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The goals of this study are 1) to test the best theoretical transition probabilities for Ca I (a relatively light alkaline earth spectrum) from a modern ab initio calculation using configuration interaction plus many body perturbation theory against the best modern experimental transition probabilities, and 2) to produce as accurate and comprehensive a line list of Ca I transition probabilities as is currently possible based on this comparison. We report new Ca I radiative lifetime measurements from a laser-induced fluorescence (LIF) experiment and new emission branching fraction measurements from a 0.5 m focal length grating spectrometer with a detector array. We combine these data for upper levels that have both a new lifetime and new branching fractions to report log(gf)s for two multiplets consisting of nine transitions. Detailed comparisons are made between theory and experiment, including the measurements reported herein and a selected set of previously published experimental transition probabilities. We find that modern theory compares favorably to experimental measurements in most instances where such data exist. A final list of 202 recommended transition probabilities is presented, which covers lines of Ca I with wavelengths ranging from 2200 - 10,000 Angstroms. These are mostly selected from theory, but are augmented with high quality experimental measurements from this work and from the literature. The recommended transition probabilities are used in a redetermination of the Ca abundance in the Sun and in the metal-poor star HD 84937.
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We report new branching fraction measurements for 199 UV and optical transitions of Hf II. These transitions range in wavelength (wavenumber) from 2068- 6584 A (48322-15183 cm-1) and originate in 17 odd-parity upper levels ranging in energy from 38578-53227 cm-1. The branching fractions are combined with radiative lifetimes reported in an earlier study to produce a set of transition probabilities and log(gf) values with accuracy ranging from 5-25%. Comparison is made to transition probabilities from the literature where such data exist. We use these new transition probabilities to derive improved Hf abundances in two metal-poor stars. HD 196944 is enhanced in s-process elements, and we derive log epsilon (Hf) = -0.72 +/- 0.03 (sigma = 0.09) from 12 Hf II lines. HD 222925 is enhanced in r-process elements, and we derive log epsilon (Hf) = 0.32 +/- 0.03 (sigma = 0.11) from 20 Hf II lines. These measurements greatly expand the number of potentially useful Hf II lines for analysis in UV and optical spectra.
We use 3D-PDR, a three-dimensional astrochemistry code for modeling photodissociation regions (PDRs), to post-process hydrodynamic simulations of turbulent, star-forming clouds. We focus on the transition from atomic to molecular gas, with specific attention to the formation and distribution of H, C+, C, H2 and CO. First, we demonstrate that the details of the cloud chemistry and our conclusions are insensitive to the simulation spatial resolution, to the resolution at the cloud edge, and to the ray angular resolution. We then investigate the effect of geometry and simulation parameters on chemical abundances and find weak dependence on cloud morphology as dictated by gravity and turbulent Mach number. For a uniform external radiation field, we find similar distributions to those derived using a one-dimensional PDR code. However, we demonstrate that a three-dimensional treatment is necessary for a spatially varying external field, and we caution against using one-dimensional treatments for non-symmetric problems. We compare our results with the work of Glover et al. (2010), who self-consistently followed the time evolution of molecule formation in hydrodynamic simulations using a reduced chemical network. In general, we find good agreement with this in situ approach for C and CO abundances. However, the temperature and H2 abundances are discrepant in the boundary regions (Av < 5), which is due to the different number of rays used by the two approaches.
(Abridged) Extremely metal-poor stars contain the fossil records of the chemical composition of the early Galaxy. The NLTE profiles of the calcium lines were computed in a sample of 53 extremely metal-poor stars with a modified version of the program MULTI. With our new model atom we are able to reconcile the abundance of Ca deduced from the Ca I and Ca II lines in Procyon. -We find that [Ca/Fe] = 0.50 $pm$ 0.09 in the early Galaxy, a value slightly higher than the previous LTE estimations. -The scatter of the ratios [X/Ca] is generally smaller than the scatter of the ratio [X/Mg] where X is a light metal (O, Na, Mg, Al, S, and K) with the exception of Al. These scatters cannot be explained by error of measurements, except for oxygen. Surprisingly, the scatter of [X/Fe] is always equal to, or even smaller than, the scatter around the mean value of [X/Ca]. -We note that at low metallicity, the wavelength of the Ca I resonance line is shifted relative to the (weaker) subordinate lines, a signature of the effect of convection. -The Ca abundance deduced from the Ca I resonance line (422.7 nm) is found to be systematically smaller at very low metallicity, than the abundance deduced from the subordinate lines.
Recent radiative lifetime measurements accurate to +/- 5% using laser-induced fluorescence (LIF) on 43 even-parity and 15 odd-parity levels of Ce II have been combined with new branching fractions measured using a Fourier transform spectrometer (FTS) to determine transition probabilities for 921 lines of Ce II. This improved laboratory data set has been used to determine a new solar photospheric Ce abundance, log epsilon = 1.61 +/- 0.01 (sigma = 0.06 from 45 lines), a value in excellent agreement with the recommended meteoritic abundance, log epsilon = 1.61 +/- 0.02. Revised Ce abundances have also been derived for the r-process-rich metal-poor giant stars BD+17 3248, CS 22892-052, CS 31082-001, HD 115444 and HD 221170. Between 26 and 40 lines were used for determining the Ce abundance in these five stars, yielding a small statistical uncertainty of 0.01 dex similar to the Solar result. The relative abundances in the metal-poor stars of Ce and Eu, a nearly pure r-process element in the Sun, matches r-process only model predictions for Solar System material. This consistent match with small scatter over a wide range of stellar metallicities lends support to these predictions of elemental fractions. A companion paper includes an interpretation of these new precision abundance results for Ce as well as new abundance results and interpretations for Pr, Dy and Tm.
Aims: We measure transition probabilities for Cr II transitions from the z ^4H_J, z ^2D_J, y ^4F_J, and y ^4G_J levels in the energy range 63000 to 68000 cm^{-1}. Methods: Radiative lifetimes were measured using time-resolved laser-induced fluorescence from a laser-produced plasma. In addition, branching fractions were determined from intensity-calibrated spectra recorded with a UV Fourier transform spectrometer. The branching fractions and radiative lifetimes were combined to yield accurate transition probabilities and oscillator strengths. Results: We present laboratory measured transition probabilities for 145 Cr II lines and radiative lifetimes for 14 Cr II levels. The laboratory-measured transition probabilities are compared to the values from semi-empirical calculations and laboratory measurements in the literature.
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