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Register a new userExploring multichannel superconductivity in ThFeAsN
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We investigate theoretically the superconducting state of the undoped Fe-based superconductor ThFeAsN. Using input from $ab~initio$ calculations, we solve the Fermi-surface based, multichannel Eliashberg equations for Cooper-pair formation mediated by spin and charge fluctuations, and by the electron-phonon interaction (EPI). Our results reveal that spin fluctuations alone, when coupling only hole-like with electron-like energy bands, can account for a critical temperature $T_c$ up to $sim7.5,mathrm{K}$ with an $s_{pm}$-wave superconducting gap symmetry, which is a comparatively low $T_c$ with respect to the experimental value $T_c^{mathrm{exp}}=30,mathrm{K}$. Other combinations of interaction kernels (spin, charge, electron-phonon) lead to a suppression of $T_c$ due to phase frustration of the superconducting gap. We qualitatively argue that the missing ingredient to explain the gap magnitude and $T_c$ in this material is the first-order correction to the EPI vertex. In the noninteracting state this correction adopts a form supporting the $s_{pm}$ gap symmetry, in contrast to EPI within Migdals approximation, i.e., EPI without vertex correction, and therefore it enhances tendencies arising from spin fluctuations.
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Unlike the widely studied ReFeAsO series, the newly discovered iron-based superconductor ThFeAsN exhibits a remarkably high critical temperature of 30 K, without chemical doping or external pressure. Here we investigate in detail its magnetic and superconducting properties via muon-spin rotation/relaxation ($mu$SR) and nuclear magnetic resonance (NMR) techniques and show that ThFeAsN exhibits strong magnetic fluctuations, suppressed below 35 K, but no magnetic order. This contrasts strongly with the ReFeAsO series, where stoichiometric parent materials order antiferromagnetically and superconductivity appears only upon doping. The ThFeAsN case indicates that Fermi-surface modifications due to structural distortions and correlation effects are as important as doping in inducing superconductivity. The direct competition between antiferromagnetism and superconductivity, which in ThFeAsN (as in LiFeAs) occurs at already zero doping, may indicate a significant deviation of the $s$-wave superconducting gap in this compound from the standard $s^{pm}$ scenario.
Chains of magnetic atoms placed on the surface of an s-wave superconductor with large spin-orbit coupling provide a promising platform for the realization of topological superconducting states characterized by the presence of Majorana zero-energy modes. In this work we study the properties of the one-dimensional chain of Yu-Shiba-Rusinov states induced by magnetic impurities using a realistic model for the magnetic atoms that include the presence of multiple scattering channels. These channels are mixed by the spin-orbit coupling and, via the hybridization of the Yu-Shiba-Rusinov states at different sites of the chain, result in a multi-band structure for the chain. We obtain the topological phase diagram for such band structure. We identify the parameter regimes for which the different bands lead to a topological phase and show that the inclusion of higher bands can greatly enlarge the phase space for the realization of topological states.
The exploration of topological superconductivity and Majorana zero modes has become a rapidly developing field. Many types of proposals to realize topological superconductors have been presented, and significant advances have been recently made. In this review, we conduct a survey on the experimental progress in possible topological superconductors and induced superconductivity in topological insulators or semimetals as well as artificial structures. The approaches to inducing superconductivity in topological materials mainly include high pressure application, the hard-tip point contact method, chemical doping or intercalation, the use of artificial topological superconductors, and electric field gating. The evidence supporting topological superconductivity and signatures of Majorana zero modes are also discussed and summarized.
We report the first nitrogen-containing iron-pnictide superconductor ThFeAsN, which is synthesized by a solid-state reaction in an evacuated container. The compound crystallizes in a ZrCuSiAs-type structure with the space group P4/nmm and lattice parameters a=4.0367(1) {AA} and c=8.5262(2) {AA} at 300 K. The electrical resistivity and dc magnetic susceptibility measurements indicate superconductivity at 30 K for the nominally undoped ThFeAsN.
ThFeAsN$_{1-x}$O$_x$ ($0leq xleq0.6$) system with heavy electron doping has been studied by the measurements of X-ray diffraction, electrical resistivity, magnetic susceptibility and specific heat. The non-doped compound exhibits superconductivity at $T_mathrm{c}^mathrm{onset}=30$ K, which is possibly due to an internal uniaxial chemical pressure that is manifested by the extremely small value of As height with respect to the Fe plane. With the oxygen substitution, the $T_mathrm{c}$ value decreases rapidly to below 2 K for $0.1leq xleq0.2$, and surprisingly, superconductivity re-appears in the range of $0.25leq xleq0.5$ with a maximum $T_mathrm{c}^mathrm{onset}$ of 17.5 K at $x=0.3$. For the normal-state resistivity, while the samples in intermediate non-superconducting interval exhibit Fermi liquid behavior, those in other regions show a non-Fermi-liquid behavior. The specific heat jump for the superconducting sample of $x=0.4$ is $Delta C/(gamma T_mathrm{c})=0.89$, which is discussed in terms of anisotropic superconducting gap. The peculiar phase diagram in ThFeAsN$_{1-x}$O$_x$ presents additional ingredients for understanding the superconducting mechanism in iron-based superconductors.
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