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Register a new userEnergy spectrum of semimetallic HgTe quantum wells
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Quantum wells (QWs) based on mercury telluride (HgTe) thin films provide a large scale of unusual physical properties starting from an insulator via a two-dimensional Dirac semimetal to a three-dimensional topological insulator. These properties result from the dramatic change of the QW band structure with the HgTe film thickness. Although being a key property, these energy dispersion relations cannot be reflected in experiments due to the lack of appropriate tools. Here we report an experimental and theoretical study of two HgTe quantum wells with inverted energy spectrum in which two-dimensional semimetallic states are realized. Using magneto-optical spectroscopy at sub-THz frequencies we were able to obtain information about electron and hole cyclotron masses at all relevant Fermi level positions and different charge densities. The outcome is also supported by a Shubnikov-de Haas analysis of capacitance measurements, which allows obtaining information about the degeneracy of the active modes. From these data, it is possible to reconstruct electron and hole dispersion relations. Detailed comparative analysis of the energy dispersion relations with theoretical calculations demonstrates a good agreement, reflecting even several subtle features like band splitting, the second conduction band, and the overlaps between the first conduction and first valence band. Our study demonstrates that the cyclotron resonance experiments can be efficiently used to directly obtain the band structures of semimetallic 2D materials.
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The results of experimental study of interference induced magnetoconductivity in narrow HgTe quantum wells of hole-type conductivity with a normal energy spectrum are presented. Interpretation of the data is performed with taking into account the strong spin-orbit splitting of the energy spectrum of the two-dimensional hole subband. It is shown that the phase relaxation time found from the analysis of the shape of magnetoconductivity curves for the relatively low conductivity when the Fermi level lies in the monotonic part of the energy spectrum of the valence band behaves itself analogously to that observed in narrow HgTe quantum wells of electron-type conductivity. It increases in magnitude with the increasing conductivity and decreasing temperature following the $1/T$ law. Such a behavior corresponds to the inelasticity of electron-electron interaction as the main mechanism of the phase relaxation and agrees well with the theoretical predictions. For the higher conductivity, despite the fact that the dephasing time remains inversely proportional to the temperature, it strongly decreases with the increasing conductivity. It is presumed that a nonmonotonic character of the hole energy spectrum could be the reason for such a peculiarity. An additional channel of the inelastic interaction between the carriers in the main and secondary maxima occurs when the Fermi level arrives the secondary maxima in the depth of the valence.
We propose a minimal effective two-dimensional Hamiltonian for HgTe/CdHgTe quantum wells (QWs) describing the side maxima of the first valence subband. By using the Hamiltonian, we explore the picture of helical edge states in tensile and compressively strained HgTe QWs. We show that both dispersion and probability density of the edge states can differ significantly from those predicted by the Bernevig-Hughes-Zhang (BHZ) model. Our results pave the way towards further theoretical investigations of HgTe-based quantum spin Hall insulators with direct and indirect band gaps beyond the BHZ model.
The results of experimental study of the magnetoresistivity, the Hall and Shubnikov-de Haas effects for the heterostructure with HgTe quantum well of 20.2 nm width are reported. The measurements were performed on the gated samples over the wide range of electron and hole densities including vicinity of a charge neutrality point. Analyzing the data we conclude that the energy spectrum is drastically different from that calculated in framework of $kP$-model. So, the hole effective mass is equal to approximately $0.2 m_0$ and practically independent of the quasimomentum ($k$) up to $k^2gtrsim 0.7times 10^{12}$ cm$^{-2}$, while the theory predicts negative (electron-like) effective mass up to $k^2=6times 10^{12}$ cm$^{-2}$. The experimental effective mass near k=0, where the hole energy spectrum is electron-like, is close to $-0.005 m_0$, whereas the theoretical value is about $-0.1 m_0$.
The solutions for the helical edge states for an effective continuum model for the quantum spin Hall effect in HgTe/CdTe quantum wells are presented. For a sample of a large size, the solution gives the linear dispersion for the edge states. However, in a finite strip geometry, the edge states at two sides will couple with each other, which leads to a finite energy gap in the spectra. The gap decays in an exponential law of the width of sample. The magnetic field dependence of the edge states illustrates the difference of the edge states from those of a conventional quantum Hall strip of two-dimensional electron gas.
Using $vec{k}$$cdot$$vec{p}$ theory, we derive an effective four band model describing the physics of the typical two-dimensional topological insulator (HgTe/CdTe quantum well) in the presence of out-of-plane in z-direction inversion breaking and in-plane confining potentials. We find that up to third order in perturbation theory, only the inversion breaking potential generates new elements to the four band Hamiltonian that are off-diagonal in spin space. When this new effective Hamiltonian is folded into an effective two band model for the conduction (electron) or valence (heavy hole) bands, two competing terms appear: (1) a Rashba spin-orbit interaction originating from inversion breaking potential in z-direction and (2) an in-plane Pauli term as a consequence of the in-plane confining potential. Spin transport in the conduction band is further analysed within the Landauer-Buttiker formalism. We find that for asymmetrically doped HgTe quantum wells, the behaviour of the spin-Hall conductance is dominated by the Rashba term.
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