Fractionalization on the surface: Is type-II terminated 1T-TaS$_2$ surface an anomalously realized spin liquid?


Abstract in English

The type-II terminated 1T-TaS$_2$ surface of a three-dimensional 1T-TaS$_2$ bulk material realizes the effective spin-1/2 degree of freedom on each David-star cluster with ${T^2=-1}$ such that the time reversal symmetry is realized anomalously, despite the bulk three-dimensional 1T-TaS$_2$ material has an even number of electrons per unit cell with ${T^2=+1}$. This surface is effectively viewed as a spin-1/2 triangular lattice magnet, except with a symmetry-protected topological bulk. We further propose this surface termination realizes a spinon Fermi surface spin liquid with the surface fractionalization but with a non-exotic three-dimensional bulk. We analyze possible experimental consequences of the type-II terminated surface spin liquid.

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