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Register a new userChemistry of a light impurity in a Bose-Einstein condensate
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In ultracold atomic gases, a unique interplay arises between phenomena known from condensed matter physics, few-body physics and chemistry. Similar to an electron in a solid, an impurity in an ultracold gas can get dressed by excitations from the medium, forming a quasiparticle called the polaron. We study how dressing of an impurity leads to a modification of its chemical reactivity. Using a Gaussian state variational method in the frame of the impurity, we demonstrate that three-body correlations lead to an instability of the polaron. This instability is connected to an Efimov resonance, but shifted to smaller interactions by many-body effects, showing that polaron formation stimulates Efimov physics and the associated chemistry.
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We compare and contrast the mean-field and many-body properties of a Bose-Einstein condensate trapped in a double well potential with a single impurity atom. The mean-field solutions display a rich structure of bifurcations as parameters such as the boson-impurity interaction strength and the tilt between the two wells are varied. In particular, we study a pitchfork bifurcation in the lowest mean-field stationary solution which occurs when the boson-impurity interaction exceeds a critical magnitude. This bifurcation, which is present for both repulsive and attractive boson-impurity interactions, corresponds to the spontaneous formation of an imbalance in the number of particles between the two wells. If the boson-impurity interaction is large, the bifurcation is associated with the onset of a Schroedinger cat state in the many-body ground state. We calculate the coherence and number fluctuations between the two wells, and also the entanglement entropy between the bosons and the impurity. We find that the coherence can be greatly enhanced at the bifurcation.
We investigate a Bose-Einstein condensate in strong interaction with a single impurity particle. While this situation has received considerable interest in recent years, the regime of strong coupling remained inaccessible to most approaches due to an instability in Bogoliubov theory arising near the resonance. We present a nonlocal extension of Gross-Pitaevskii theory that is free of such divergences and does not require the use of the Born approximation in any of the interaction potentials. We find a new dynamical transition regime between attractive and repulsive polarons, where an interaction quench results in a finite number of coherent oscillations in the density profiles of the medium and in the contact parameter before equilibrium is reached.
We analyze the properties of an impurity in a dilute Bose-Einstein condensate (BEC). First the quasiparticle residue of a static impurity in an ideal BEC is shown to vanish with increasing particle number as a stretched exponential, leading to a bosonic orthogonality catastrophe. Then we introduce a variational ansatz, which recovers this exact result and describes the macroscopic dressing of the impurity including its back-action onto the BEC as well as boson-boson repulsion beyond the Bogoliubov approximation. This ansatz predicts that the orthogonality catastrophe also occurs for mobile impurities, whenever the BEC becomes ideal. Finally, we show that our ansatz agrees well with experimental results.
The variational Feynman formalism for the polaron, extended to an all-coupling treatment of bipolarons, is applied for two impurity atoms in a Bose-Einstein condensate. This shows that if the polaronic coupling strength is large enough the impurities will form a bound state (the bipolaron). As a function of the mutual repulsion between the impurities two types of bipolaron are distinguished: a tightly bound bipolaron at weak repulsion and a dumbbell bipolaron at strong repulsion. Apart from the binding energy, also the evolution of the bipolaron radius and its effective mass are examined as a function of the strength of the repulsive interaction between the impurities and of the polaronic cupling strength. We then apply the strong-coupling formalism to multiple impuritiy atoms in a condensate which leads to the prediction of multi-polaron formation in the strong coupling regime. The results of the two formalisms are compared for two impurities in a condensate which results in a general qualitative agreement and a quantitative agreement at strong coupling. Typically the system of impurity atoms in a Bose-Einstein condensate is expected to exhibit the polaronic weak coupling regime. However, the polaronic coupling strength is in principle tunable with a Feshbach resonance.
Mobile impurities in a Bose-Einstein condensate form quasiparticles called polarons. Here, we show that two such polarons can bind to form a bound bipolaron state. Its emergence is caused by an induced nonlocal interaction mediated by density oscillations in the condensate, and we derive using field theory an effective Schrodinger equation describing this for arbitrarily strong impurity-boson interaction. We furthermore compare with Quantum Monte Carlo simulations finding remarkable agreement, which underlines the predictive power of the developed theory. It is found that bipolaron formation typically requires strong impurity interactions beyond the validity of more commonly used weak-coupling approaches that lead to local Yukawa-type interactions. We predict that the bipolarons are observable in present experiments and describe a procedure to probe their properties.
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