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Register a new userNon-equilibrium Quantum Langevin dynamics of a charged particle in a magnetic field : Response function, position-velocity and velocity autocorrelation functions
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Added by
Suraka Bhattacharjee
Publication date
2021
fields
Physics
and research's language is
English
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We use the Quantum Langevin equation as a starting point to study the response function, the position-velocity correlation function and the velocity autocorrelation function of a charged Quantum Brownian particle in a magnetic field coupled to a bath. We study two bath models -- the Ohmic bath model and the Drude bath model and make a detailed comparison in various time-temperature regimes. For both bath models there is a competition between the cyclotron frequency and the viscous damping rate giving rise to a transition from an oscillatory to a monotonic behaviour as the damping rate is increased. In the zero point fluctuation dominated low temperature regime, non-trivial noise correlations lead to some interesting features in this transition. We study the role of the memory time scale which comes into play in the Drude model and study the effect of this additional time scale. We discuss the experimental implications of our analysis in the context of experiments in cold ions.
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A simple ansatz for the study of velocity autocorrelation functions in fluids at different timescales is proposed. The ansatz is based on an effective summation of the infinite continued fraction at a reasonable assumption about convergence of relaxation times of the higher order memory functions, which have a purely kinetic origin. The VAFs obtained within our approach are compared with the results of the Markovian approximation for memory kernels. It is shown that although in the overdamped regime both approaches agree to a large extent at the initial and intermediate times of the system evolution, our formalism yields power law relaxation of the VAFs which is not observed at the description with a finite number of the collective modes. Explicit expressions for the transition times from kinetic to hydrodynamic regimes are obtained from the analysis of the singularities of spectral functions in the complex frequency plane.
Velocity autocorrelation functions (VAF) of the fluids are studied on short- and long-time scales within a unified approach. This approach is based on an effective summation of the infinite continued fraction at a reasonable assumption about convergence of relaxation times of the high order memory functions, which have purely kinetic origin. The VAFs obtained within our method are compared with computer simulation data for the liquid Ne at different densities and the results, which follow from the Markovian approximation for the highest order kinetic kernels. It is shown that in all the thermodynamic points and at the chosen level of the hierarchy, our results agree much better with the MD data than those of the Markovian approximation. The density dependence of the transition time, needed for the fluid to attain the hydrodynamic stage of evolution, is evaluated. The common and distinctive features of our method are discussed in their relations to the generalized collective mode (GCM) theory, the mode coupling theory (MCT), and some other theoretical approaches.
Extending a previous study of the velocity autocorrelation function (VAF) in a simulated Lennard-Jones fluid to cover higher-density and lower-temperature states, we show that the recently demonstrated multiexponential expansion allows for a full account and understanding of the dynamical processes encompassed by a fundamental quantity as the VAF. In particular, besides obtaining evidence of a persisting long-time tail, we assign specific and unambiguous physical meanings to groups of exponential modes related to the longitudinal and transverse collective dynamics, respectively. We have made this possible by consistently introducing the interpretation of the VAF frequency spectrum as a global density of states in fluids, generalizing a solid-state concept, and by giving to specific spectral components, obtained via the VAF exponential expansion, the corresponding meaning of partial densities of states relative to specific dynamical processes. The clear identification of a high-frequency oscillation of the VAF with the near-top excitation frequency in the dispersion curve of acoustic waves is a neat example of the power of the method. As for the transverse mode contribution, its analysis turns out to be particularly important, because the multiexponential expansion reveals a transition marking the onset of propagating excitations when the density is increased above a threshold value. While this finding agrees with recent literature debating the issue of dynamical crossover boundaries, such as the one identified with the Frenkel line, we can add detailed information on the modes involved in this specific process in the domains of both time and frequency. This will help obtain a still missing full account of transverse dynamics, in its nonpropagating and propagating aspects which are linked by dynamical transitions depending on both the thermodynamic states and the excitation wavevectors.
Using the recently constructed covariant Ito-Langevin dynamics, we develop a covariant theory of non-equilibrium thermodynamics that is applicable to small systems with multiplicative noises and with slow variables forming curved manifolds. Assuming instantaneous detailed balance, we derive expressions for work, heat, entropy production, and free energy both at ensemble level, as well as at the level of individual dynamic trajectory. We also relate time-reversal asymmetry to entropy production, and derive its consequences such as fluctuation theorem and work relation. The theory is based on Ito-calculus, is fully covariant under time-independent nonlinear transformation of variables, and is applicable to systems strongly coupled to environments.
Recently, it has been shown that there is a trade-off relation between thermodynamic cost and current fluctuations, referred to as the thermodynamic uncertainty relation (TUR). The TUR has been derived for various processes, such as discrete-time Markov jump processes and overdamped Langevin dynamics. For underdamped dynamics, it has recently been reported that some modification is necessary for application of the TUR. In this study, we present a more generalized TUR, applicable to a system driven by a velocity-dependent force in the context of underdamped Langevin dynamics, by extending the theory of Vu and Hasegawa [preprint arXiv:1901.05715]. We show that our TUR accurately describes the trade-off properties of a molecular refrigerator (cold damping), Brownian dynamics in a magnetic field, and an active particle system.
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