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Register a new userFractional corner magnetization of collinear antiferromagnets
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Recent studies revealed that the electric multipole moments of insulators result in fractional electric charges localized to the hinges and corners of the sample. We here explore the magnetic analog of this relation. We show that a collinear antiferromagnet with spin $S$ defined on a $d$-dimensional cubic lattice features fractionally quantized magnetization $M_{text{c}}^z=S/2^d$ at the corners. We find that the quantization is robust even in the presence of gapless excitations originating from the spontaneous formation of the Neel order, although the localization length diverges, suggesting a power-law localization of the corner magnetization. When the spin rotational symmetry about the $z$ axis is explicitly broken, the corner magnetization is no longer sharply quantized. Even in this case, we numerically find that the deviation from the quantized value is negligibly small based on quantum Monte Carlo simulations.
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Recent developments in higher-order topological phases have elucidated on the relationship between nontrivial multipole moments in the bulk and the emergence of fractionally quantized charges at the boundary. Here, we put on the table a proposal of the three-dimensional octupole insulator with fractionally quantized corner charges $pm e/8$: sodium chloride, commonly known as table salt. The fractional quantization of the corner charge is unaffected by the quantum fluctuation of the electric charge per ion, as we demonstrate explicitly with ab initio calculations. We further show that the electrostatic signature of the fractional charge is well-preserved even when the ideal crystal is sprinkled with defects, and provide a systematic analysis on how the corner charge contribution could be isolated from the electric-field corrections originating from realistic surface relaxation. Our results suggest that the observation of corner charges from quantized multipole moments in solids might be around the corner.
We discuss the ground-state degeneracy of spin-$1/2$ kagome-lattice quantum antiferromagnets on magnetization plateaus by employing two complementary methods: the adiabatic flux insertion in closed boundary conditions and a t Hooft anomaly argument on inherent symmetries in a quasi-one-dimensional limit. The flux insertion with a tilted boundary condition restricts the lower bound of the ground-state degeneracy on $1/9$, $1/3$, $5/9$, and $7/9$ magnetization plateaus under the $mathrm{U(1)}$ spin-rotation and the translation symmetries: $3$, $1$, $3$, and $3$, respectively. This result motivates us further to develop an anomaly interpretation of the $1/3$ plateau. Taking advantage of the insensitivity of anomalies to spatial anisotropies, we examine the existence of the unique gapped ground state on the $1/3$ plateau from a quasi-one-dimensional viewpoint. In the quasi-one-dimensional limit, kagome antiferromagnets are reduced to weakly coupled three-leg spin tubes. Here, we point out the following anomaly description of the $1/3$ plateau. While a simple $S=1/2$ three-leg spin tube cannot have the unique gapped ground state on the $1/3$ plateau because of an anomaly between a $mathbb Z_3times mathbb Z_3$ symmetry and the translation symmetry at the $1/3$ filling, the kagome antiferromagnet breaks explicitly one of the $mathbb Z_3$ symmetries related to a $mathbb Z_3$ cyclic transformation of spins in the unit cell. Hence the kagome antiferromagnet can have the unique gapped ground state on the $1/3$ plateau.
A formula for the corner charge in terms of the bulk quadrupole moment is derived for two-dimensional periodic systems. This is an analog of the formula for the surface charge density in terms of the bulk polarization. In the presence of an $n$-fold rotation symmetry with $n=3$, $4$, and $6$, the quadrupole moment is quantized and is independent of the spread or shape of Wannier orbitals, depending only on the location of Wannier centers of filled bands. In this case, our formula predicts the fractional part of the quadrupole moment purely from the bulk property. The system can contain many-body interactions as long as the ground state is gapped and topologically trivial in the sense it is smoothly connected to a product state limit. An extension of these results to three-dimensional systems is also discussed. In three dimensions, in general, even the fractional part of the corner charge is not fully predictable from the bulk perspective even in the presence of point group symmetry.
The Casimir effect is a general phenomenon in physics, which arises when the vacuum fluctuation of an arbitrary field is modified by static or slowly varying boundary. However, its spin version is rarely addressed, mainly due to the fact that a macroscopic boundary in quantum spin systems is hard to define. In this article, we explore the spin Casimir effect induced by the zero-point fluctuation of spin waves in a general non-collinear ordered quantum antiferromagnet. This spin Casimir effect results in a spin torque between local spins and further causes various singular and divergent results in the framework of spin-wave theory, which invalidate the standard $1/S$ expansion procedure. To avoid this dilemma, we develop a self-consistent spin-wave expansion approach, which preserves the spin-wave expansion away from singularities and divergence. A detailed spin-wave analysis of the antiferromagnetic spin-1/2 Heisenberg model on a spatially anisotropic triangular lattice is undertaken within our approach. Our results indicate that the spiral order is only stable in the region $0.5<alpha<1.2$, where $alpha$ is the ratio of the coupling constants. In addition, the instability in the region $1.2<alpha<2$ is owing to the spin Casimir effect instead of the vanishing sublattice magnetization. And this extended spiral instable region may host some quantum disordered phases besides the quantum order by disorder induced Neel phase. Furthermore, our method provides an efficient and convenient tool that can estimate the correct exchange parameters and outline the quantum phase diagrams, which can be useful for experimental fitting processes in frustrated quantum magnets.
The classical spin-flop is the field-driven first-order reorientation transition in easy-axis antiferromagnets. A comprehensive phenomenological theory of easy-axis antiferromagnets displaying spin-flops is developed. It is shown how the hierarchy of magnetic coupling strengths in these antiferromagnets causes a strongly pronounced two-scale character in their magnetic phase structure. In contrast to the major part of the magnetic phase diagram, these antiferromagnets near the spin-flop region are described by an effective model akin to uniaxial ferromagnets. For a consistent theoretical description both higher-order anisotropy contributions and dipolar stray-fields have to be taken into account near the spin-flop. In particular, thermodynamically stable multidomain states exist in the spin-flop region, owing to the phase coexistence at this first-order transition. For this region, equilibrium spin-configurations and parameters of the multidomain states are derived as functions of the external magnetic field. The components of the magnetic susceptibility tensor are calculated for homogeneous and multidomain states in the vicinity of the spin-flop. The remarkable anomalies in these measurable quantities provide an efficient method to investigate magnetic states and to determine materials parameters in bulk and confined antiferromagnets, as well as in nanoscale synthetic antiferromagnets. The method is demonstrated for experimental data on the magnetic properties near the spin-flop region in the orthorhombic layered antiferromagnet (C_2H_5NH_3)_2CuCl_4.
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