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Register a new userRobust topological state against magnetic impurities observed in superconductor PbTaSe2
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Magnetic impurities deposited on topological superconductor candidate PbTaSe2 can introduce a non-splitting zero-energy state inside the superconducting gap, which has been proposed as a field-free platform for topological zero modes. However, it is still unclear how robust the topological state in PbTaSe2 is against magnetic impurities, which is related to the topological nature of the zero-energy state as well as its potential for quantum computation. In this work, we use scanning tunneling microscopy (STM) to study the topological surface state in the normal state of PbTaSe2 under the perturbation of magnetic impurities. We visualize the quasi-particle interference (QPI) arising from the topological surface state. We then deposit Fe impurities on the surface to form atomic Fe adatoms. We find that each Fe adatom sits at a unique interstitial position on the surface and features a local state at high energies, both of which are consistent with our first-principles calculation that further reveals its large magnetic moment. Our systematic Fe deposition and subsequent measurements show that the arc-like QPI pattern at the Fermi energy is robust with up to 3% Fe coverage where the atomic nature of Fe adatoms still holds. Our results provide evidence that the topological surface state at the Fermi energy in PbTaSe2 is robust against dilute magnetic impurities.
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A notable characteristic of PbTaSe$_2$, a prototypical noncentrosymmetric (NCS) superconductor, is that its superconductivity can be modulated through a structural transition under hydrostatic pressure [Phys. Rev. B 95, 224508 (2017)]. Here we report on simultaneous pressure-sensitive point-contact Andreev reflection (PCAR) spectroscopy and bulk resistance measurements on PbTaSe$_2$, to elucidate the nature of the surface and bulk superconductivity and their evolution with hydrostatic pressure. It is found that in high pressure region the superconducting gap opening temperature $T_c^A$ is significantly lower that the bulk resistive transition temperature $T_c^R$, revealing a clear experimental signature of surface-bulk separation associated with enhanced antisymmetric spin-orbit coupling (ASOC). The PCAR spectra, reflecting the superconducting surface state, are analyzed with the Blonder-Tinkham-Klapwijk theory, yielding an isotropic $s$-wave full BCS-gap in the strong coupling regime. Analysis based on a modified McMillan formula indicates a sizable coupling strength contributed from ASOC for the superconducting surface state. These results suggest the coexistence of full gap $s$-wave superconductivity and topological surface states in PbTaSe$_2$, indicating that this NSC with significantly enhanced ASOC may offer a solid platform to investigate the topological aspect in the superconducting condensate.
In superconductors, the condensation of Cooper pairs gives rise to fluxoid quantization in discrete units of $Phi_0 = hc / 2e$. The denominator of $2e$ is the signature of electron pairing, which is evidenced by a number of macroscopic quantum phenomena, such as the Little-Parks effect and the Josephson effect, where the critical temperature or the critical current oscillates in the period of $Phi_0$. Here we report the observation of fractional Little-Parks effect in mesoscopic rings of epitaxial $beta$-Bi$_2$Pd, a topological superconductor. Besides $Phi_0$, novel Little-Parks oscillation periodicities of $2Phi_0$, $3Phi_0$ and $4Phi_0$ are also observed, implying quasiparticles with effective charges being a fraction of a Cooper pair. We show that the fractional Little-Parks effect may be closely related to the fractional Josephson effect, which is a key signature of chiral Majorana edge states.
Spontaneous symmetry breaking has been a paradigm to describe the phase transitions in condensed matter physics. In addition to the continuous electromagnetic gauge symmetry, an unconventional superconductor can break discrete symmetries simultaneously, such as time reversal and lattice rotational symmetry. In this work we report a characteristic in-plane 2-fold behaviour of the resistive upper critical field and point-contact spectra on the superconducting semimetal PbTaSe2 with topological nodal-rings, despite its hexagonal lattice symmetry (or D_3h in bulk while C_3v on surface, to be precise). However, we do not observe any lattice rotational symmetry breaking signal from field-angle-dependent specific heat. It is worth noting that such surface-only electronic nematicity is in sharp contrast to the observation in the topological superconductor candidate, CuxBi2Se3, where the nematicity occurs in various bulk measurements. In combination with theory, superconducting nematicity is likely to emerge from the topological surface states of PbTaSe2, rather than the proximity effect. The issue of time reversal symmetry breaking is also addressed. Thus, our results on PbTaSe2 shed new light on possible routes to realize nematic superconductivity with nontrivial topology.
In a magnetic field, superconductivity is manifested by total magnetic field expulsion (Meissner effect) or by the penetration of integer multiples of the flux quantum {Phi}_0. Here we present experimental results revealing magnetic dipoles formed by Meissner current flowing around artificially introduced topological defects (lattice of antidots). By using scanning Hall probe microscopy, we have detected ordered magnetic dipole lattice generated at spatially periodic antidots in a Pb superconducting film. While the conventional homogeneous Meissner state breaks down, the total magnetic flux of the magnetic dipoles remains quantized and is equal to zero. The observed magnetic dipoles strongly depend on the intensity and direction of the locally flowing Meissner current, making the magnetic dipoles an effective way to monitor the local supercurrent. We have also investigated the first step of the vortex depinning process, where, due to the generation of magnetic dipoles, the pinned Abrikosov vortices are deformed and shifted from their original pinning sites.
We report on the observation of bulk superconductivity from dc magnetization measurements in a cylindrical single crystal of CuxBi2Se3. The magnitude of the magnetization in the Meissner state is very small and the magnetic-field dependence of the magnetization just above the lower critical field Hc1 is very different from those of usual type-II superconductors. We studied the character of the vortex state theoretically in a spin-triplet pairing superconductor and compared it with the experimental results. The results showed that, the superconductivity observed in CuxBi2Se3 is consistent with the spin-triplet pairing superconductivity with odd parity. We also observed a rapid relaxation phenomenon of the superconducting diamagnetism.
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