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Register a new userActivating superconductivity in a repulsive system by high-energy degrees of freedom
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We discuss superconducting pairing in a narrow conduction band sandwiched between unoccupied and occupied bands, an arrangement that enables an unconventional pairing mechanism governed by Coulomb repulsion. Pairing interaction originates from repulsion-assisted scattering between far-out pair states in the higher-energy bands and those at the Fermi level. Optimizing the bandstructure design and carrier density in order to bring plasma frequency below the bandgap renders the repulsion unscreened for the processes with a large frequency transfer. This allows the pairing to fully benefit from the pristine Coulomb repulsion strength. The repulsion-induced attraction is particularly strong in two dimensions and is assisted by a low density of carriers and the resulting low plasma frequency values. We assess the possible connection of this mechanism to superconductivity in magic-angle twisted bilayer graphene where the bandstructure features wide dispersive upper and lower minibands. We use a simple model to illustrate the importance of the far-out pairs in these bands and predict testable signatures of this superconductivity mechanism.
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We discuss a pairing mechanism in interacting two-dimensional multipartite lattices that intrinsically leads to a second order topological superconducting state with a spatially modulated gap. When the chemical potential is close to Dirac points, oppositely moving electrons on the Fermi surface undergo an interference phenomenon in which the Berry phase converts a repulsive electron-electron interaction into an effective attraction. The topology of the superconducting phase manifests as gapped edge modes in the quasiparticle spectrum and Majorana Kramers pairs at the corners. We present symmetry arguments which constrain the possible form of the electron-electron interactions in these systems and classify the possible superconducting phases which result. Exact diagonalization of the Bogoliubov-de Gennes Hamiltonian confirms the existence of gapped edge states and Majorana corner states, which strongly depend on the spatial structure of the gap. Possible applications to vanadium-based superconducting kagome metals AV$_3$Sb$_3$ (A=K,Rb,Cs) are discussed.
The interplay of structural and electronic phases in iron-based superconductors is a central theme in the search for the superconducting pairing mechanism. While electronic nematicity, defined as the breaking of four-fold symmetry triggered by electronic degrees of freedom, is competing with superconductivity, the effect of purely structural orthorhombic order is unexplored. Here, using x-ray diffraction (XRD), we reveal a new structural orthorhombic phase with an exceptionally high onset temperature ($T_mathrm{ort} sim 250$ K), which coexists with superconductivity ($T_mathrm{c} = 25$ K), in an electron-doped iron-pnictide superconductor far from the underdoped region. Furthermore, our angle-resolved photoemission spectroscopy (ARPES) measurements demonstrate the absence of electronic nematic order as the driving mechanism, in contrast to other underdoped iron pnictides where nematicity is commonly found. Our results establish a new, high temperature phase in the phase diagram of iron-pnictide superconductors and impose strong constraints for the modeling of their superconducting pairing mechanism.
We demonstrate that the recently discovered triple-Q (3Q) magnetic structure, when embedded in a magnet-superconductor hybrid (MSH) system, gives rise to the emergence of topological superconductivity. We investigate the structure of chiral Majorana edge modes at domain walls, and show that they can be distinguished from trivial in-gap modes through the spatial distribution of the induced supercurrents. Finally, we show that topological superconductivity in 3Q MSH systems is a robust phenomenon that does not depend on the relative alignment of the magnetic and superconducting layers, or on the presence of electronic degrees of freedom in the magnetic layer.
We present an in-depth classification of the topological phases and Majorana fermion (MF) excitations that arise from the bulk interplay between unconventional multiband spin-singlet superconductivity and various magnetic textures. We focus on magnetic texture crystals with a periodically-repeating primitive cell of the helix, whirl, and skyrmion types. Our analysis is relevant for a wide range of layered materials and hybrid devices, and accounts for both strong and weak, as well as crystalline topological phases. We identify a multitude of accessible topological phases which harbor flat, uni- or bi-directional, (quasi-)helical, or chiral MF edge modes. This rich variety of MFs originates from the interplay between topological phases with gapped and nodal bulk energy spectra, with the resulting types of spectra and MFs controlled by the size of the pairing and magnetic gaps.
Non-trivial topology and unconventional pairing are two central guiding principles in the contemporary search for and analysis of superconducting materials and heterostructure compounds. Previously, a topological superconductor has been predominantly conceived to result from a topologically non-trivial band subject to intrinsic or external superconducting proximity effect. Here, we propose a new class of topological superconductors which are uniquely induced by unconventional pairing. They exhibit a boundary-obstructed higher-order topological character and, depending on their dimensionality, feature unprecedently robust Majorana bound states or hinge modes protected by chiral symmetry. We predict the 112-family of iron pnictides, such as Ca$_{1-x}$La$_x$FeAs$_2$, to be a highly suited material candidate for our proposal, which can be tested by edge spectroscopy. Because of the boundary-obstruction, the topologically non-trivial feature of the 112 pnictides does not reveal itself for a bulk-only torus band analysis without boundaries, and as such had evaded previous investigations. Our proposal not only opens a new arena for highly stable Majorana modes in high-temperature superconductors, but also provides the smoking gun evidence for extended s-wave order in the iron pnictides.
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