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Register a new userEmergent dark states from superradiant dynamics in multilevel atoms in a cavity
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Added by
Asier Pi\\~neiro Orioli
Publication date
2021
fields
Physics
and research's language is
English
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We investigate the collective decay dynamics of atoms with a generic multilevel structure (angular momenta $Fleftrightarrow F$) coupled to two light modes of different polarization inside a cavity. In contrast to two-level atoms, we find that multilevel atoms can harbour eigenstates that are perfectly dark to cavity decay even within the subspace of permutationally symmetric states (collective Dicke manifold). The dark states arise from destructive interference between different internal transitions and are shown to be entangled. Remarkably, the superradiant decay of multilevel atoms can end up stuck in one of these dark states, where a macroscopic fraction of the atoms remains excited. This opens the door to the preparation of entangled dark states of matter through collective dissipation useful for quantum sensing and quantum simulation. Our predictions should be readily observable in current optical cavity experiments with alkaline-earth atoms or Raman-dressed transitions.
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We propose to use fermionic atoms with degenerate ground and excited internal levels ($F_grightarrow F_e$), loaded into the motional ground state of an optical lattice with two atoms per lattice site, to realize dark states with no radiative decay. The physical mechanism behind the dark states is an interplay of Pauli blocking and multilevel dipolar interactions. The dark states are independent of lattice geometry, can support an extensive number of excitations and can be coherently prepared using a Raman scheme taking advantage of the quantum Zeno effect. These attributes make them appealing for atomic clocks, quantum memories, and quantum information on decoherence free subspaces.
We propose an experimental realization of a time crystal using an atomic Bose-Einstein condensate in a high finesse optical cavity pumped with laser light detuned to the blue side of the relevant atomic resonance. By mapping out the dynamical phase diagram, we identify regions in parameter space showing stable limit cycle dynamics. Since the model describing the system is time-independent, the emergence of a limit cycle phase indicates the breaking of continuous time translation symmetry. Employing a semiclassical analysis to demonstrate the robustness of the limit cycles against perturbations and quantum fluctuations, we establish the emergence of a time crystal.
We investigate the subradiance properties of $ngeq 2$ multilevel fermionic atoms loaded into the lowest motional level of a single trap (e.g.~a single optical lattice site or an optical tweezer). As pointed out in our previous work [arXiv:1907.05541], perfectly dark subradiant states emerge from the interplay between fermionic statistics and dipolar interactions. While in [arXiv:1907.05541] we focused on the $n=2$ case, here we provide an in-depth analysis of the single-site dark states for generic filling $n$, and show a tight connection between generic dark states and total angular momentum eigenstates. We show how the latter can also be used to understand the full eigenstate structure of the single-site problem, which we analyze numerically. Apart from this, we discuss two possible schemes to coherently prepare dark states using either a Raman transition or an external magnetic field to lift the Zeeman degeneracy. Although the analysis focuses on the single-site problem, we show that multi-site dark states can be trivially constructed in any geometry out of product states of single-site dark states. Finally, we discuss some possible implementations with alkaline-earth(-like) atoms such as $^{171}$Yb or $^{87}$Sr loaded into optical lattices, where they could be used for potential applications in quantum metrology and quantum information.
We achieve the strong coupling regime between an ensemble of phosphorus donor spins in a highly enriched $^{28}$Si crystal and a 3D dielectric resonator. Spins were polarized beyond Boltzmann equilibrium using spin selective optical excitation of the no-phonon bound exciton transition resulting in $N$ = $3.6cdot10^{13}$ unpaired spins in the ensemble. We observed a normal mode splitting of the spin ensemble-cavity polariton resonances of 2$gsqrt{N}$ = 580 kHz (where each spin is coupled with strength $g$) in a cavity with a quality factor of 75,000 ($gamma ll kappa approx$ 60 kHz where $gamma$ and $kappa$ are the spin dephasing and cavity loss rates, respectively). The spin ensemble has a long dephasing time (T$_2^*$ = 9 $mu$s) providing a wide window for viewing the dynamics of the coupled spin ensemble-cavity system. The free induction decay shows up to a dozen collapses and revivals revealing a coherent exchange of excitations between the superradiant state of the spin ensemble and the cavity at the rate $gsqrt{N}$. The ensemble is found to evolve as a single large pseudospin according to the Tavis-Cummings model due to minimal inhomogeneous broadening and uniform spin-cavity coupling. We demonstrate independent control of the total spin and the initial Z-projection of the psuedospin using optical excitation and microwave manipulation respectively. We vary the microwave excitation power to rotate the pseudospin on the Bloch sphere and observe a long delay in the onset of the superradiant emission as the pseudospin approaches full inversion. This delay is accompanied by an abrupt $pi$ phase shift in the peusdospin microwave emission. The scaling of this delay with the initial angle and the sudden phase shift are explained by the Tavis-Cummings model.
We derive a master equation for a superradiant medium which includes multilevel interference betwen the individual scatterers. The derivation relies on the Born-Markov approximation and implements the coarse graining formalism. The master equation fulfils the Lindblad form and contains terms describing single-atom multilevel interference, multi-atom interference between identical transitions, and multi-atom interference between different electronic transitions with parallel dipoles. This formalism is then applied to determine the excitation spectrum of two emitters using the parameters of the Hydrogen transitions 2S$_{1/2},to$4P$_{1/2}$ and 2S$_{1/2},to$4P$_{3/2}$, where the gap between the parallel dipoles is of the order of GHz. The distortion of the signal due to the interplay of multilevel and multi-emitter interference is analysed as a function of their distance. These results suggest that interference between parallel dipolar transition can significantly affect the spectroscopic properties of optically dense media.
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