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Register a new userContinuous-Wave Frequency Upconversion with a Molecular Optomechanical Nanocavity
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Frequency upconversion is a cornerstone of electromagnetic signal processing, analysis and detection. It is used to transfer energy and information from one frequency domain to another where transmission, modulation or detection is technically easier or more efficient. Optomechanical transduction is emerging as a flexible approach to coherent frequency upconversion; it has been successfully demonstrated for conversion from radio- and microwaves (kHz to GHz) to optical fields. Nevertheless, optomechanical transduction of multi-THz and mid-infrared signals remains an open challenge. Here, we utilize molecular cavity optomechanics to demonstrate upconversion of sub-microwatt continuous-wave signals at $sim$32~THz into the visible domain at ambient conditions. The device consists in a plasmonic nanocavity hosting a small number of molecules. The incoming field resonantly drives a collective molecular vibration, which imprints an optomechanical modulation on a visible pump laser and results in Stokes and anti-Stokes upconverted Raman sidebands with sub-natural linewidth, indicating a coherent process. The nanocavity offers 13 orders of magnitude enhancement of upconversion efficiency per molecule compared to free space, with a measured phonon-to-photon internal conversion efficiency larger than $10^{-4}$ per milliwatt of pump power. Our results establish a flexible paradigm for optomechanical frequency conversion using molecular oscillators coupled to plasmonic nanocavities, whose vibrational and electromagnetic properties can be tailored at will using chemical engineering and nanofabrication.
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The mechanical properties of light have found widespread use in the manipulation of gas-phase atoms and ions, helping create new states of matter and realize complex quantum interactions. The field of cavity-optomechanics strives to scale this interaction to much larger, even human-sized mechanical objects. Going beyond the canonical Fabry-Perot cavity with a movable mirror, here we explore a new paradigm in which multiple cavity-optomechanical elements are wired together to form optomechanical circuits. Using a pair of optomechanical cavities coupled together via a phonon waveguide we demonstrate a tunable delay and filter for microwave-over-optical signal processing. In addition, we realize a tight-binding form of mechanical coupling between distant optomechanical cavities, leading to direct phonon exchange without dissipation in the waveguide. These measurements indicate the feasibility of phonon-routing based information processing in optomechanical crystal circuitry, and further, to the possibility of realizing topological phases of photons and phonons in optomechanical cavity lattices.
Electromagnetically induced transparency has great theoretical and experimental importance in many physics subjects, such as atomic physics, quantum optics, and more recent cavity optomechanics. Optical delay is the most prominent feature of electromagnetically induced transparency, and in cavity optomechanics optical delay is limited by mechanical dissipation rate of sideband-resolved mechanical modes. Here we demonstrate a cascaded optical transparency scheme by leveraging the parametric phonon-phonon coupling in a multimode optomechanical system, where a low damping mechanical mode in the unresolved-sideband regime is made to couple to an intermediate, high frequency mechanical mode in the resolved-sideband regime of an optical cavity. Extended optical delay and higher transmission, as well as optical advancing are demonstrated. These results provide a route to realize ultra-long optical delay, indicating a significant step toward integrated classical and quantum information storage devices.
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