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Register a new userDecoupled nematic and magnetic criticality in FeSe$_{1-x}$S$_{x}$
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Electronic nematicity in correlated metals often occurs alongside another instability such as magnetism. As a result, the question remains whether nematicity alone can drive unconventional superconductivity or anomalous (quantum critical) transport in such systems. In FeSe, nematicity emerges in isolation, providing a unique opportunity to address this question. Studies to date, however, have proved inconclusive; while signatures of nematic criticality are observed upon sulfur substitution, they appear to be quenched under the application of pressure due to the emergent magnetism. Here, we study the temperature and pressure dependence of the low-temperature resistivity of FeSe$_{1-x}$S$_{x}$ crystals at $x$ values just beyond the nematic quantum critical point. Two distinct components to the resistivity are revealed; one whose magnitude falls with increasing pressure and one which grows upon approaching the magnetic state at higher pressures. These findings indicate that nematic and magnetic critical fluctuations in FeSe$_{1-x}$S$_{x}$ are completely decoupled, in marked contrast to other Fe-based superconductors, and that nematic fluctuations alone may be responsible for the transport signatures of quantum criticality found in FeSe$_{1-x}$S$_{x}$ at ambient pressure.
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The interplay between the nematic order and magnetism in FeSe is not yet well understood. There is a controversy concerning the relationship between orbital and spin degrees of freedom in FeSe and their relevance for superconductivity. Here we investigate the effect of S substitution on the nematic transition temperature ($T_{rm n}$) and the low-energy spin fluctuations (SF) in FeSe single crystals. We show that the low-energy SF emerge below the nematic transition. The difference between the onset temperature for the critical SF ($T_{rm SF}$) and $T_{rm n}$ is small for FeSe but significantly increases with S substitution. Below $T_{rm SF}$ the Korringa relation is violated and the effective muon hyperfine coupling constant changes a sign. Our results exclude a direct coupling of the low-energy SF to the electronic nematic order indicating a presence of multiple spin degrees of freedom in FeSe$_{rm 1-x}$S$_{rm x}$.
In this paper we review some of our recent experimental and theoretical results on transport and thermodynamic properties of heavy-fermion alloys Ce(1-x)Yb(x)CoIn5. Charge transport measurements under magnetic field and pressure on these single crystalline alloys revealed that: (i) relatively small Yb substitution suppresses the field induced quantum critical point, with a complete suppression for nominal Yb doping x>0.20; (ii) the superconducting transition temperature Tc and Kondo lattice coherence temperature T* decrease with x, yet they remain finite over the wide range of Yb concentrations; (iii) both Tc and T* increase with pressure; (iv) there are two contributions to resistivity, which show different temperature and pressure dependences, implying that both heavy and light quasiparticles contribute to inelastic scattering. We also analyzed theoretically the pressure dependence of both T* and Tc within the composite pairing theory. In the purely static limit, when we ignore the lattice dynamics, we find that the composite pairing mechanism necessarily causes opposite behaviors of T* and Tc with pressure: if T* grows with pressure, Tc must decrease with pressure and vice versa.
We report the evolution of nematic fluctuations in FeSe$_{1-x}$S$_x$ single crystals as a function of Sulfur content $x$ across the nematic quantum critical point (QCP) $x_csim$ 0.17 via Raman scattering. The Raman spectra in the $B_{1g}$ nematic channel consist of two components, but only the low energy one displays clear fingerprints of critical behavior and is attributed to itinerant carriers. Curie-Weiss analysis of the associated nematic susceptibility indicates a substantial effect of nemato-elastic coupling which shifts the location of the nematic QCP. We argue that this lattice-induced shift likely explains the absence of any enhancement of the superconducting transition temperature at the QCP. The presence of two components in the nematic fluctuations spectrum is attributed to the dual aspect of electronic degrees of freedom in Hunds metals, with both itinerant carriers and local moments contributing to the nematic susceptibility.
We investigated the magnetic properties of (La$_{1-x}$Ba$_{x}$)(Zn$_{1-x}$Mn$_{x}$)AsO with $x$ varying from 0.005 to 0.05 at an external magnetic field of 1000 Oe. For doping levels of $x$ $leq$ 0.01, the system remains paramagnetic down to the lowest measurable temperature of 2 K. Only when the doping level increases to $x$ = 0.02 does the ferromagnetic ordering appear. Our analysis indicates that antiferromagnetic exchange interactions dominate for $x$ $leq$ 0.01, as shown by the negative Weiss temperature fitted from the magnetization data. The Weiss temperature becomes positive, i.e., ferromagnetic coupling starts to dominate, for $x$ $geq$ 0.02. The Mn-Mn spin interaction parameter $mid$$2J/k_B$$mid$ is estimated to be in the order of 10 K for both $x$ $leq$ 0.01 (antiferromagnetic ordered state) and $x$ $geq$ 0.02 (ferromagnetic ordered state). Our results unequivocally demonstrate the competition between ferromagnetic and antiferromagnetic exchange interactions in carrier-mediated ferromagnetic systems.
Understanding superconductivity requires detailed knowledge of the normal electronic state from which it emerges. A nematic electronic state that breaks the rotational symmetry of the lattice can potentially promote unique scattering relevant for superconductivity. Here, we investigate the normal transport of superconducting FeSe$_{1-x}$S$_x$ across a nematic phase transition using high magnetic fields up to 69 T to establish the temperature and field-dependencies. We find that the nematic state is an anomalous non-Fermi liquid, dominated by a linear resistivity at low temperatures that can transform into a Fermi liquid, depending on the composition $x$ and the impurity level. Near the nematic end point, we find an extended temperature regime with $T^{1.5}$ resistivity. The transverse magnetoresistance inside the nematic phase has as a $H^{1.55}$ dependence over a large magnetic field range and it displays an unusual peak at low temperatures inside the nematic phase. Our study reveals anomalous transport inside the nematic phase, driven by the subtle interplay between the changes in the electronic structure of a multi-band system and the unusual scattering processes affected by large magnetic fields and disorder
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