Universal size-dependent nonlinear charge transport in single crystals of the Mott insulator Ca2RuO4


Abstract in English

The surprisingly low current densities required for inducing the insulator to metal transition has made Ca$_2$RuO$_4$ an attractive candidate material for developing novel Mott-based electronics devices. The mechanism underlying the resistive switching, however, remains to be a controversial topic in the field of correlated electron systems. Here we report a four orders of magnitude increase in the current density required for driving Ca$_2$RuO$_4$ out of the insulating state upon decreasing the crystal size. We investigate this unprecedented effect by conducting an extensive size-dependent study of electrical transport in high-purity Ca$_2$RuO$_4$ single crystals. We establish that the size dependence is not a result of Joule heating, by integrating a microscopic platinum thermometer. Our detailed study demonstrates that the universally observed transport characteristics of Ca$_2$RuO$_4$ are a result of a strongly inhomogenous current distribution in the nominally homogeneous crystal.

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