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Register a new userEmergent Interfacial Superconductivity between Twisted Cuprate Superconductors
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Shu Yang Frank Zhao
Publication date
2021
fields
Physics
and research's language is
English
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Twisted interfaces between stacked van der Waals cuprate crystals enable tunable Josephson coupling between in-plane anisotropic superconducting order parameters. Employing a novel cryogenic assembly technique, we fabricate Josephson junctions with an atomically sharp twisted interface between Bi2Sr2CaCu2O8+x crystals. The Josephson critical current density sensitively depends on the twist angle, reaching the maximum value comparable to that of the intrinsic junctions at small twisting angles, and is suppressed by almost 2 orders of magnitude yet remains finite close to 45 degree twist angle. Through the observation of fractional Shapiro steps and the analysis of Fraunhofer patterns we show that the remaining superconducting coherence near 45 degree is due to the co-tunneling of Cooper pairs, a necessary ingredient for high-temperature topological superconductivity.
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Twisted bilayers of high-$T_c$ cuprate superconductors have been argued to form topological phases with spontaneously broken time reversal symmetry ${cal T}$ for certain twist angles. With the goal of helping to identify unambiguous signatures of these topological phases in transport experiments, we theoretically investigate a suite of Josephson phenomena between twisted layers. We find an unusual non-monotonic temperature dependence of the critical current at intermediate twist angles which we attribute to the unconventional sign structure of the $d$-wave order parameter. The onset of the ${cal T}$-broken phase near $45^circ$ twist is marked by a crossover from the conventional $2pi$-periodic Josephson relation $J(varphi)simeq J_csin{varphi}$ to a $pi$-periodic function as the single-pair tunneling becomes dominated by a second order process that involves two Cooper pairs. Despite this fundamental change, the critical current remains a smooth function of the twist angle $theta$ and temperature $T$ implying that a measurement of $J_c$ alone will not be a litmus test for the ${cal T}$-broken phase. To obtain clear signatures of the ${cal T}$-broken phase one must measure $J_c$ in the presence of an applied magnetic field or radio-frequency drive, where the resulting Fraunhofer patterns and Shapiro steps are altered in a characteristic manner. We discuss these results in light of recent experiments on twisted bilayers of the high-$T_c$ cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+delta}$.
Geometrical Berry phase is recognized as having profound implications for the properties of electronic systems. Over the last decade, Berry phase has been essential to our understanding of new materials, including graphene and topological insulators. The Berry phase can be accessed via its contribution to the phase mismatch in quantum oscillation experiments, where electrons accumulate a phase as they traverse closed cyclotron orbits in momentum space. The high-temperature cuprate superconductors are a class of materials where the Berry phase is thus far unknown despite the large body of existing quantum oscillations data. In this report we present a systematic Berry phase analysis of Shubnikov - de Haas measurements on the hole-doped cuprates YBa$_2$Cu$_3$O$_{y}$, YBa$_2$Cu$_4$O$_8$, HgBa$_2$CuO$_{4 + delta}$, and the electron-doped cuprate Nd$_{2-x}$Ce$_x$CuO$_4$. For the hole-doped materials, a trivial Berry phase of 0 mod $2pi$ is systematically observed whereas the electron-doped Nd$_{2-x}$Ce$_x$CuO$_4$ exhibits a significant non-zero Berry phase. These observations set constraints on the nature of the high-field normal state of the cuprates and points towards contrasting behaviour between hole-doped and electron-doped materials. We discuss this difference in light of recent developments related to charge density-wave and broken time-reversal symmetry states.
Motivated by the recent proposals for unconventional emergent physics in twisted bilayers of nodal superconductors, we study the peculiarities of the Josephson effect at the twisted interface between $d$-wave superconductors. We demonstrate that for clean interfaces with a twist angle $theta_0$ in the range $0^circ<theta_0<45^circ$ the critical current can exhibit nonmonotonic temperature dependence with a maximum at a nonzero temperature as well as a complex dependence on the twist angle at low temperatures. The former is shown to arise quite generically due to the contributions of the momenta around the gap nodes, which are negative for nonzero twist angles. It is demonstrated that these features reflect the geometry of the Fermi surface and are sensitive to the form of the momentum dependence of the tunneling at the twisted interface. Close to $theta_0=45^circ$ we find that the critical current does not vanish due to Cooper pair cotunneling, which leads to a transition to a time-reversal breaking topological superconducting $d+id$ phase. Weak interface roughness, quasiperiodicity, and inhomogeneity broaden the momentum dependence of the interlayer tunneling leading to a critical current $I_csim cos(2theta_0)$ with $cos(6theta_0)$ corrections. Furthermore, strong disorder at the interface is demonstrated to suppress the time-reversal breaking superconducting phase near $theta_0=45^circ$. Last, we provide a comprehensive theoretical analysis of experiments that can reveal the full current-phase relation for twisted superconductors close to $theta_0=45^circ$. In particular, we demonstrate the emergence of the Fraunhofer interference pattern near $theta_0=45^circ$, while accounting for realistic sample geometries, and show that its temperature dependence can yield unambiguous evidence of Cooper pair cotunneling, necessary for topological superconductivity.
Magic-angle twisted trilayer graphene (MATTG) recently emerged as a highly tunable platform for studying correlated phases of matter, such as correlated insulators and superconductivity. Superconductivity occurs in a range of doping levels that is bounded by van Hove singularities which stimulates the debate of the origin and nature of superconductivity in this material. In this work, we discuss the role of spin-fluctuations arising from atomic-scale correlations in MATTG for the superconducting state. We show that in a phase diagram as function of doping ($ u$) and temperature, nematic superconducting regions are surrounded by ferromagnetic states and that a superconducting dome with $T_c approx 2,mathrm{K}$ appears between the integer fillings $ u =-2$ and $ u = -3$. Applying a perpendicular electric field enhances superconductivity on the electron-doped side which we relate to changes in the spin-fluctuation spectrum. We show that the nematic unconventional superconductivity leads to pronounced signatures in the local density of states detectable by scanning tunneling spectroscopy measurements.
Magic-angle twisted bilayer graphene (TBG), with rotational misalignment close to 1.1$^circ$, features isolated flat electronic bands that host a rich phase diagram of correlated insulating, superconducting, ferromagnetic, and topological phases. The origins of the correlated insulators and superconductivity, and the interplay between them, are particularly elusive. Both states have been previously observed only for angles within $pm0.1^circ$ from the magic-angle value and occur in adjacent or overlapping electron density ranges; nevertheless, it is still unclear how the two states are related. Beyond the twist angle and strain, the dependence of the TBG phase diagram on the alignment and thickness of insulating hexagonal boron nitride (hBN) used to encapsulate the graphene sheets indicates the importance of the microscopic dielectric environment. Here we show that adding an insulating tungsten-diselenide (WSe$_2$) monolayer between hBN and TBG stabilizes superconductivity at twist angles much smaller than the established magic-angle value. For the smallest angle of $theta$ = 0.79$^circ$, we still observe clear superconducting signatures, despite the complete absence of the correlated insulating states and vanishing gaps between the dispersive and flat bands. These observations demonstrate that, even though electron correlations may be important, superconductivity in TBG can exist even when TBG exhibits metallic behaviour across the whole range of electron density. Finite-magnetic-field measurements further reveal breaking of the four-fold spin-valley symmetry in the system, consistent with large spin-orbit coupling induced in TBG via proximity to WSe$_2$. Our results highlight the importance of symmetry breaking effects in stabilizing electronic states in TBG and open new avenues for engineering quantum phases in moire systems.
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