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Tackling the phase problem of diffraction for retrieval of photonic structures formed in nanocomposite materials

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 Added by Juergen Klepp
 Publication date 2020
  fields Physics
and research's language is English




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We experimentally demonstrate how to solve the phase problem of diffraction using multi-wave interference with standard diffraction experimental setups without the need for taking any auxiliary data. In particular, we show that the phases of the Fourier components of a periodic structure can be fully recovered by deliberately choosing a probe wavelength of the diffracting radiation much smaller than the lattice constant. In the course of the demonstration, we accurately determine the refractive index profile of nanocomposite phase gratings by light and neutron diffraction measurements.



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Refraction and diffraction of waves in natural crystals and artificial crystals formed by anisotropically scattering centers are considered. A detailed study of the electromagnetic wave refraction in a two-dimensional photonic crystal formed by parallel threads is given by way of example. The expression is derived for the effective amplitude of wave scattering by a thread (in a crystal) for the case when scattering by a single thread in a vacuum is anisotropic. It is established that for a wave with orthogonal polarization, unlike a wave with parallel polarization, the index of refraction in crystals built from metallic threads can be greater than unity, and Vavilov-Chrernkov radiation becomes possible in them. The set of equations describing the dynamical diffraction of waves in crystals is derived for the case when scattering by a single center in a vacuum is anisotropic. Because a most general approach is applied to the description of the scattering process, the results thus obtained are valid for a wide range of cases without being restricted to either electromagnetic waves or crystals built from threads.
In both light optics and electron optics, the amplitude of a wave scattered by an object is an observable that is usually recorded in the form of an intensity distribution in a real space image or a diffraction image. In contrast, retrieval of the phase of a scattered wave is a well-known challenge, which is usually approached by interferometric or numerical methods. In electron microscopy, as a result of constraints in the lens setup, it is particularly difficult to retrieve the phase of a diffraction image. Here, we use a defocused beam generated by a nanofabricated hologram to form a reference wave that can be interfered with a diffracted beam. This setup provides an extended interference region with the sample wavefunction in the Fraunhofer plane. As a case study, we retrieve the phase of an electron vortex beam. Beyond this specific example, the approach can be used to retrieve the wavefronts of diffracted beams from a wide range of samples.
Coherent diffraction imaging (CDI) is high-resolution lensless microscopy that has been applied to image a wide range of specimens using synchrotron radiation, X-ray free electron lasers, high harmonic generation, soft X-ray laser and electrons. Despite these rapid advances, it remains a challenge to reconstruct fine features in weakly scattering objects such as biological specimens from noisy data. Here we present an effective iterative algorithm, termed oversampling smoothness (OSS), for phase retrieval of noisy diffraction intensities. OSS exploits the correlation information among the pixels or voxels in the region outside of a support in real space. By properly applying spatial frequency filters to the pixels or voxels outside the support at different stage of the iterative process (i.e. a smoothness constraint), OSS finds a balance between the hybrid input-output (HIO) and error reduction (ER) algorithms to search for a global minimum in solution space, while reducing the oscillations in the reconstruction. Both our numerical simulations with Poisson noise and experimental data from a biological cell indicate that OSS consistently outperforms the HIO, ER-HIO and noise robust (NR)-HIO algorithms at all noise levels in terms of accuracy and consistency of the reconstructions. We expect OSS to find application in the rapidly growing CDI field as well as other disciplines where phase retrieval from noisy Fourier magnitudes is needed.
Here we would like to discuss the light transmission modulation by periodic and disordered one dimensional (1D) photonic structures. In particular, we will present some theoretical and experimental findings highlighting the peculiar optical properties of: i) 1D periodic and disordered photonic structures made with two or more materials; ii) 1D photonic structures in which the homogeneity or the aggregation of the high refractive index layers is controlled. We will focus also on the fabrication aspects of these structures.
We demonstrate that light is subject to anomalous (i.e., negative) diffraction when propagating in the presence of hyperbolic dispersion. We show that light propagation in hyperbolic media resembles the dynamics of a quantum particle of negative mass moving in a two-dimensional potential. The negative effective mass implies time reversal if the medium is homogeneous. Such property paves the way to diffraction compensation, spatial analogue of dispersion compensating fibers in the temporal domain. At variance with materials exhibiting standard elliptic dispersion, in inhomogeneous hyperbolic materials light waves are pulled towards regions with a lower refractive index. In the presence of a Kerr-like optical response, bright (dark) solitons are supported by a negative (positive) nonlinearity.
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