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Identifying intrinsic and extrinsic mechanisms of anisotropic magnetoresistance with terahertz probes

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 Added by Kab-Jin Kim
 Publication date 2021
  fields Physics
and research's language is English




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Identifying the intrinsic and extrinsic origins of magneto-transport in spin-orbit coupled systems has long been a central theme in condensed matter physics. However, it has been elusive owing to the lack of an appropriate experimental tool. In this work, using terahertz time-domain spectroscopy, we unambiguously disentangle the intrinsic and extrinsic contributions to the anisotropic magnetoresistance (AMR) of a permalloy film. We find that the scattering-independent intrinsic contribution to AMR is sizable and is as large as the scattering-dependent extrinsic contribution to AMR. Moreover, the portion of intrinsic contribution to total AMR increases with increasing temperature due to the reduction of extrinsic contribution. Further investigation reveals that the reduction of extrinsic contribution is caused by the phonon/magnon-induced negative AMR. Our result will stimulate further researches on other spin-orbit-interaction-induced phenomena for which identifying the intrinsic and extrinsic contributions is important.



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Anisotropic magnetoresistance (AMR) is a ubiquitous and versatile probe of magnetic order in contemporary spintronics research. Its origins are usually ascribed to extrinsic effects (i.e. spin-dependent electron scattering), whereas intrinsic (i.e. scattering-independent) contributions are neglected. Here, we measure AMR of polycrystalline thin films of the standard ferromagnets Co, Ni, Ni81Fe19 and Ni50Fe50 over the frequency range from DC to 28 THz. The large bandwidth covers the regimes of both diffusive and ballistic intraband electron transport and, thus, allows us to separate extrinsic and intrinsic AMR components. Analysis of the THz response based on Boltzmann transport theory reveals that the AMR of the Ni, Ni81Fe19 and Ni50Fe50 samples is of predominantly extrinsic nature. However, the Co thin film exhibits a sizeable intrinsic AMR contribution, which is constant up to 28 THz and amounts to more than 2/3 of the DC AMR contrast of 1%. These features are attributed to the hexagonal structure of the Co crystallites. They are interesting for applications in terahertz spintronics and terahertz photonics. Our results show that broadband terahertz electromagnetic pulses provide new and contact-free insights into magneto-transport phenomena of standard magnetic thin films on ultrafast time scales.
Chiral anomaly induced negative magnetoresistance (NMR) has been widely used as a critical transport evidence on the existence of Weyl fermions in topological semimetals. In this mini review, we discuss the general observation of the NMR phenomena in non-centrosymmetric NbP and NbAs. We show that NMR can be contributed by intrinsic chiral anomaly of Weyl fermions and/or extrinsic effects, such as superimposition of Hall signals, field-dependent inhomogeneous current flow in the bulk, i.e. current jetting, and weak localization (WL) of coexistent trivial carriers. Such WL controlled NMR is heavily dependent on sample quality, and is characterized by pronounced crossover from positive to negative MR growth at elevated temperatures, as a result of the competition between the phase coherence time and the spin-orbital scattering constant of the bulk trivial pockets. Thus, the correlation of NMR and chiral anomaly needs to be scrutinized, without the support of other complimentary techniques. Due to the lifting of spin degeneracy, the spin orientations of Weyl fermions are either parallel or antiparallel to the momentum, a unique physical property known as helicity. The conservation of helicity provides strong protection for the transport of Weyl fermions, which can only be effectively scattered by magnetic impurities. Chemical doping of magnetic and non-magnetic impurities are thus more convincing in probing the existence of Weyl fermions than the NMR method.
It is a well established fact that some YSO jets (e.g. RW Aur) display different propagation speeds between their blue and red shifted parts, a feature possibly associated with the central engine or the environment in which the jet propagates. In order to understand the origin of asymmetric YSO jet velocities, we investigate the efficiency of two candidate mechanisms, one based on the intrinsic properties of the system and one based on the role of the external medium. In particular, a parallel or anti-parallel configuration between the protostellar magnetosphere and the disk magnetic field is considered and the resulting dynamics are examined both in an ideal and a resistive magneto-hydrodynamical (MHD) regime. Moreover, we explore the effects of a potential difference in the pressure of the environment, as a consequence of the non-uniform density distribution of molecular clouds. Ideal and resistive axisymmetric numerical simulations are carried out for a variety of models, all of which are based on a combination of two analytical solutions, a disk wind and a stellar outflow. We find that jet velocity asymmetries can indeed occur both when multipolar magnetic moments are present in the star-disk system as well as when non-uniform environments are considered. The latter case is an external mechanism that can easily explain the large time scale of the phenomenon, whereas the former one naturally relates it to the YSO intrinsic properties. [abridged]
180 - J. H. Chen , C. Jang , S. Xiao 2007
The linear dispersion relation in graphene[1,2] gives rise to a surprising prediction: the resistivity due to isotropic scatterers (e.g. white-noise disorder[3] or phonons[4-8]) is independent of carrier density n. Here we show that acoustic phonon scattering[4-6] is indeed independent of n, and places an intrinsic limit on the resistivity in graphene of only 30 Ohm at room temperature (RT). At a technologically-relevant carrier density of 10^12 cm^-2, the mean free path for electron-acoustic phonon scattering is >2 microns, and the intrinsic mobility limit is 2x10^5 cm^2/Vs, exceeding the highest known inorganic semiconductor (InSb, ~7.7x10^4 cm^2/Vs[9]) and semiconducting carbon nanotubes (~1x10^5 cm^2/Vs[10]). We also show that extrinsic scattering by surface phonons of the SiO2 substrate[11,12] adds a strong temperature dependent resistivity above ~200 K[8], limiting the RT mobility to ~4x10^4 cm^2/Vs, pointing out the importance of substrate choice for graphene devices[13].
We examine magnetic relaxation in polycrystalline Fe films with strong and weak crystallographic texture. Out-of-plane ferromagnetic resonance (FMR) measurements reveal Gilbert damping parameters of $approx$ 0.0024 for Fe films with thicknesses of 4-25 nm, regardless of their microstructural properties. The remarkable invariance with film microstructure strongly suggests that intrinsic Gilbert damping in polycrystalline Fe is a local property of nanoscale crystal grains, with limited impact from grain boundaries and film roughness. By contrast, the in-plane FMR linewidths of the Fe films exhibit distinct nonlinear frequency dependences, indicating the presence of strong extrinsic damping. To fit our experimental data, we have used a grain-to-grain two-magnon scattering model with two types of correlation functions aimed at describing the spatial distribution of inhomogeneities in the film. However, neither of the two correlation functions is able to reproduce the experimental data quantitatively with physically reasonable parameters. Our finding points to the need to further examine the fundamental impact of film microstructure on extrinsic damping.
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