date 2001
  fields Physics
and research's language is English




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The slow dynamics (10^-6 s - 10^4 s) of the magnetization in the paramagnetic phase, predicted by Glauber for 1d Ising ferromagnets, has been observed with ac susceptibility and SQUID magnetometry measurements in a molecular chain comprising alternating Co{2+} spins and organic radical spins strongly antiferromagnetically coupled. An Arrhenius behavior with activation energy Delta=152 K has been observed for ten decades of relaxation time and found to be consistent with the Glauber model. We have extended this model to take into account the ferrimagnetic nature of the chain as well as its helicoidal structure.



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We study the time evolution of the local magnetization in the critical Ising chain in a transverse field after a sudden change of the parameters at a defect. The relaxation of the defect magnetization is algebraic and the corresponding exponent, which is a continuous function of the defect parameters, is calculated exactly. In finite chains the relaxation is oscillating in time and its form is conjectured on the basis of precise numerical calculations.
66 - Yi Liao , Ping-Xing Chen 2018
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The ground state and magnetization process of the mixed spin-(1,1/2) Ising diamond chain is exactly solved by employing the generalized decoration-iteration mapping transformation and the transfer-matrix method. The decoration-iteration transformation is first used in order to establish a rigorous mapping equivalence with the corresponding spin-1 Blume-Emery-Griffiths chain in a non-zero magnetic field, which is subsequently exactly treated within the framework of the transfer-matrix technique. It is shown that the ground-state phase diagram includes just four different ground states and the low-temperature magnetization curve may exhibit an intermediate plateau precisely at one half of the saturation magnetization. Our rigorous results disprove recent Monte Carlo simulations of Zihua Xin et al. [Z. Xin, S. Chen, C. Zhang, J. Magn. Magn. Mater. 324 (2012) 3704], which imply an existence of the other magnetization plateaus at 0.283 and 0.426 of the saturation magnetization.
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