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Register a new userUltrafast coherent all-optical switching of an antiferromagnet with the inverse Faraday effect
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We explore the possibility of ultrafast, coherent all-optical magnetization switching in antiferromagnets by studying the action of the inverse Faraday effect in CrPt, an easy-plane antiferromagnet. Using a combination of density functional theory and atomistic spin dynamics simulations, we show how a circularly polarized laser pulse can switch the order parameter of the antiferromagnet within a few hundred femtoseconds. This nonthermal switching takes place on an elliptical path, driven by the staggered magnetic moments induced by the inverse Faraday effect and leading to reliable switching between two perpendicular magnetic states.
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Using time-resolved magneto-optical Kerr effect (TR-MOKE) method, helicity-dependent all-optical magnetization switching (HD-AOS) is observed in ferrimagnetic TbFeCo films. The thermal effect and opto-magneto effects are separately justified after single circularly polarized laser pulse. The integral evolution of this ultrafast switching is characterized on different time scales and the defined magnetization reversal time of 460 fs is the fastest ever observed. Combining the heat effect and inverse Faraday effect (IFE), micromagnetic simulations based on a single macro-spin model are performed that reproduce HD-AOS following a linear reversal mechanism.
Future information technology demands ultimately fast, low-loss quantum control. Intense light fields have facilitated important milestones, such as inducing novel states of matter, accelerating electrons ballistically, or coherently flipping the valley pseudospin. These dynamics leave unique signatures, such as characteristic bandgaps or high-order harmonic radiation. The fastest and least dissipative way of switching the technologically most important quantum attribute - the spin - between two states separated by a potential barrier is to trigger an all-coherent precession. Pioneering experiments and theory with picosecond electric and magnetic fields have suggested this possibility, yet observing the actual dynamics has remained out of reach. Here, we show that terahertz (1 THz = 10$^{12}$ Hz) electromagnetic pulses allow coherent navigation of spins over a potential barrier and we reveal the corresponding temporal and spectral fingerprints. This goal is achieved by coupling spins in antiferromagnetic TmFeO$_{3}$ with the locally enhanced THz electric field of custom-tailored antennas. Within their duration of 1 ps, the intense THz pulses abruptly change the magnetic anisotropy and trigger a large-amplitude ballistic spin motion. A characteristic phase flip, an asymmetric splitting of the magnon resonance, and a long-lived offset of the Faraday signal are hallmarks of coherent spin switching into adjacent potential minima, in agreement with a numerical simulation. The switchable spin states can be selected by an external magnetic bias. The low dissipation and the antennas sub-wavelength spatial definition could facilitate scalable spin devices operating at THz rates.
The manipulation of the magnetic direction by using the ultrafast laser pulse is attractive for its great advantages in terms of speed and energy efficiency for information storage applications. However, the heating and helicity effects induced by circularly polarized laser excitation are entangled in the helicity-dependent all-optical switching (HD-AOS), which hinders the understanding of magnetization dynamics involved. Here, by applying a dual-pump laser excitation, first with a linearly polarized (LP) laser pulse followed by a circularly polarized (CP) laser pulse, we identify the timescales and contribution from heating and helicity effects in HD-AOS with a Pt/Co/Pt triple layer. When the sample is preheated by the LP laser pulses to a nearly fully demagnetized state, CP laser pulses with a much-reduced power switches the samples magnetization. By varying the time delay between the two pump pulses, we show that the helicity effect, which gives rise to the deterministic helicity induced switching, onsets instantly upon laser excitation, and only exists for less than 0.2 ps close to the laser pulse duration of 0.15 ps. The results reveal that that the transient magnetization state upon which CP laser pulses impinge is the key factor for achieving HD-AOS, and importantly, the tunability between heating and helicity effects with the unique dual-pump laser excitation approach will enable HD-AOS in a wide range of magnetic material systems for the potential ultrafast spintronics applications.
Single-mode high-index-contrast waveguides have been ubiquitously exploited in optical, microwave, and phononic structures for achieving enhanced wave-matter interactions. Although micro-scale optomechanical and electro-optical devices have been widely studied, optomagnonic devices remain a grand challenge at the microscale. Here, we introduce a planar optomagnonic waveguide platform based on a ferrimagnetic insulator that simultaneously supports single transverse mode of spin waves (magnons) and highly confined optical modes. The co-localization of spin and light waves gives rise to enhanced inverse Faraday effect, and as a result, magnons are excited by an effective magnetic field generated by interacting optical photons. Moreover, the strongly enhanced optomagnonic interaction allows us to observe such effect using low-power (milliwatt level) light signals in the continuous-wave form, as opposed to high-intensity (megawatt peak power) light pulses that are typically required in magnetic bulk materials or thin films. The optically-driven magnons are detected electrically with preserved phase coherence, showing the feasibility for launching spin waves with low-power continuous optical fields.
An analytic expression is given for the inverse Faraday effect, i.e. for the magnetization occurring in a transparent medium exposed to a circularly polarized high-frequency electromagnetic wave. Using a microscopic approach the magnetization of the medium due to the inverse Faraday effect is identified as the result of microscopic solenoidal currents generated by the electromagnetic wave. In contrast to the better known phenomenological derivation, the microscopic treatment provides important information on the frequency dependence of the inverse Faraday effect.
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