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Register a new userControlled plasmon-enhanced fluorescence by spherical microcavity
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A surrounding electromagnetic environment can engineer spontaneous emissions from quantum emitters through the Purcell effect. For instance, a plasmonic antenna can efficiently confine an electromagnetic field and enhance the fluorescent process. In this study, we demonstrate that a photonic microcavity can modulate plasmon-enhanced fluorescence by engineering the local electromagnetic environment. Consequently, we constructed a plasmon-enhanced emitter (PE-emitter), which comprised a nanorod and a nanodiamond, using the nanomanipulation technique. Furthermore, we controlled a polystyrene sphere approaching the PE-emitter and investigated in situ the associated fluorescent spectrum and lifetime. The emission of PE-emitter can be enhanced resonantly at the photonic modes as compared to that within the free spectral range. The spectral shape modulated by photonic modes is independent of the separation between the PS sphere and PE-emitter. The band integral of the fluorescence decay rate can be enhanced or suppressed after the PS sphere couples to the PE-emitters, depending on the coupling strength between the plasmonic antenna and the photonic cavity. These findings can be utilized in sensing and imaging applications.
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Interference patterns of surface plasmon polaritons(SPPs) are observed in the extraordinary optical transmission through subwavelength holes in optically thick metal plate. It is found that the phase of incident light can be transferred to SPPs. We can control the destructive and constructive interference of SPPs by modulating the relative phase between two incident beams. Using a slightly displaced Mach-Zehnder interferometer, we also observe a SPPs interference pattern composed of bright and dark stripes.
Mid-infrared photothermal microscopy is a new chemical imaging technology in which a visible beam senses the photothermal effect induced by a pulsed infrared laser. This technology provides infrared spectroscopic information at sub-micron spatial resolution and enables infrared spectroscopy and imaging of living cells and organisms. Yet, current mid-infrared photothermal imaging sensitivity suffers from a weak dependance of scattering on temperature and the image quality is vulnerable to the speckles caused by scattering. Here, we present a novel version of mid-infrared photothermal microscopy in which thermo-sensitive fluorescent probes are harnessed to sense the mid-infrared photothermal effect. The fluorescence intensity can be modulated at the level of 1% per Kelvin, which is 100 times larger than the modulation of scattering intensity. In addition, fluorescence emission is free of speckles, thus much improving the image quality. Moreover, fluorophores can target specific organelles or biomolecules, thus augmenting the specificity of photothermal imaging. Spectral fidelity is confirmed through fingerprinting a single bacterium. Finally, the photobleaching issue is successfully addressed through the development of a wide-field fluorescence-enhanced mid-infrared photothermal microscope which allows video rate bond-selective imaging of biological specimens.
Surface plasmon polaritons have attracted varies of interests due to its special properties, especially in the polarization-controlled devices. Typically, the polarization-controlled devices include directional coupling, focusing lens and plasmonic vortex lens, and almost all of them are controlled by the input circularly polarized light or the linearly polarized light. We present a novel device that realize the functions of directional coupling and focusing with high polarization extinction ratio for arbitrary spin of input light. This device offers opportunities for polarization sensing, polarization splitting and polarization-multiplexed near-field images and surface plasmon holography in the future.
A compact high repetition rate attosecond light source based on a standard laser oscillator combined with plasmonic enhancement is presented. At repetition rates of tens of MHz, we predict focusable pulses with durations of ~< 300 attoseconds, and collimation angles ~< 5 degrees. Attosecond pulse parameters are robust with respect variations of driver pulse focus and duration.
Controlling the directionality of surface plasmon polaritons (SPPs) has been widely studied, while the direction of SPPs was always switched by orthogonal polarizations in the reported methods. Here, we present a scheme to control the directionality of SPPs by arbitrary spin polarizations. Extremely, the device can split two quite adjacent polarization components to two opposite directions. The versatility of the presented design scheme can offer opportunities for polarization sensing, polarization splitting and polarization-controlled plasmonic devices.
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