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Register a new userPlanar nano-optics in anisotropic media: anomalous refraction and diffraction-free lensing of highly confined polaritons
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As one of the most fundamental optical phenomena, refraction between isotropic media is characterized by light bending towards the normal to the boundary when passing from a low- to a high-refractive-index medium. However, in anisotropic media, refraction is a much more exotic phenomenon. The most general case of refraction between two anisotropic media remains unexplored, particularly in natural media and at the nanoscale. Here, we visualize and comprehensively study refraction of electromagnetic waves between two strongly anisotropic (hyperbolic) media, and, importantly, we do it with the use of polaritons confined to the nanoscale in a low-loss natural medium, alpha-MoO3. Our images show refraction of polaritons under the general case in which both the direction of propagation and the wavevector are not collinear. As they traverse planar nanoprisms tailored in alpha-MoO3, refracted polaritons exhibit non-intuitive directions of propagation, enabling us to unveil an exotic optical effect: bending-free refraction. Furthermore, we succeed in developing the first in-plane refractive hyperlens, which yields foci as small as lamdap/6, being lamdap the polariton wavelength (lamda0/50 with respect to the wavelength of light in free space). Our results set the grounds for planar nano-optics in strongly anisotropic media, with potential for unprecedented control of the flow of energy at the nanoscale.
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2D materials support unique excitations of quasi-particles that consist of a material excitation and photons called polaritons. Especially interesting are in-plane propagating polaritons which can be confined to a single monolayer and carry large momentum. In this work, we report the existence of a new type of in-plane propagating polariton, supported on monolayer transition-metal-dicalcogonide (TMD) in the visible spectrum, which has not yet been observed. This 2D in-plane exciton-polariton (2DEP) is described by the coupling of an electromagnetic light field with the collective oscillations of the excitons supported by monolayer TMDs. We expose the specific experimental conditions required for the excitation of the 2DEP and show that these can be created if the TMD is encapsulated with hexagonal-boron-nitride (hBN) and cooled to cryogenic temperatures. In addition, we compare the properties of the 2DEPs with those of surface-plasmons-polaritons (SPPs) at the same spectral range, and find that the 2DEP exhibit over two orders-of-magnitude larger wavelength confinement. Finally, we propose two configurations for the possible experimental observation of 2DEPs.
We have examined superfluid properties of $^4$He confined to a nano-porous Gelsil glass that has nanopores 2.5 nm in diameter. The pressure-temperature phase diagram was determined by torsional oscillator, heat capacity and pressure studies. The superfluid transition temperature $T_{mathrm c}$ approaches zero at 3.4 MPa, indicating a novel quantum superfluid transition. By heat capacity measurements, the nonsuperfluid phase adjacent to the superfluid and solid phases is identified to be a nanometer-scale, localized Bose condensation state, in which global phase coherence is destroyed. At high pressures, the superfluid density has a $T$-linear term, and $T_{mathrm c}$ is proportional to the zero-temperature superfluid density. These results strongly suggest that phase fluctuations in the superfluid order parameter play a dominant role on the phase diagram and superfluid properties.
We discuss the propagation of an electromagnetic field in an inhomogeneously anisotropic material where the optic axis is rotated in the transverse plane but is invariant along the propagation direction. In such a configuration, the evolution of an electromagnetic wavepacket is governed by the Pancharatnam-Berry phase (PBP), responsible for the appearance of an effective photonic potential. In a recent paper [A. Alberucci et al., Electromagnetic confinement via spin-orbit interaction in anisotropic dielectrics, ACS Photonics textbf{3}, 2249 (2016)] we demonstrated that the effective potential supports transverse confinement. Here we find the profile of the quasi-modes and show that the photonic potential arises from the Kapitza effect of light. The theoretical results are confirmed by numerical simulations, accounting for the medium birefringence. Finally, we analyze in detail a configuration able to support non-leaky guided modes.
High-index dielectrics can confine light into nano-scale leading to enhanced nonlinear response. However, increased momentum in these media can deteriorate the overlap between different harmonics which hinders efficient nonlinear interaction in wavelength-scale resonators in the absence of momentum matching. Here, we propose an alternative approach for light confinement in anisotropic particles. The extra degree of freedom in anisotropic media allows us to control the evanescent waves near the center and the radial momentum away from the center, independently. This can lead to a strong light confinement as well as an excellent field overlap between different harmonics which is ideal for nonlinear wavelength conversion. Controlling the evanescent fields can also help to surpass the constrains on the radiation bandwidth of isotropic dielectric antennas. This can improve the light coupling into these particles, which is crucial for nano-scale nonlinear optics. We estimate the second-harmonic generation efficiency as well as optical parametric oscillation threshold in these particles to show the strong nonlinear response in these particles even away from the center of resonances. Our approach is promising to be realized experimentally and can be used for many applications, such as large-scale parallel sensing and computing.
Localized and propagating polaritons allow for highly sensitive analysis of (bio)chemical substances and processes. Nanoimaging of the polaritons evanescent fields allows for critically important experimental mode identification and for studying field confinement. Here we describe two setups for polariton nanoimaging and spectroscopy in liquid, which is an indispensable environment for (bio)chemical samples. We first demonstrate antenna mapping with a transflection infrared scattering-type scanning near-field optical microscope (s-SNOM), where the tip acts as a near-field scattering probe. We then demonstrate a total internal reflection (TIR) based setup, where the tip is both launching and probing ultra-confined polaritons in van der Waals materials, here phonon polaritons in hexagonal boron nitride (h-BN) flakes. This work lays the foundation for s-SNOM based polariton interferometry in liquid, which has wide application potential for in-situ studies of chemical reactions at the bare or functionalized surface of polaritonic materials, including (bio)chemical recognition analogous to the classical surface plasmon resonance spectroscopy.
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