Optical read-out of the Neel vector in metallic antiferromagnet Mn$_{2}$Au


Abstract in English

Metallic antiferromagnets with broken inversion symmetry on the two sublattices, strong spin-orbit coupling and high N{e}el temperatures offer new opportunities for applications in spintronics. Especially Mn$_{2}$Au, with high N{e}el temperature and conductivity, is particularly interesting for real-world applications. Here, manipulation of the orientation of the staggered magnetization,textit{ i.e.} the N{e}el vector, by current pulses has been recently demonstrated, with the read-out limited to studies of anisotropic magnetoresistance or X-ray magnetic linear dichroism. Here, we report on the in-plane reflectivity anisotropy of Mn$_{2}$Au (001) films, which were N{e}el vector aligned in pulsed magnetic fields. In the near-infrared, the anisotropy is $approx$ 0.6%, with higher reflectivity for the light polarized along the N{e}el vector. The observed magnetic linear dichroism is about four times larger than the anisotropic magnetoresistance. This suggests the dichroism in Mn$_{2}$Au is a result of the strong spin-orbit interactions giving rise to anisotropy of interband optical transitions, in-line with recent studies of electronic band-structure. The considerable magnetic linear dichroism in the near-infrared could be used for ultrafast optical read-out of the N{e}el vector in Mn$_{2}$Au.

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