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Register a new userEmergent ferromagnetism with Fermi-liquid behavior in proton intercalated CaRuO3
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The evolution between Fermi liquid and non-Fermi-liquid states in correlated electron systems has been a central subject in condensed matter physics because of the coupled intriguing magnetic and electronic states. An effective pathway to explore the nature of non-Fermi liquid behavior is to approach its phase boundary. Here we report a crossover from non-Fermi liquid to Fermi-liquid state in metallic CaRuO3 through ionic liquid gating induced protonation with electric field. This electronic transition subsequently triggers a reversible magnetic transition with the emergence of an exotic ferromagnetic state from this paramagnetic compound. Our theoretical analysis reveals that hydrogen incorporation plays a critical role in both the electronic and magnetic phase transitions via structural distortion and electron doping. These observations not only help understand the correlated magnetic and electronic transitions in perovskite ruthenate systems, but also provide novel pathways to design electronic phases in correlated materials.
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The perovskite ruthenate has attracted considerable interest due to reports of possible non-Fermi-liquid behavior and its proximity to a magnetic quantum critical point, yet its ground state and electronic structure remain enigmatic. Here we report the first measurements of the Fermi surface and quasiparticle dispersion in CaRuO3 through a combination of oxide molecular beam epitaxy and in situ angle-resolved photoemission spectroscopy. Our results reveal a complex and anisotropic Fermi surface consisting of small electron pockets and straight segments, consistent with the bulk orthorhombic crystal structure with large octahedral rotations. We observe a strongly band-dependent mass renormalization, with prominent heavy quasiparticle bands which lie close to the Fermi energy and exhibit strong temperature dependence. These results are consistent with a heavy Fermi liquid with a complex Fermiology and small hybridization gaps near the Fermi energy. Our results provide a unified framework for explaining previous experimental results on CaRuO3, such as its unusual optical conductivity, and demonstrate the importance of octahedral rotations in determining the quasiparticle band structure, and electron correlations in complex transition metal oxides.
The phase diagram of BaVS3 is studied under pressure using resistivity measurements. The temperature of the metal to nonmagnetic Mott insulator transition decreases under pressure, and vanishes at the quantum critical point p_cr=20kbar. We find two kinds of anomalous conducting states. The high-pressure metallic phase is a non-Fermi liquid described by Delta rho = T^n where n=1.2-1.3 at 1K < T < 60K. At p<p_cr, the transition is preceded by a wide precursor region with critically increasing resistivity which we ascribe to the opening of a soft Coulomb gap.
In this paper we study the low temperature behaviors of a system of Bose-Fermi mixtures at two dimensions. Within a self-consistent ladder diagram approximation, we show that at nonzero temperatures $Trightarrow0$ the fermions exhibit non-fermi liquid behavior. We propose that this is a general feature of Bose-Fermi mixtures at two dimensions. An experimental signature of this new state is proposed.
It is well-known that, generically, the one-dimensional interacting fermions cannot be described in terms of the Fermi liquid. Instead, they present different phenomenology, that of the Tomonaga-Luttinger liquid: the Landau quasiparticles are ill-defined, and the fermion occupation number is continuous at the Fermi energy. We demonstrate that suitable fine-tuning of the interaction between fermions can stabilize a peculiar state of one-dimensional matter, which is dissimilar to both the Tomonaga-Luttinger and Fermi liquids. We propose to call this state a quasi-Fermi liquid. Technically speaking, such liquid exists only when the fermion interaction is irrelevant (in the renormalization group sense). The quasi-Fermi liquid exhibits the properties of both the Tomonaga-Luttinger liquid and the Fermi liquid. Similar to the Tomonaga-Luttinger liquid, no finite-momentum quasiparticles are supported by the quasi-Fermi liquid; on the other hand, its fermion occupation number demonstrates finite discontinuity at the Fermi energy, which is a hallmark feature of the Fermi liquid. Possible realization of the quasi-Fermi liquid with the help of cold atoms in an optical trap is discussed.
The magnetic and magnetotransport properties of metallic 1$T$-VTe$_{2}$ single crystals were investigated at temperatures from 1.3 to 300 K and in magnetic fields up to 35 T. Upon applying a high magnetic field, it is found that the electrical resistivity displays a crossover from the logarithmic divergence of the single-impurity Kondo effect to the Fermi liquid behavior at low temperatures. The Brillouin scale of the negative magnetoresistivity above the Kondo temperature $T_{rm{K}}$ = 12 K indicates that the Kondo features originate from intercalated V ions, with $S$ = 1/2. Both magnetic susceptibility and Hall effect show an anomaly around $T_{rm{K}}$. By using the modified Hamann expression we successfully describe the temperature-dependent resistivity under various magnetic fields, which shows the characteristic peak below $T_{rm{K}}$ due to the splitting of the Kondo resonance.
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