Recent studies have demonstrated the significant roles of droplet self-spin motion in affecting the head-on collision of binary droplets. In this paper, we present a computational study by using the Volume-of-Fluid (VOF) method to investigate the spin-affected droplet separation of off-center collisions, which are more probable in reality and phenomenologically richer than head-on collisions. Different separation modes are identified through a parametric study with varying spinning speed and impact parameter. A prominent finding is that increasing the droplet spinning speed tends to suppress the reflexive separation and to promote the stretching separation. Physically, the reflexive separation is suppressed because the increased rotational energy reduces the excessive reflexive kinetic energy within the droplet, which is the cause for the droplet reflexive separation. The stretching separation is promoted because the increased droplet angular momentum enhances the local stretching flow within the droplet, which tends to separate the droplet. The roles of orbital angular momentum and spin angular momentum in affecting the droplet separation are further substantiated by studying the collision between two spinning droplets with either the same or opposite chirality. In addition, a theoretical model based on conservation laws is proposed to qualitatively describe the boundaries of coalescence-separation transition influenced by droplet self-spin motion.
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