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Direct evidence for Cooper pairing without a spectral gap in a disordered superconductor above $T_{C}$

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 Added by Koen Bastiaans
 Publication date 2021
  fields Physics
and research's language is English




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The idea that preformed Cooper pairs could exist in a superconductor above its zero-resistance state has been explored for unconventional, interface, and disordered superconductors, yet direct experimental evidence is lacking. Here, we use scanning tunneling noise spectroscopy to unambiguously show that preformed Cooper pairs exist up to temperatures much higher than the zero-resistance critical temperature $T_{C}$ in the disordered superconductor titanium nitride, by observing a clear enhancement in the shot noise that is equivalent to a change of the effective charge from 1 to 2 electron charges. We further show that spectroscopic gap fills up rather than closes when increasing temperature. Our results thus demonstrate the existence of a novel state above $T_{C}$ that, much like an ordinary metal, has no (pseudo)gap, but carries charge via paired electrons.



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In most superconductors the transition to the superconducting state is driven by the binding of electrons into Cooper-pairs. The condensation of these pairs into a single, phase coherent, quantum state takes place concomitantly with their formation at the transition temperature, $T_c$. A different scenario occurs in some disordered, amorphous, superconductors: Instead of a pairing-driven transition, incoherent Cooper pairs first pre-form above $T_c$, causing the opening of a pseudogap, and then, at $T_c$, condense into the phase coherent superconducting state. Such a two-step scenario implies the existence of a new energy scale, $Delta_{c}$, driving the collective superconducting transition of the preformed pairs. Here we unveil this energy scale by means of Andreev spectroscopy in superconducting thin films of amorphous indium oxide. We observe two Andreev conductance peaks at $pm Delta_{c}$ that develop only below $T_c$ and for highly disordered films on the verge of the transition to insulator. Our findings demonstrate that amorphous superconducting films provide prototypical disordered quantum systems to explore the collective superfluid transition of preformed Cooper-pairs pairs.
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