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Dynamical generation of spin squeezing in ultra-cold dipolar molecules

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 Added by Thomas Bilitewski
 Publication date 2020
  fields Physics
and research's language is English




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We study a bulk fermionic dipolar molecular gas in the quantum degenerate regime confined in a two-dimensional geometry. We consider two rotational states that encode a spin 1/2 degree of freedom. We derive a long-range interacting XXZ model describing the many-body spin dynamics of the molecules valid in the regime where motional degrees of freedom are frozen. Due to the spatially extended nature of the harmonic oscillator modes, the interactions in the spin model are very long-ranged and the system behaves close to the collective limit, resulting in robust dynamics and generation of entanglement in the form of spin squeezing even at finite temperature and in presence of dephasing and chemical reactions. We demonstrate how the internal state structure can be exploited to realise time-reversal and enhanced metrological sensing protocols.

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We investigate many-body spin squeezing dynamics in an XXZ model with interactions that fall off with distance $r$ as $1/r^alpha$ in $D=2$ and $3$ spatial dimensions. In stark contrast to the Ising model, we find a broad parameter regime where spin squeezing comparable to the infinite-range $alpha=0$ limit is achievable even when interactions are short-ranged, $alpha>D$. A region of collective behavior in which optimal squeezing grows with system size extends all the way to the $alphatoinfty$ limit of nearest-neighbor interactions. Our predictions, made using the discrete truncated Wigner approximation (DTWA), are testable in a variety of experimental cold atomic, molecular, and optical platforms.
We demonstrate two simple theorems about squeezing induced by bilinear spin-spin interactions that conserve spin parity -- including a vast majority of quantum spin models implemented by state-of-the-art quantum simulators. In particular we show that squeezing captures the first form of quantum correlations which are produced: 1) at equilibrium, by adiabatically turning on the spin-spin interactions starting from a factorized state aligned with an external, arbitrary field; 2) away from equilibrium, by evolving unitarily the same state with the interacting Hamiltonian.
107 - K.-K. Ni , S. Ospelkaus , D. Wang 2010
Ultracold polar molecules offer the possibility of exploring quantum gases with interparticle interactions that are strong, long-range, and spatially anisotropic. This is in stark contrast to the dilute gases of ultracold atoms, which have isotropic and extremely short-range, or contact, interactions. The large electric dipole moment of polar molecules can be tuned with an external electric field; this provides unique opportunities such as control of ultracold chemical reactions, quantum information processing, and the realization of novel quantum many-body systems. In spite of intense experimental efforts aimed at observing the influence of dipoles on ultracold molecules, only recently have sufficiently high densities been achieved. Here, we report the observation of dipolar collisions in an ultracold molecular gas prepared close to quantum degeneracy. For modest values of an applied electric field, we observe a dramatic increase in the loss rate of fermionic KRb molecules due to ultrcold chemical reactions. We find that the loss rate has a steep power-law dependence on the induced electric dipole moment, and we show that this dependence can be understood with a relatively simple model based on quantum threshold laws for scattering of fermionic polar molecules. We directly observe the spatial anisotropy of the dipolar interaction as manifested in measurements of the thermodynamics of the dipolar gas. These results demonstrate how the long-range dipolar interaction can be used for electric-field control of chemical reaction rates in an ultracold polar molecule gas. The large loss rates in an applied electric field suggest that creating a long-lived ensemble of ultracold polar molecules may require confinement in a two-dimensional trap geometry to suppress the influence of the attractive dipolar interactions.
There has been a recent surge of interest and progress in creating subwavelength free-space optical potentials for ultra-cold atoms. A key open question is whether geometric potentials, which are repulsive and ubiquitous in the creation of subwavelength free-space potentials, forbid the creation of narrow traps with long lifetimes. Here, we show that it is possible to create such traps. We propose two schemes for realizing subwavelength traps and demonstrate their superiority over existing proposals. We analyze the lifetime of atoms in such traps and show that long-lived bound states are possible. This work opens a new frontier for the subwavelength control and manipulation of ultracold matter, with applications in quantum chemistry and quantum simulation.
We show that indirect spin-spin interactions between effective spin-1/2 systems can be realized in two parallel 1D optical lattices loaded with polar molecules and/or Rydberg atoms. The effective spin can be encoded into low-energy rotational states of polar molecules or long-lived states of Rydberg atoms, tightly trapped in a deep optical lattice. The spin-spin interactions can be mediated by Rydberg atoms, placed in a parallel shallow optical lattice, interacting with the effective spins by charge-dipole (for polar molecules) or dipole-dipole (for Rydberg atoms) interaction. Indirect XX, Ising and XXZ interactions with interaction coefficients $J^{bot}$ and $J^{zz}$ sign varying with interspin distance can be realized, in particular, the $J_{1}-J_{2}$ XXZ model with frustrated ferro-(antiferro-)magnetic nearest (next-nearest) neighbor interactions.
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