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Register a new userTunable Hyperbolic Phonon Polaritons in a Gradiently-Suspended Van Der Waals {alpha}-MoO3
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Highly confined and low-loss hyperbolic phonon polaritons (HPhPs) sustained in van der Waals crystals exhibit outstanding capabilities of concentrating long-wave electromagnetic fields deep to the subwavelength region. Precise tuning on the HPhP propagation characteristics remains a great challenge for practical applications such as nanophotonic devices and circuits. Here, we show that by taking advantage of the varying air gaps in a van der Waals {alpha}-MoO3 crystal suspended gradiently, it is able to tune the wavelengths and dampings of the HPhPs propagating inside the {alpha}-MoO3. The results indicate that the dependences of polariton wavelength on gap distance for HPhPs in lower and upper Reststrahlen bands are opposite to each other. Most interestingly, the tuning range of the polariton wavelengths for HPhPs in the lower band, which exhibit in-plane hyperbolicities, is wider than that for the HPhPs in the upper band of out-of-plane hyperbolicities. A polariton wavelength elongation up to 160% and a reduction of damping rate up to 35% are obtained. These findings can not only provide fundamental insights into manipulation of light by polaritonic crystals at nanoscale, but also open up new opportunities for tunable nanophotonic applications.
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Surface phonon polaritons (SPhPs) in polar dielectrics offer new opportunities for infrared nanophotonics due to sub-diffraction confinement with low optical losses. Though the polaritonic field confinement can be significantly improved by modifying the dielectric environment, it is challenging to break the fundamental limits in photon confinement and propagation behavior of SPhP modes. In particular, as SPhPs inherently propagate isotropically in these bulk polar dielectrics, how to collectively realize ultra-large field confinement, in-plane hyperbolicity and unidirectional propagation remains elusive. Here, we report an approach to solve the aforementioned issues of bulk polar dielectrics SPhPs at one go by constructing a heterostructural interface between biaxial van der Waals material (e.g., MoO3) and bulk polar dielectric (e.g., SiC, AlN, and GaN). Due to anisotropy-oriented mode couplings at the interface, the hybridized SPhPs with a large confinement factor (>100) show in-plane hyperbolicity that has been switched to the orthogonal direction as compared to that in natural MoO3. More interestingly, this proof of concept allows steerable, angle-dependent and unidirectional polariton excitation by suspending MoO3 on patterned SiC air cavities. Our finding exemplifies a generalizable framework to manipulate the flow of nano-light and engineer unusual polaritonic responses in many other hybrid systems consisting of van der Waals materials and bulk polar dielectrics.
Hyperbolic phonon polaritons (HPhPs) sustained in van der Waals (vdW) materials exhibit extraordinary capabilities of confining long-wave electromagnetic fields to the deep subwavelength scale. In stark contrast to the uniaxial vdW hyperbolic materials such as hexagonal boron nitride (h-BN), the recently emerging biaxial hyperbolic materials such as {alpha}-MoO3 and {alpha}-V2O5 further bring new degree of freedoms in controlling light at the flatland, due to their distinctive in-plane hyperbolic dispersion. However, the controlling and focusing of such in-plane HPhPs are to date remain elusive. Here, we propose a versatile technique for launching, controlling and focusing of in-plane HPhPs in {alpha}-MoO3 with geometrically designed plasmonic antennas. By utilizing high resolution near-field optical imaging technique, we directly excited and mapped the HPhPs wavefronts in real space. We find that subwavelength manipulating and focusing behavior are strongly dependent on the curvature of antenna extremity. This strategy operates effectively in a broadband spectral region. These findings can not only provide fundamental insights into manipulation of light by biaxial hyperbolic crystals at nanoscale, but also open up new opportunities for planar nanophotonic applications.
The exploitation of phonon-polaritons in nanostructured materials offers a pathway to manipulate infrared (IR) light for nanophotonic applications. Notably, hyperbolic phonons polaritons (HP2) in polar bidimensional crystals have been used to demonstrate strong electromagnetic field confinement, ultraslow group velocities, and long lifetimes (~ up to 8 ps). Here we present nanobelts of {alpha}-phase molybdenum trioxide ({alpha}-MoO3) as a low-dimensional medium supporting HP2 modes in the mid- and far-IR ranges. By real-space nanoimaging, with IR illuminations provided by synchrotron and tunable lasers, we observe that such HP2 response happens via formation of Fabry-Perot resonances. We remark an anisotropic propagation which critically depends on the frequency range. Our findings are supported by the convergence of experiment, theory, and numerical simulations. Our work shows that the low dimensionality of natural nanostructured crystals, like {alpha}-MoO3 nanobelts, provides an attractive platform to study polaritonic light-matter interactions and offer appealing cavity properties that could be harnessed in future designs of compact nanophotonic devices.
Van der Waals heterostructures assembled from layers of 2D materials have attracted considerable interest due to their novel optical and electrical properties. Here we report a scattering-type scanning near field optical microscopy study of hexagonal boron nitride on black phosphorous (h-BN/BP) heterostructures, demonstrating the first direct observation of in-plane anisotropic phonon polariton modes in vdW heterostructures. Strikingly, the measured in-plane optical anisotropy along armchair and zigzag crystal axes exceeds the ratio of refractive indices of BP in the x-y plane. We explain that this enhancement is due to the high confinement of the phonon polaritons in h-BN. We observe a maximum in-plane optical anisotropy of {alpha}_max=1.25 in the 1405-1440 cm-1 frequency spectrum. These results provide new insights on the behavior of polaritons in vdW heterostructures, and the observed anisotropy enhancement paves the way to novel nanophotonic devices and to a new way to characterize optical anisotropy in thin films.
yperbolic polaritons in van der Waals materials recently attract a lot of attention, owing to their strong electromagnetic field confinement, ultraslow group velocities and long lifetimes. Typically, volume confined hyperbolic polaritons (HPs) are studied. Here we show the first near-field optical images of hyperbolic surface polarities, HSPs, which are confined and guided at the edges of thin flakes of a vdW material. To that end, we applied scattering-type scanning near-field optical microscopy (s-SNOM) for launching and real-space nanoimaging of hyperbolic surface phonon polariton modes on a hexagonal boron nitride, h-BN, flake. Our imaging data reveal that the fundamental HSP mode exhibits stronger field confinement, smaller group velocities and nearly identical lifetimes, as compared to the fundamental HP mode of the same h-BN flake. Our experimental data, corroborated by theory, establish a solid basis for future studies and applications of HPs and HSPs in vdW materials.
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