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Register a new userMicrowave Electrodynamics of the Electron-Doped Cuprate Superconductors Pr_(2-x)Ce_(x)CuO_(4-y) and Nd_(2-x)Ce_(x)CuO_(4-y)
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The pairing state symmetry of the electron-doped cuprate superconductors is thought to be s-wave in nature, in contrast with their hole-doped counterparts which exhibit a d-wave symmetry. We re-examine this issue based on recent improvements in our electron-doped materials and our measurement techniques. We report microwave cavity perturbation measurements of the temperature dependence of the penetration depth of Pr_(2-x)Ce_(x)CuO_(4-y) and Nd_(2-x)Ce_(x)CuO_(4-y) crystals. Our data strongly suggest that the pairing symmetry in these materials is not s-wave.
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We use transport and neutron-scattering measurements to show that a magnetic-field-induced transition from noncollinear to collinear spin arrangement in adjacent CuO_{2} planes of lightly electron-doped Pr_{1.3-x}La_{0.7}Ce_{x}CuO_{4} (x=0.01) crystals affects significantly both the in-plane and out-of-plane resistivity. In the high-field collinear state, the magnetoresistance (MR) does not saturate, but exhibits an intriguing four-fold-symmetric angular dependence, oscillating from being positive at B//[100] to being negative at B//[110]. The observed MR of more than 30% at low temperatures induced by a modest modification of the spin structure indicates an unexpectedly strong spin-charge coupling in electron-doped cuprates.
We present a detailed temperature-dependent Raman light scattering study of optical phonons in molecular-beam-epitaxy-grown films of the electron-doped superconductor La_{2-x}Ce_{x}CuO_{4} close to optimal doping (x ~ 0.08, T_c = 29 K and x ~ 0.1, T_c = 27 K). The main focus of this work is a detailed characterization and microstructural analysis of the films. Based on micro-Raman spectroscopy in combination with x-ray diffraction, energy-dispersive x-ray analysis, and scanning electron microscopy, some of the observed phonon modes can be attributed to micron-sized inclusions of Cu_{2}O. In the slightly underdoped film (x ~ 0.08), both the Cu_{2}O modes and others that can be assigned to the La_{2-x}Ce_{x}CuO_{4} matrix show pronounced softening and narrowing upon cooling below T ~ T_c. Based on control measurements on commercial Cu_{2}O powders and on a comparison to prior Raman scattering studies of other high-temperature superconductors, we speculate that proximity effects at La_{2-x}Ce_{x}CuO_{4}/Cu_{2}O interfaces may be responsible for these anomalies. Experiments on the slightly overdoped La_{2-x}Ce_{x}CuO_{4} film (x ~ 0.1) did not reveal comparable phonon anomalies.
Low energy polarized electronic Raman scattering of the electron doped superconductor Nd_1.85Ce_0.15CuO_4 (T_c=22 K) has revealed a nonmonotonic d_{x^2-y^2} superconducting order parameter. It has a maximum gap of 4.4 k_BT_c at Fermi surface intersections with antiferromagnetic Brillouin zone (the ``hot spots) and a smaller gap of 3.3 k_BT_c at fermionic Brillouin zone boundaries. The gap enhancement in the vicinity of the ``hot spots emphasizes role of antiferromagnetic fluctuations and similarity in the origin of superconductivity for electron- and hole-doped cuprates.
Phononic and magnetic Raman scattering are studied in La$_{2-x-y}$Nd$_{y}$Sr$_{x}$CuO$_{4}$ with three doping concentrations: x ~ 1/8, y = 0; x ~ 1/8, y = 0.4; and x = 0.01, y = 0. We observe strong disorder in the tilt pattern of the CuO_{6} octahedra in both the orthorhombic and tetragonal phases which persist down to 10 K and are coupled to bond disorder in the cation layers around 1/8 doping independent of Nd concentration. The weak magnitude of existing charge/spin modulations in the Nd doped structure does not allow us to detect the specific Raman signatures on lattice dynamics or two-magnon scattering around 2200 cm-1.
We study long wavelength magnetic excitations in lightly doped La_{2-x}Sr_{x}CuO_{4} (x < 0.03) detwinned crystals. The lowest energy magnetic anisotropy induced gap can be understood in terms of the antisymmetric spin interaction inside the antiferromagnetic (AF) phase. The second magnetic resonace, analyzed in terms of in-plane spin anisotropy, shows unconventional behavior within the AF state and led to the discovery of collective spin excitations pertaining to a field induced magnetically ordered state. This state persists in a 9 T field to more than 100 K above the N{e}el temperature in x = 0.01.
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