No Arabic abstract
Magnetic state of exchanged biased CoO(20nm)/Co($d_F$) bilayer ($d_F$=5-20nm) was studied by means of polarized neutron reflectometry. By spacing of CoO/Co bilayer and Al$_2$O$_3$ substrate with Nb(20nm) layer we created waveguide structure which allowed us to significantly enhance intensity of spin-flip (SF) scattering in the position of optical resonances. For the trained sample with thinnest Co(5nm) we detected strong SF scattering at the resonance position (up to 30% of incoming intensity) speaking about high non-collinearity of the system. As $d_F$ increases, the intensity of SF scattering linearly decreases. At the same time we observed asymmetry of up-down and down-up scattering channels at the resonance positions. We attribute this asymmetry to the Zeeman splitting of neutrons energies with different initial polarization taking place in high external field. Analysis, however, shows that the applied in the PNR experiment external field is not enough to quantitatively explain the observed asymmetry for the samples with $d_F > $ 5nm and we have to postulate presence of additional magnetic field produced by sample. We attribute this additional field to the stray field produced by chiral Bloch domain walls. The chirality of the domain walls can be explained by Dzyaloshinskii-Moriya interaction arising at the CoO/Co interface. Our results can be useful for designing of spintronic devices using exchange bias effect.
We performed non-local electrical measurements of a series of Py/Cu lateral spin valve devices with different Cu thicknesses. We show that both the spin diffusion length of Cu and the apparent spin polarization of Py increase with Cu thickness. By fitting the results to a modified spin-diffusion model, we show that the spin diffusion length of Cu is dominated by spin-flip scattering at the surface. In addition, the dependence of spin polarization of Py on Cu thickness is due to a strong spin-flip scattering at the Py/Cu interface.
A magnetic helix arises in chiral magnets with a wavelength set by the spin-orbit coupling. We show that the helimagnetic order is a nanoscale analog to liquid crystals, exhibiting topological structures and domain walls that are distinctly different from classical magnets. Using magnetic force microscopy and micromagnetic simulations, we demonstrate that - similar to cholesteric liquid crystals - three fundamental types of domain walls are realized in the helimagnet FeGe. We reveal the micromagnetic wall structure and show that they can carry a finite skyrmion charge, permitting coupling to spin currents and contributions to a topological Hall effect. Our study establishes a new class of magnetic nano-objects with non-trivial topology, opening the door to innovative device concepts based on helimagnetic domain walls.
The magnetic properties of CuO encompass several contemporary themes in condensed matter physics, including quantum magnetism, magnetic frustration, magnetically-induced ferroelectricity and orbital currents. Here we report polarized and unpolarized neutron inelastic scattering measurements which provide a comprehensive map of the cooperative spin dynamics in the low temperature antiferromagnetic (AFM) phase of CuO throughout much of the Brillouin zone. At high energies ($E gtrsim 100$,meV) the spectrum displays continuum features consistent with the des Cloizeax--Pearson dispersion for an ideal $S=frac{1}{2}$ Heisenberg AFM chain. At lower energies the spectrum becomes more three-dimensional, and we find that a linear spin-wave model for a Heisenberg AFM provides a very good description of the data, allowing for an accurate determination of the relevant exchange constants in an effective spin Hamiltonian for CuO. In the high temperature helicoidal phase, there are features in the measured low-energy spectrum that we could not reproduce with a spin-only model. We discuss how these might be associated with the magnetically-induced multiferroic behavior observed in this phase.
The utility of nanoscaled ferromagnetic particles requires both stabilized moments and maximized switching speeds. During reversal, the spatial modulation of the nanoparticle magnetization evolves in time, and the energy differences between each new configuration are accomodated by the absorption or emission spin waves with different wavelengths and energy profiles. The switching speed is limited by how quickly this spin wave energy is dissipated. We present here the first observation of dispersing spin waves in a nanoscaled system, using neutron scattering to detect spin waves in the CoO shells of exchange biased Co core- CoO shell nanoparticles. Their dispersion is little affected by finite size effects, but the spectral weight shifts to energies and wave vectors which increase with decreasing system size. Core-shell coupling leads to a substantial enhancement of the CoO spin wave population above its conventional thermal level, suggesting a new mechanism for dissipating core switching energy.
The Q dependence of the inelastic neutron scattering (INS) intensity of transitions within the ground-state spin multiplet of single-molecule magnets (SMMs) is considered. For these transitions, the Q dependence is related to the spin density map in the ground state, which in turn is governed by the Heisenberg exchange interactions in the cluster. This provides the possibility to infer the exchange-coupling constants from the Q dependence of the INS transitions within the spin ground state. The potential of this strategy is explored for the M = +-10 -> +- 9 transition within the S = 10 multiplet of the molecule Mn12 as an example. The Q dependence is calculated for powder as well as single-crystal Mn12 samples for various exchange-coupling situations discussed in the literature. The results are compared to literature data on a powder sample of Mn12 and to measurements on an oriented array of about 500 single-crystals of Mn12. The calculated Q dependence exhibits significant variation with the exchange-coupling constants, in particular for a single-crystal sample, but the experimental findings did not permit an unambiguous determination. However, although challenging, suitable experiments are within the reach of todays instruments.