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Photonic Bound-States-in-the-Continuum Observed with an Electron Nanoprobe

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 Added by Zhaogang Dong Dr
 Publication date 2021
  fields Physics
and research's language is English




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Bound-states-in-the-continuum (BIC)is a wave-mechanical concept that generates resonances with vanishing spectral linewidths. It has many practical applications in Optics, such as narrow-band filters, mirror-less lasing, and nonlinear harmonic generation. As true BIC optical modes non-radiative and confined to the near field of nanostructures, they cannot be excited using propagating light. As a result, their direct experimental observation has been elusive. Rather than using light, we demonstrate probing BIC modes on arrays of silicon nanoantennas using a focused beam of electrons in a tranmission electron microscope. By combining cathodoluminescence (CL) and monochromated electron energy-loss spectroscopy (EELS) with controlled nanofabrication, we provide direct experimental evidence of true BIC modes, and demonstrate a BIC mode in the visible spectrum at 720 nm. The ability to observe and quantify these guided resonances with a spatial precision more than two orders of magnitude higher than previous far-field measurements allows the probing of individual elements in the nano-antenna arrays. The high-resolution experimental results are supported by numerical simulations as well as multipolar decomposition analysis, allowing us to demonstrate that the coherent interaction length of the quasi-BIC resonance requires at least 6 neighboring antenna elements, achieving over 60 times higher emissivity than for unpatterned silicon.



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Bound states in the continuum (BICs) are radiationless localized states embedded in the part of the parameter space that otherwise corresponds to radiative modes. Many decades after their original prediction and early observations in acoustic systems, such states have been demonstrated recently in photonic structures with engineered geometries. Here, we put forward a mechanism, based on waveguiding structures that contain anisotropic birefringent materials, that affords the existence of BICs with fundamentally new properties. In particular, anisotropy-induced BICs may exist in symmetric as well as in asymmetric geometries; they form in tunable angular propagation directions; their polarization may be pure transverse electric, pure transverse magnetic or full vector with tunable polarization hybridity; and they may be the only possible bound states of properly designed structures, and thus appear as a discrete, isolated bound state embedded in a whole sea of radiative states.
Bound states in the continuum (BICs) in photonic crystals represent the unique solutions of wave equations possessing an infinite quality-factor. We design a type of bilayer photonic crystal and study the influence of symmetry and coupling between TE and TM polarizations on BICs. The BIC modes possess $C_{3v}$ symmetry in the x-y plane while the mirror-flip symmetry in the z-direction is broken, and they provide selective coupling into different layers by varying frequency. The enhanced TE-TM coupling due to broken mirror-flip symmetry in the z-direction gives rise to high-Q factor BIC states with unique spatial characteristics. We show the emergence of such BIC states even in the presence of coupling between the TE- and TM-like modes, which is different from the existing single polarization BIC models. We propose to study BICs in multilayer systems, and the results may be helpful in designing photonic settings to observe and manipulate BICs with various symmetries and polarizations for practical applications.
In the last decade, symmetry-protected bound states in the continuum (BICs) have proven to be an important design principle for creating and enhancing devices reliant upon states with high quality (Q) factors, such as sensors, lasers, and those for harmonic generation. However, as we show, current implementations of symmetry-protected BICs in photonic crystal slabs can only be found at the center of the Brillouin zone and below the Bragg-diffraction limit, which fundamentally restricts their use to single-frequency applications. By 3D-micro printing a photonic crystal structure using two-photon polymerization, we demonstrate that this limitation can be overcome by altering the radiative environment surrounding the slab to be a three-dimensional photonic crystal. This allows for the protection of a line of BICs by embedding it in a symmetry bandgap of the crystal. Moreover, we experimentally verify that just a single layer of this photonic crystal environment is sufficient. This concept significantly expands the design freedom available for developing next-generation devices with high-Q states.
Higher-order topological insulators (HOTIs) are recently discovered topological phases, possessing symmetry-protected corner states with fractional charges. An unexpected connection between these states and the seemingly unrelated phenomenon of bound states in the continuum (BICs) was recently unveiled. When nonlinearity is added to a HOTI system, a number of fundamentally important questions arise. For example, how does nonlinearity couple higher-order topological BICs with the rest of the system, including continuum states? In fact, thus far BICs in nonlinear HOTIs have remained unexplored. Here, we demonstrate the interplay of nonlinearity, higher-order topology, and BICs in a photonic platform. We observe topological corner states which, serendipitously, are also BICs in a laser-written second-order topological lattice. We further demonstrate nonlinear coupling with edge states at a low nonlinearity, transitioning to solitons at a high nonlinearity. Theoretically, we calculate the analog of the Zak phase in the nonlinear regime, illustrating that a topological BIC can be actively tuned by both focusing and defocusing nonlinearities. Our studies are applicable to other nonlinear HOTI systems, with promising applications in emerging topology-driven devices.
We show that point defects in two-dimensional photonic crystals can support bound states in the continuum (BICs). The mechanism of confinement is a symmetry mismatch between the defect mode and the Bloch modes of the photonic crystal. These BICs occur in the absence of bandgaps and therefore provide an alternative mechanism to confine light. Furthermore, we show that such BICs can propagate in a fiber geometry and exhibit arbitrarily small group velocity which could serve as a platform for enhancing non-linear effects and light-matter interactions in structured fibers.
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