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Register a new userSpin-Orbit Coupled Exciton-Polariton Condensates in Lead Halide Perovskites
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Spin-orbit coupling (SOC) is responsible for a range of spintronic and topological processes in condensed matter. Here we show photonic analogs of SOCs in exciton-polaritons and their condensates in microcavities composed of birefringent lead halide perovskite single crystals. The presence of crystalline anisotropy coupled with splitting in the optical cavity of the transverse electric (TE) and transverse magnetic (TM) modes gives rise to a non-Abelian gauge field, which can be described by the Rashba-Dresselhaus Hamiltonian near the degenerate points of the two polarization modes. With increasing density, the exciton polaritons with pseudospin textures undergo phase transitions to competing condensates with orthogonal polarizations. These condensates inherit strong nonlinearity from their excitonic components and may serve as quantum simulators of many-body SOC processes.
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Recently a new type of system exhibiting spontaneous coherence has emerged -- the exciton-polariton condensate. Exciton-polaritons (or polaritons for short) are bosonic quasiparticles that exist inside semiconductor microcavities, consisting of a superposition of an exciton and a cavity photon. Above a threshold density the polaritons macroscopically occupy the same quantum state, forming a condensate. The lifetime of the polaritons are typically comparable to or shorter than thermalization times, making them possess an inherently non-equilibrium nature. Nevertheless, they display many of the features that would be expected of equilibrium Bose-Einstein condensates (BECs). The non-equilibrium nature of the system raises fundamental questions of what it means for a system to be a BEC, and introduces new physics beyond that seen in other macroscopically coherent systems. In this review we focus upon several physical phenomena exhibited by exciton-polariton condensates. In particular we examine topics such as the difference between a polariton BEC, a polariton laser, and a photon laser, as well as physical phenomena such as superfluidity, vortex formation, BKT (Berezinskii-Kosterlitz-Thouless) and BCS (Bardeen-Cooper-Schrieffer) physics. We also discuss the physics and applications of engineered polariton structures.
We introduce the phenomenon of spiraling vortices in driven-dissipative (non-equilibrium) exciton-polariton condensates excited by a non-resonant pump beam. At suitable low pump intensities, these vortices are shown to spiral along circular trajectories whose diameter is inversely proportional to the effective mass of the polaritons, while the rotation period is mass independent. Both diameter and rotation period are inversely proportional to the pump intensity. Stable spiraling patterns in the form of complexes of multiple mutually-interacting vortices are also found. At elevated pump intensities, which create a stronger homogeneous background, we observe more complex vortex trajectories resembling Spirograph patterns.
Exciton-polaritons are a coherent electron-hole-photon (e-h-p) system where condensation has been observed in semiconductor microcavities. In contrast to equilibrium Bose-Einstein condensation (BEC) for long lifetime systems, polariton condensates have a dynamical nonequilibrium feature owing to the similar physical structure that they have to semiconductor lasers. One of the distinguishing features of a condensate to a laser is the presence of strong coupling between the matter and photon fields. Irrespective of its equilibrium or nonequilibrium nature, exciton-polariton have been observed to maintain strong coupling. We show that by investigating high density regime of exciton-polariton condensates, the negative branch directly observed in photoluminescence. This is evidence that the present e-h-p system is still in the strong coupling regime, contrary to past results where the system reduced to standard lasing at high density.
For a coherent quantum mechanical two-level system driven with a linearly time-dependent detuning, the Landau-Zener model has served over decades as a textbook model of quantum dynamics. A particularly intriguing question is whether that framework can be extended to capture an intrinsical nonequilibrium nature for a quantum system with coherent and dissipative dynamics occurring on an equal footing. In this work, we are motivated to investigate the Landau-Zenner problem of polariton condensates in a periodic potential under nonresonant pumping, considering driven-dissipative Gross-Pitaevskii equations coupled to the rate equation of a reservoir. Using a two-mode approach, we find fluctuation of the reservoir can be considered as a constant and the relative phase plays a very important role. The evolution of the dissipative Landau-Zener model we obtain presents its adiabatic process very different from the closed system because the fluctuation of the reservoir has a peak and leads to the damping of the condensates. We substitute the fluctuation of the reservoir to Hamiltonian and get an effective two-level model. The motion of Hamiltonian in phase space is also discussed and is directly corresponding to the pumping rate. The instability of the band structure can also be studied by the curvatures in phase space and there may be two loops in the middle of the Brillouin zone when the pumping rate is far beyond the threshold.
Bogoliubovs theory states that self-interaction effects in Bose-Einstein condensates produce a characteristic linear dispersion at low momenta. One of the curious features of Bogoliubovs theory is that the new quasiparticles in the system are linear combinations of creation and destruction operators of the bosons. In exciton-polariton condensates, this gives the possibility of directly observing the negative branch of the Bogoliubov dispersion in the photoluminescence (PL) emission. Here we theoretically examine the PL spectra of exciton-polariton condensates taking into account of reservoir effects. At sufficiently high excitation densities, the negative dispersion becomes visible. We also discuss the possibility for relaxation oscillations to occur under conditions of strong reservoir coupling. This is found to give a secondary mechanism for making the negative branch visible.
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