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Spontaneous Parametric Down-Conversion from Resonant Metasurfaces

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 Publication date 2021
  fields Physics
and research's language is English




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All-dielectric optical metasurfaces are a workhorse in nano-optics due to both their ability to manipulate light in different degrees of freedom and their excellent performance at light frequency conversion. Here, we demonstrate first-time generation of photon pairs via spontaneous parametric-down conversion in lithium niobate quantum optical metasurfaces with electric and magnetic Mie-like resonances at various wavelengths. By engineering the quantum optical metasurface, we tailor the photon-pair spectrum in a controlled way. Within a narrow bandwidth around the resonance, the rate of pair production is enhanced up to two orders of magnitude compared to an unpatterned film of the same thickness and material. These results enable flat-optics sources of entangled photons -- a new promising platform for quantum optics experiments.



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High-efficient and high-purity photon sources are highly desired for quantum information processing. We report the design of a chip-scale hybrid SixNy and thin film periodically-poled lithium niobate waveguide for generating high-purity type-II spontaneous parametric down conversion (SPDC) photons in telecommunication band. The modeled second harmonic generation efficiency of 225% W^(-1)*cm^(-2) is obtained at 1560nm. Joint spectral analysis is performed to estimate the frequency correlation of SPDC photons, yielding intrinsic purity with up to 95.17%. The generation rate of these high-purity photon pairs is estimated to be 2.87 * 10^7 pairs/s/mW within the bandwidth of SPDC. Our chip-scale hybrid waveguide design has the potential for large scale on-chip quantum information processing and integrated photon-efficient quantum key distribution through high-dimensional time-energy encoding.
Spontaneous Parametric Down-Conversion (SPDC), also known as parametric fluorescence, parametric noise, parametric scattering and all various combinations of the abbreviation SPDC, is a non-linear optical process where a photon spontaneously splits into two other photons of lower energies. One would think that this article is about particle physics and yet it is not, as this process can occur fairly easily on a day to day basis in an optics laboratory. Nowadays, SPDC is at the heart of many quantum optics experiments for applications in quantum cryptography, quantum simulation, quantum metrology but also for testing fundamentals laws of physics in quantum mechanics. In this article, we will focus on the physics of this process and highlight few important properties of SPDC. There will be two parts: a first theoretical one showing the particular quantum nature of SPDC and the second part, more experimental and in particular focusing on applications of parametric down-conversion. This is clearly a non-exhaustive article about parametric down-conversion as there is a tremendous literature on the subject, but it gives the necessary first elements needed for a novice student or researcher to work on SPDC sources of light.
Miniaturised entangled photon sources are highly demanded for the development of integrated quantum photonics. Since the invention of subwavelength optical metasurfaces and their successes at replacing bulky optical components, the possibility of implementing entangled photon sources on such devices is actively investigated. Here, as a first step towards the development of quantum optical metasurfaces (QOM), we demonstrate photon pair generation via spontaneous parametric down-conversion (SPDC) from subwavelength films. We achieved photon pair generation with a high coincidence-to-accidental ratio in lithium niobate and gallium phosphide nanofilms. In addition, we have measured the SPDC frequency spectrum via fibre spectroscopy, obtaining photon pairs with a spectral bandwidth of 500;nm, limited only by the overall detection efficiency. Moreover, we have observed the vacuum field enhancement due to a Fabry-Perot resonance inside the nonlinear films. Our experiments lay the groundwork for the future development of flat SPDC sources, including QOM.
We present an experimental characterization of the statistics of multiple photon pairs produced by spontaneous parametric down-conversion realized in a nonlinear medium pumped by high-energy ultrashort pulses from a regenerative amplifier. The photon number resolved measurement has been implemented with the help of a fiber loop detector. We introduce an effective theoretical description of the observed statistics based on parameters that can be assigned direct physical nterpretation. These parameters, determined for our source from the collected experimental data, characterize the usefulness of down-conversion sources in multiphoton interference schemes that underlie protocols for quantum information processing and communication.
An important step for photonic quantum technologies is the demonstration of a quantum advantage through boson sampling. In order to prevent classical simulability of boson sampling, the photons need to be almost perfectly identical and almost without losses. These two requirements are connected through spectral filtering, improving one leads to a decrease of the other. A proven method of generating single photons is spontaneous parametric downconversion (SPDC). We show that an optimal trade-off between indistinguishability and losses can always be found for SPDC. We conclude that a 50-photon scattershot boson-sampling experiment using SPDC sources is possible from a computational complexity point of view. To this end, we numerically optimize SPDC sources under the regime of weak pumping and with a single spatial mode.
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