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Register a new userUnconventional rheological properties in systems of deformable particles
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We demonstrate the existence of unconventional rheological and memory properties in systems of soft-deformable particles whose energy depends on their shape, via numerical simulations. At large strains, these systems experience an unconventional shear weakening transition characterized by an increase in the mechanical energy and a drastic drop in shear stress, which stems from the emergence of short-ranged tetratic order. In these weakened states, the contact network evolves reversibly under strain reversal, keeping memory of its initial state, while the microscopic dynamics is irreversible.
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We investigate the structural, vibrational, and mechanical properties of jammed packings of deformable particles with shape degrees of freedom in three dimensions (3D). Each 3D deformable particle is modeled as a surface-triangulated polyhedron, with spherical vertices whose positions are determined by a shape-energy function with terms that constrain the particle surface area, volume, and curvature, and prevent interparticle overlap. We show that jammed packings of deformable particles without bending energy possess low-frequency, quartic vibrational modes, whose number decreases with increasing asphericity and matches the number of missing contacts relative to the isostatic value. In contrast, jammed packings of deformable particles with non-zero bending energy are isostatic in 3D, with no quartic modes. We find that the contributions to the eigenmodes of the dynamical matrix from the shape degrees of freedom are significant over the full range of frequency and shape parameters for particles with zero bending energy. We further show that the ensemble-averaged shear modulus $langle G rangle$ scales with pressure $P$ as $langle G rangle sim P^{beta}$, with $beta approx 0.75$ for jammed packings of deformable particles with zero bending energy. In contrast, $beta approx 0.5$ for packings of deformable particles with non-zero bending energy, which matches the value for jammed packings of soft, spherical particles with fixed shape. These studies underscore the importance of incorporating particle deformability and shape change when modeling the properties of jammed soft materials.
We discuss in this work the validity of the theoretical solution of the nonlinear Couette flow for a granular impurity obtained in a recent work [preprint arXiv:0802.0526], in the range of large inelasticity and shear rate. We show there is a good agreement between the theoretical solution and Monte Carlo simulation data, even under these extreme conditions. We also discuss an extended theoretical solution that would work for large inelasticities in ranges of shear rate $a$ not covered by our previous work (i.e., below the threshold value $a_{th}$ for which uniform shear flow may be obtained) and compare also with simulation data. Preliminary results in the simulations give useful insight in order to obtain an exact and general solution of the nonlinear Couette flow (both for $age a_{th}$ and $a<a_{th}$).
The soft-disk model previously developed and applied by Durian [D. J. Durian, Phys. Rev. Lett. 75, 4780 (1995)] is brought to bear on problems of foam rheology of longstanding and current interest, using two-dimensional systems. The questions at issue include the origin of the Herschel-Bulkley relation, normal stress effects (dilatancy), and localization in the presence of wall drag. We show that even a model that incorporates only linear viscous effects at the local level gives rise to nonlinear (power-law) dependence of the limit stress on strain rate. With wall drag, shear localization is found. Its nonexponential form and the variation of localization length with boundary velocity are well described by a continuum model in the spirit of Janiaud et al. [Phys. Rev. Lett. 97, 038302 (2006)]. Other results satisfactorily link localization to model parameters, and hence tie together continuum and local descriptions.
Different from previous modelings of self-propelled particles, we develop a method to propel the particles with a constant average velocity instead of a constant force. This constant propulsion velocity (CPV) approach is validated by its agreement with the conventional constant propulsion force (CPF) approach in the flowing regime. However, the CPV approach shows its advantage of accessing quasistatic flows of yield stress fluids with a vanishing propulsion velocity, while the CPF approach is usually unable to because of finite system size. Taking this advantage, we realize the cyclic self-propulsion and study the evolution of the propulsion force with propelled particle displacement, both in the quasistatic flow regime. By mapping shear stress and shear rate to propulsion force and propulsion velocity, we find similar rheological behaviors of self-propelled systems to sheared systems, including the yield force gap between the CPF and CPV approaches, propulsion force overshoot, reversible-irreversible transition under cyclic propulsion, and propulsion bands in plastic flows. These similarities suggest the underlying connections between self-propulsion and shear, although they act on systems in different ways.
We study a simple scalar constitutive equation for a shear-thickening material at zero Reynolds number, in which the shear stress sigma is driven at a constant shear rate dotgamma and relaxes by two parallel decay processes: a nonlinear decay at a nonmonotonic rate R(sigma_1) and a linear decay at rate lambdasigma_2. Here sigma_{1,2}(t) = tau_{1,2}^{-1}int_0^tsigma(t)exp[-(t-t)/tau_{1,2}] {rm d}t are two retarded stresses. For suitable parameters, the steady state flow curve is monotonic but unstable; this arises when tau_2>tau_1 and 0>R(sigma)>-lambda so that monotonicity is restored only through the strongly retarded term (which might model a slow evolution of material structure under stress). Within the unstable region we find a period-doubling sequence leading to chaos. Instability, but not chaos, persists even for the case tau_1to 0. A similar generic mechanism might also arise in shear thinning systems and in some banded flows.
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