No Arabic abstract
We develop the theory of propagation of laser wave in a gas of two-level atoms (with an optical transition frequency $omega^{}_0$) under the condition of inhomogeneous Doppler broadening, considering the self-consistent solution of the Maxwell-Bloch equations in the mean-field approximation and for one-atomic density matrix. The nonlinear effects in the atomic density $n$, caused by the free motion of atoms, are found. These effects distort the lineshape (shift, asymmetry, broadening), but are not associated with atom-atom interaction. Moreover, in the case $nk^{-3}_0<1$ (where $k^{}_0=omega^{}_0/c$) and temperatures $Tgtrsim 300$~K, these quasi-collective effects exceed the well-known influence of the dipole-dipole interatomic interaction (e.g., Lorentz-Lorenz shift) by more than one order of magnitude. It was also found that for some area of parameters, the frequency interval appears, within which the non-trivial self-consistent solution of the Maxwell-Bloch equations is absent at all. Thus, the physical picture of collective effects in a gas medium should be substantially revised.
Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra-violet) -- IR (infrared) measurement, the XUV photon energy is scanned between SI{20.4}{electronvolt} and the ionization threshold at SI{24.6}{electronvolt}, revealing electric dipole-forbidden transitions for a temporally overlapping IR pulse ($sim!SI{e12}{wattper centimetersquared}$). The interpretation of the experimental results is supported by numerically solving the time-dependent Schrodinger equation in a single-active-electron approximation.
In dense atomic gases the interaction between transition dipoles and photons leads to the formation of many-body states with collective dissipation and long-ranged forces. Despite decades of research, a full understanding of this paradigmatic many-body problem is still lacking. Here, we put forward and explore a scenario in which a dense atomic gas is weakly excited by an off-resonant laser field. We develop the theory for describing such dressed many-body ensembles and show that collective excitations are responsible for the emergence of many-body interactions, i.e. effective potentials that cannot be represented as a sum of binary terms. We illustrate how interaction effects may be probed through microwave spectroscopy via the analysis of time-dependent line-shifts, and show that these signals are sensitive to the phase pattern of the dressing laser. Our study offers a new perspective on dense atomic ensembles interacting with light and promotes this platform as a setting for the exploration of rich non-equilibrium many-body physics.
An atom moving in a spatially periodic field experiences a temporary periodic perturbation and undergoes a resonance transition between atomic internal states when the transition frequency is equal to the atomic velocity divided by the field period. We demonstrated that spin nutation was induced by this resonant transition in a polarized rubidium (Rb) atomic beam passing through a magnetic lattice. The lattice was produced by current flowing through an array of parallel wires crossing the beam. This array structure, reminiscent of a multiwire chamber for particle detection, allowed the Rb beam to pass through the lattice at a variety of incident angles. The dephasing of spin nutation was reduced by varying the incident angle.
We investigate collective emission from coherently driven ultracold $ ^{88} $ Sr atoms. We perform two sets of experiments, using a strong and weak transition that are insensitive and sensitive, respectively, to atomic motion at one microKelvin. We observe highly directional forward emission with a peak intensity that is enhanced, for the strong transition, by > $ 10 ^3 $ compared to that in the transverse direction. This is accompanied by substantial broadening of spectral lines. For the weak transition, the forward enhancement is substantially reduced due to motion. Meanwhile, a density-dependent frequency shift of the weak transition (~10% of the natural linewidth) is observed. In contrast, this shift is suppressed to <1% of the natural linewidth for the strong transition. Along the transverse direction, we observe strong polarization dependences of the fluorescence intensity and line broadening for both transitions. The measurements are reproduced with a theoretical model treating the atoms as coherent, interacting, radiating dipoles.
Cooperative scattering has been the subject of intense research in the last years. In this article, we discuss the concept of cooperative scattering from a broad perspective. We briefly review the various collective effects that occur when light interacts with an ensemble of atoms. We show that some effects that have been recently discussed in the context of single-photon superradiance, or cooperative scattering in the linear-optics regime, can also be explained by standard optics, i.e., using macroscopic quantities such as the susceptibility or the diffusion coefficient. We explain why some collective effects depend on the atomic density, and others on the optical depth. In particular, we show that, for a large and dilute atomic sample driven by a far-detuned laser, the decay of the fluorescence, which exhibits superradiant and subradiant dynamics, depends only on the on-resonance optical depth. We also discuss the link between concepts that are independently studied in the quantum-optics community and in the mesoscopic-physics community. We show that the coupled-dipole model predicts a departure from Ohms law for the diffuse light, that incoherent multiple scattering can induce a saturation of fluorescence and we also show the similarity between the weak-localization correction to the diffusion coefficient and the inaccuracy of Lorentz local field correction to the susceptibility.