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Non-orthogonal Spin-Momentum Locking

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 Added by T. Hakioglu
 Publication date 2020
  fields Physics
and research's language is English




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Spin-momentum locking is a unique feature of spin-orbit coupled materials and a key to their promise of applications in spintronics and quantum computation. Much of the existing work has been focused on an orthogonal locking between the directions of spin and momentum vectors in the context of both topological and non-topological materials. Mechanisms responsible for non-orthogonal spin-momentum locking (NOSML) have drawn little attention, although an NOSML effect has been reported on the topological surface of $alpha$-$Sn$. Here, we demonstrate how spin-orbit scattering from non-magnetic impurities can produce the NOSML state. The parameter describing spin-orbit coupling strength in our analysis of the NOMSL could be extracted directly from the spin-resolved angle-resolved photoemission (S-ARPES) spectra. Our formalism is applicable to all spin-orbit coupled systems and not limited only to topological states. An understanding of NOSML effects bears on spin-orbit dependent phenomena more generally, including issues of spin-to-charge conversion and the interpretation of quasiparticle interference (QPI) patterns and scanning-tunneling spectra (STS) in materials.



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Three-dimensional (3D) topological insulators (TIs) are known to carry 2D Dirac-like topological surface states in which spin-momentum locking prohibits backscattering. When thinned down to a few nanometers, the hybridization between the topological surface states at the top and bottom surfaces results in a topological quantum phase transition, which can lead to the emergence of a quantum spin Hall phase. Here, we study the thickness-dependent transport properties across the quantum phase transition on the example of (Bi$_{0.16}$Sb$_{0.84}$)$_2$Te$_3$ films, with a four-tip scanning tunnelling microscope. Our findings reveal an exponential drop of the conductivity below the critical thickness. The steepness of this drop indicates the presence of spin-conserving backscattering between the top and bottom surface states, effectively lifting the spin-momentum locking and resulting in the opening of a gap at the Dirac point. Our experiments provide crucial steps towards the detection of quantum spin Hall states in transport measurements.
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