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Register a new userDensity Response of the Warm Dense Electron Gas beyond Linear Response Theory: Excitation of Harmonics
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In a recent Letter, Dornheim et al. [PRL 125, 085001 (2020)] have investigated the nonlinear density response of the uniform electron gas in the warm dense matter regime. More specifically, they have studied the cubic response function at the first harmonic, which cannot be neglected in many situations of experimental relevance. In this work, we go one step further and study the full spectrum of excitations at the higher harmonics of the original perturbation based on extensive new ab initio path integral Monte Carlo (PIMC) simulations. We find that the dominant contribution to the density response beyond linear response theory is given by the quadratic response function at the second harmonic in the moderately nonlinear regime. Furthermore, we show that the nonlinear density response is highly sensitive to exchange-correlation effects, which makes it a potentially valuable new tool of diagnostics. To this end, we present a new theoretical description of the nonlinear electronic density response based on the recent effective static approximation to the local field correction [PRL 125, 235001 (2020)], which accurately reproduces our PIMC data with negligible computational cost.
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In a recent Letter [T.~Dornheim emph{et al.}, Phys.~Rev.~Lett.~textbf{125}, 085001 (2020)], we have presented the first emph{ab initio} results for the nonlinear density response of electrons in the warm dense matter regime. In the present work, we extend these efforts by carrying out extensive new path integral Monte Carlo (PIMC) simulations of a emph{ferromagnetic} electron gas that is subject to an external harmonic perturbation. This allows us to unambiguously quantify the impact of spin-effects on the nonlinear density response of the warm dense electron gas. In addition to their utility for the description of warm dense matter in an external magnetic field, our results further advance our current understanding of the uniform electron gas as a fundamental model system, which is important in its own right.
In a recent letter [textit{Phys.~Rev.~Lett.}~textbf{125}, 085001 (2020)], Dornheim textit{et al.}~have presented the first textit{ab initio} path integral Monte Carlo (PIMC) results for the nonlinear electronic density response at warm dense matter (WDM) conditions. In the present work, we extend these considerations by exploring the relation between the nonlinear response and three-/four-body correlation functions from many-body theory. In particular, this connection directly implies a comparably increased sensitivity of the nonlinear response to electronic exchange-correlation (XC) effects, which is indeed confirmed by our analysis over the entire relevant range of densities ($r_s=0.5,dots,10$) and temperatures ($theta=0.01,dots,4$). Finally, our work suggests the possibility of deliberately probing the nonlinear regime to experimentally probe three- and potentially even four-body correlation functions in WDM.
Warm dense matter (WDM) has emerged as one of the frontiers of both experimental and theoretical physics and is challenging traditional concepts of plasma, atomic, and condensed-matter physics. While it has become common practice to model correlated electrons in WDM within the framework of Kohn-Sham density functional theory, quantitative benchmarks of exchange-correlation (XC) functionals under WDM conditions are yet incomplete. Here, we present the first assessment of common XC functionals against exact path-integral Monte Carlo calculations of the harmonically perturbed thermal electron gas. This system is directly related to the numerical modeling of X-Ray scattering experiments on warm dense samples. Our assessment yields the parameter space where common XC functionals are applicable. More importantly, we pinpoint where the tested XC functionals fail when perturbations on the electronic structure are imposed. We indicate the lack of XC functionals that take into account the needs of WDM physics in terms of perturbed electronic structures.
The increasing number of mass events involving large crowds calls for a better understanding of the dynamics of dense crowds. Inquiring into the possibility of a mechanical description of these dynamics, we experimentally study the crossing of dense static crowds by a cylindrical intruder, a mechanical test which is classical for granular matter. The analysis of our experiments reveals robust features in the crowds response, comprising both similarities and discrepancies with the response of granular media. Common features include the presence of a depleted region behind the intruder and the short-range character of the perturbation. On the other hand, unlike grains, pedestrians anticipate the intruders passage by moving much before contact and their displacements are mostly lateral, hence not aligned with the forces exerted by the intruder. Similar conclusions are reached when the intruder is not a cylinder, but a single crossing pedestrian. Thus, our work shows that pedestrian interactions even at high densities (3 to 6 ped/m 2) do not reduce to mechanical ones. More generally, the avoidance strategies evidenced by our findings question the incautious use of force models for dense crowds.
In general, linear response theory expresses the relation between a driving and a physical systems response only to first order in perturbation theory. In the context of charge transport, this is the linear relation between current and electromotive force expressed in Ohms law. We show here that, in the case of the quantum Hall effect, all higher order corrections vanish. We prove this in a fully interacting setting and without flux averaging.
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