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Register a new userSpin-polarized imaging of strongly interacting fermions in the ferrimagnetic state of Weyl candidate CeBi
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CeBi has an intricate magnetic phase diagram whose fully-polarized state has recently been suggested as a Weyl semimetal, though the role of $f$ states in promoting strong interactions has remained elusive. Here we focus on the less-studied, but also time-reversal symmetry-breaking ferrimagnetic phase of CeBi, where our density functional theory (DFT) calculations predict additional Weyl nodes near the Fermi level $E_mathrm{F}$. We use spin-polarized scanning tunneling microscopy and spectroscopy to image the surface ferrimagnetic order on the itinerant Bi $p$ states, indicating their orbital hybridization with localized Ce $f$ states. We observe suppression of this spin-polarized signature at $E_mathrm{F}$, coincident with a Fano line shape in the conductance spectra, suggesting the Bi $p$ states partially Kondo screen the $f$ magnetic moments, and this $p-f$ hybridization causes strong Fermi-level band renormalization. The $p$ band flattening is supported by our quasiparticle interference (QPI) measurements, which also show band splitting in agreement with DFT, painting a consistent picture of a strongly interacting magnetic Weyl semimetal.
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We predict that CeBi in the ferromagnetic state is a Weyl semimetal. Our calculations within density functional theory show the existence of two pairs of Weyl nodes on the momentum path $(0, 0, k_z)$ at $15$ meV} above and $100$ meV below the Fermi level. Two corresponding Fermi arcs are obtained on surfaces of mirror-symmetric (010)-oriented slabs at $E=15$ meV and both arcs are interrupted into three segments due to hybridization with a set of trivial surface bands. By studying the spin texture of surface states, we find the two Fermi arcs are strongly spin-polarized but in opposite directions, which can be detected by spin-polarized ARPES measurements. Our theoretical study of quasiparticle interference (QPI) for a nonmagnetic impurity at the Bi site also reveals several features related to the Fermi arcs. Specifically, we predict that the spin polarization of the Fermi arcs leads to a bifurcation-shaped feature only in the spin-dependent QPI spectrum, serving as a fingerprint of the Weyl nodes.
Linear dichroism -- the polarization dependent absorption of electromagnetic waves -- is routinely exploited in applications as diverse as structure determination of DNA or polarization filters in optical technologies. Here filamentary absorbers with a large length-to-width ratio are a prerequisite. For magnetization dynamics in the few GHz frequency regime strictly linear dichroism was not observed for more than eight decades. Here, we show that the bulk chiral magnet Cu$_{2}$OSeO$_{3}$ exhibits linearly polarized magnetization dynamics at an unexpectedly small frequency of about 2 GHz. Unlike optical filters that are assembled from filamentary absorbers, the magnet provides linear polarization as a bulk material for an extremely wide range of length-to-width ratios. In addition, the polarization plane of a given mode can be switched by 90$^circ$ via a tiny variation in width. Our findings shed a new light on magnetization dynamics in that ferrimagnetic ordering combined with anisotropic exchange interaction offers strictly linear polarization and cross-polarized modes for a broad spectrum of sample shapes. The discovery allows for novel design rules and optimization of microwave-to-magnon transduction in emerging microwave technologies.
Materials where the electronic bands have unusual topologies allow for the realization of novel physics and have a wide range of potential applications. When two electronic bands with linear dispersions intersect at a point, the excitations could be described as Weyl fermions which are massless particles with a particular chirality. Here we report evidence for the presence of Weyl fermions in the ferromagnetic state of the low-carrier density, strongly correlated Kondo lattice system CeSb, from electronic structure calculations and angle-dependent magnetoresistance measurements. When the applied magnetic field is parallel to the electric current, a pronounced negative magnetoresistance is observed within the ferromagnetic state, which is destroyed upon slightly rotating the field away. These results give evidence for CeSb belonging to a new class of Kondo lattice materials with Weyl fermions in the ferromagnetic state.
We have developed a polarized hard X-ray photoemission (HAXPES) system to study the ground-state symmetry of strongly correlated materials. The linear polarization of the incoming X-ray beam is switched by the transmission-type phase retarder composed of two diamond (100) crystals. The best degree of the linear polarization $P_L$ is $-0.96$, containing the vertical polarization component of 98%. A newly developed low temperature two-axis manipulator enables easy polar and azimuthal rotations to select the detection direction of photoelectrons. The lowest temperature achieved is 9 K, offering us a chance to access the ground state even for the strongly correlated electron systems in cubic symmetry. The co-axial sample monitoring system with the long-working-distance microscope enables us to keep measuring the same region on the sample surface before and after rotation procedures. Combining this sample monitoring system with a micro-focused X-ray beam by means of an ellipsoidal Kirkpatrick-Baez mirror (25 $mu$m $times$ 25 $mu$m (FWHM)), we have demonstrated the polarized valence-band HAXPES on NiO for voltage application as resistive random access memories to reveal the origin of the metallic spectral weight near the Fermi level.
A combined analytical and numerical study is performed of the mapping between strongly interacting fermions and weakly interacting spins, in the framework of the Hubbard, t-J and Heisenberg models. While for spatially homogeneous models in the thermodynamic limit the mapping is thoroughly understood, we here focus on aspects that become relevant in spatially inhomogeneous situations, such as the effect of boundaries, impurities, superlattices and interfaces. We consider parameter regimes that are relevant for traditional applications of these models, such as electrons in cuprates and manganites, and for more recent applications to atoms in optical lattices. The rate of the mapping as a function of the interaction strength is determined from the Bethe-Ansatz for infinite systems and from numerical diagonalization for finite systems. We show analytically that if translational symmetry is broken through the presence of impurities, the mapping persists and is, in a certain sense, as local as possible, provided the spin-spin interaction between two sites of the Heisenberg model is calculated from the harmonic mean of the onsite Coulomb interaction on adjacent sites of the Hubbard model. Numerical calculations corroborate these findings also in interfaces and superlattices, where analytical calculations are more complicated.
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