No Arabic abstract
We develop a novel method based in the sparse random graph to account the interplay between geometric frustration and disorder in cluster magnetism. Our theory allows to introduce the cluster network connectivity as a controllable parameter. Two types of inner cluster geometry are considered: triangular and tetrahedral. The theory was developed for a general, non-uniform intra-cluster interactions, but in the present paper the results presented correspond to uniform, anti-ferromagnetic (AF) intra-clusters interactions $J_{0}/J$. The clusters are represented by nodes on a finite connectivity random graph, and the inter-cluster interactions are random Gaussian distributed. The graph realizations are treated in replica theory using the formalism of order parameter functions, which allows to calculate the distribution of local fields and, as a consequence, the relevant observable. In the case of triangular cluster geometry, there is the onset of a classical Spin Liquid state at a temperature $T^{*}/J$ and then, a Cluster Spin Glass (CSG) phase at a temperature $T_{f}/J$. The CSG ground state is robust even for very weak disorder or large negative $J_{0}/J$. These results does not depend on the network connectivity. Nevertheless, variations in the connectivity strongly affect the level of frustration $f_{p}=-Theta_{CW}/T_{f}$ for large $J_{0}/J$. In contrast, for the non-frustrated tetrahedral cluster geometry, the CSG ground state is suppressed for weak disorder or large negative $J_{0}/J$. The CSG boundary phase presents a re-entrance which is dependent on the network connectivity.
We analytically and numerically characterize the structure of hard-sphere fluids in order to review various geometrical frustration scenarios of the glass transition. We find generalized polytetrahedral order to be correlated with increasing fluid packing fraction, but to become increasingly irrelevant with increasing dimension. We also find the growth in structural correlations to be modest in the dynamical regime accessible to computer simulations.
Using tempered Monte Carlo simulations, we study the the spin-glass phase of dense packings of Ising dipoles pointing along random axes. We consider systems of L^3 dipoles (a) placed on the sites of a simple cubic lattice with lattice constant $d$, (b) placed at the center of randomly closed packed spheres of diameter d that occupy a 64% of the volume. For both cases we find an equilibrium spin-glass phase below a temperature T_sg. We compute the spin-glass overlap parameter q and their associated correlation length xi_L. From the variation of xi_L with T and L we determine T_sg for both systems. In the spin-glass phase, we find (a) <q> decreases algebraically with L, and (b) xi_L/L does not diverge as L increases. At very low temperatures we find comb-like distributions of q that are sample-dependent. We find that the fraction of samples with cross-overlap spikes higher than a certain value as well as the average width of the spikes are size independent quantities. All these results are consistent with a quasi-long-range order in the spin-glass phase, as found previously for very diluted dipolar systems.
The interplay between quantum fluctuations and disorder is investigated in a spin-glass model, in the presence of a uniform transverse field $Gamma$, and a longitudinal random field following a Gaussian distribution with width $Delta$. The model is studied through the replica formalism. This study is motivated by experimental investigations on the LiHo$_x$Y$_{1-x}$F$_4$ compound, where the application of a transverse magnetic field yields rather intriguing effects, particularly related to the behavior of the nonlinear magnetic susceptibility $chi_3$, which have led to a considerable experimental and theoretical debate. We analyzed two situations, namely, $Delta$ and $Gamma$ considered as independent, as well as these two quantities related as proposed recently by some authors. In both cases, a spin-glass phase transition is found at a temperature $T_f$; moreover, $T_f$ decreases by increasing $Gamma$ towards a quantum critical point at zero temperature. The situation where $Delta$ and $Gamma$ are related appears to reproduce better the experimental observations on the LiHo$_x$Y$_{1-x}$F$_4$ compound, with the theoretical results coinciding qualitatively with measurements of the nonlinear susceptibility. In this later case, by increasing $Gamma$, $chi_3$ becomes progressively rounded, presenting a maximum at a temperature $T^*$ ($T^*>T_f$). Moreover, we also show that the random field is the main responsible for the smearing of the nonlinear susceptibility, acting significantly inside the paramagnetic phase, leading to two regimes delimited by the temperature $T^*$, one for $T_f<T<T^*$, and another one for $T>T^*$. It is argued that the conventional paramagnetic state corresponds to $T>T^*$, whereas the temperature region $T_f<T<T^*$ may be characterized by a rather unusual dynamics, possibly including Griffiths singularities.
The left-right chiral and ferromagnetic-antiferromagnetic double spin-glass clock model, with the crucially even number of states q=4 and in three dimensions d=3, has been studied by renormalization-group theory. We find, for the first time to our knowledge, four different spin-glass phases, including conventional, chiral, and quadrupolar spin-glass phases, and phase transitions between spin-glass phases. The chaoses, in the different spin-glass phases and in the phase transitions of the spin-glass phases with the other spin-glass phases, with the non-spin-glass ordered phases, and with the disordered phase, are determined and quantified by Lyapunov exponents. It is seen that the chiral spin-glass phase is the most chaotic spin-glass phase. The calculated phase diagram is also otherwise very rich, including regular and temperature-inverted devils staircases and reentrances.
URh_2Ge_2 occupies an extraordinary position among the heavy-electron 122-compounds, by exhibiting a previously unidentified form of magnetic correlations at low temperatures, instead of the usual antiferromagnetism. Here we present new results of ac and dc susceptibilities, specific heat and neutron diffraction on single-crystalline as-grown URh_2Ge_2. These data clearly indicate that crystallographic disorder on a local scale produces spin glass behavior in the sample. We therefore conclude that URh_2Ge_2 is a 3D Ising-like, random-bond, heavy-fermion spin glass.