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Register a new userEnhanced lasing action and spontaneous emission in periodic plasmonic nanohole arrays
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Periodic arrays of air nanoholes in thin metal films that support surface plasmon resonances can provide an alternative approach for boosting the light-matter interactions at the nanoscale. Indeed, nanohole arrays have garnered great interest in recent years for their use in biosensing, light emission enhancement and spectroscopy. However, the large-scale use of nanohole arrays in emerging technology requires new low-cost fabrication techniques. Here, we demonstrate a simple technique to fabricate nanohole arrays and examine their photonic applications. In contrast to the complicated and most commonly used electron beam lithography technique, hexagonal arrays of nanoholes are fabricated by using a simple combination of shadowing nanosphere lithography technique and electron beam deposition. These arrays are shown to offer enhancements in the lasing emission of an organic dye liquid gain medium with a quality factor above 150. Additionally, a 7-fold increase in Purcell factor is observed for CdSe quantum dot-integrated nanohole arrays.
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Prospects of using metal hole arrays for the enhanced optical detection of molecular chirality in nanosize volumes are investigated. Light transmission through the holes filled with an optically active material is modeled and the activity enhancement by more than an order of magnitude is demonstrated. The spatial resolution of the chirality detection is shown to be of a few tens of nanometers. From comparing the effect in arrays of cylindrical holes and holes of complex chiral shape, it is concluded that the detection sensitivity is determined by the plasmonic near field enhancement. The intrinsic chirality of the arrays due to their shape appears to be less important.
We report on lasing at visible wavelengths in arrays of ferromagnetic Ni nanodisks overlaid with an organic gain medium. We demonstrate that by placing an organic gain material within the mode volume of the plasmonic nanoparticles both the radiative and, in particular, the high ohmic losses of Ni nanodisk resonances can be compensated. Under increasing pump fluence, the systems exhibit a transition from lattice-modified spontaneous emission to lasing, the latter being characterized by highly directional and sub-nanometer linewidth emission. By breaking the symmetry of the array, we observe tunable multimode lasing at two wavelengths corresponding to the particle periodicity along the two principal directions of the lattice. Our results pave the way for loss-compensated magnetoplasmonic devices and topological photonics.
We experimentally realized an optical nanofiber-based cavity by combining a 1-D photonic crystal and Bragg grating structures. The cavity morphology comprises a periodic, triplex air-cube introduced at the waist of the nanofiber. The cavity has been theoretically characterized using FDTD simulations to obtain the reflection and transmission spectra. We have also experimentally measured the transmission spectra and a Q-factor of ~784(87) for a very short periodic structure has been observed. The structure provides strong confinement of the cavity field and its potential for optical network integration makes it an ideal candidate for use in nanophotonic and quantum information systems.
The ability to harness light-matter interactions at the few-photon level plays a pivotal role in quantum technologies. Single photons - the most elementary states of light - can be generated on-demand in atomic and solid state emitters. Two-photon states are also key quantum assets, but achieving them in individual emitters is challenging because their generation rate is much slower than competing one-photon processes. We demonstrate that atomically thin plasmonic nanostructures can harness two-photon spontaneous emission, resulting in giant far-field two-photon production, a wealth of resonant modes enabling tailored photonic and plasmonic entangled states, and plasmon-assisted single-photon creation orders of magnitude more efficient than standard one-photon emission. We unravel the two-photon spontaneous emission channels and show that their spectral line-shapes emerge from an intricate interplay between Fano and Lorentzian resonances. Enhanced two-photon spontaneous emission in two-dimensional nanostructures paves the way to an alternative efficient source of light-matter entanglement for on-chip quantum information processing and free-space quantum communications.
The photothermal energy conversion in hanging and floating polyaniline (PANi)-cotton fabrics is investigated using a model based on the heat diffusion equation. Perfect absorption and anti-reflection of wet hanging PANi-cotton fabrics cause quick transfer of total incident light into water confining nearly 100 $%$ of the sunlight. As a result, a hanging membrane is found to have more attractive properties than a floating above water fabric. We find, however, that the photothermal properties of a floating PANi-cotton membrane can greatly be enhanced by dispersing TiN nanoparticles in the water below the fabric. The calculated temperature gradients for TiN nanoparticle solutions show that the absorbed energy grows with increasing the nanoparticle density and that the photothermal process occurs mostly near the surface. The collective heating effects depend on the size and density of nanoparticles, which can further be used to modulate the photothermal process.
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