Electric field and substrate effects dominate spin-phonon relaxation in graphene


Abstract in English

Experimental spin relaxation times in graphene, critical for spintronics and quantum information technologies, are two orders of magnitude below previous theoretical predictions for spin-phonon relaxation. Here, ab initio density-matrix dynamics simulations reveal that electric fields and substrates strongly reduce spin-phonon relaxation time to the nanosecond scale, in agreement with experiments. Our predicted out-of-plane to in-plane lifetime ratio exceeds 1/2 on boron nitride substrates, matching experiment unlike previous models, suggesting that spin-phonon relaxation is dominant in graphene at room temperature.

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