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Register a new userSingle organic molecules for photonic quantum technologies
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Isolating single molecules in the solid state has allowed fundamental experiments in basic and applied sciences. When cooled down to liquid helium temperature, certain molecules show transition lines, that are tens of megahertz wide, limited only by the excited state lifetime. The extreme flexibility in the synthesis of organic materials provides, at low costs, a wide palette of emission wavelengths and supporting matrices for such single chromophores. In the last decades, the controlled coupling to photonic structures has led to an optimized interaction efficiency with light. Molecules can hence be operated as single photon sources and as non-linear elements with competitive performance in terms of coherence, scalability and compatibility with diverse integrated platforms. Moreover, they can be used as transducers for the optical read-out of fields and material properties, with the promise of single-quanta resolution in the sensing of charges and motion. We show that quantum emitters based on single molecules hold promise to play a key role in the development of quantum science and technologies.
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Large-scale quantum technologies require exquisite control over many individual quantum systems. Typically, such systems are very sensitive to environmental fluctuations, and diagnosing errors via measurements causes unavoidable perturbations. In this work we present an in situ frequency locking technique that monitors and corrects frequency variations in single photon sources based on microring resonators. By using the same classical laser fields required for photon generation as a probe to diagnose variations in the resonator frequency, our protocol applies feedback control to correct photon frequency errors in parallel to the optical quantum computation without disturbing the physical qubit. We implement our technique on a silicon photonic device and demonstrate sub 1 pm frequency stabilization in the presence of applied environmental noise, corresponding to a fractional frequency drift of <1 % of a photon linewidth. Using these methods we demonstrate feedback controlled quantum state engineering. By distributing a single local oscillator across a single chip or network of chips, our approach enables frequency locking of many single photon sources for large-scale photonic quantum technologies.
Current proposals for scalable photonic quantum technologies require on-demand sources of indistinguishable single photons with very high efficiency (having unheralded loss below $1%$). Even with recent progress in the field there is still a significant gap between the requirements and state of the art performance. Here, we propose an on-chip source of multiplexed, heralded photons. Using quantum feedback control on a photon storage cavity with an optimized driving protocol, we estimate an on-demand efficiency of $99%$ and unheralded loss of order $1%$, assuming high efficiency detectors and intrinsic cavity quality factors of order $10^8$. We further explain how temporal- and frequency-multiplexing can be used in parallel to significantly reduce device requirements if single photon frequency conversion is possible with efficiency in the same range of $99%$.
Rare-earth ions in crystals are a proven solid-state platform for quantum technologies in the ensemble regime and attractive for new opportunities at the single ion level. Among the trivalent rare earths, ${}^{171}mathrm{Yb}^{3+}$ is unique in that it possesses a single 4f excited-state manifold and is the only paramagnetic isotope with a nuclear spin of 1/2. In this work, we present measurements of the optical and spin properties of $^{171}$Yb$^{3+}$:YVO$_4$ to assess whether this distinct energy level structure can be harnessed for quantum interfaces. The material was found to possess large optical absorption compared to other rare-earth-doped crystals owing to the combination of narrow inhomogeneous broadening and a large transition oscillator strength. In moderate magnetic fields, we measure optical linewidths less than 3 kHz and nuclear spin linewidths less than 50 Hz. We characterize the excited-state hyperfine and Zeeman interactions in this system, which enables the engineering of a $Lambda$-system and demonstration of all-optical coherent control over the nuclear spin ensemble. Given these properties, $^{171}$Yb$^{3+}$:YVO$_4$ has significant potential for building quantum interfaces such as ensemble-based memories, microwave-to-optical transducers, and optically addressable single rare-earth-ion spin qubits.
Quantum networks play a crucial role for distributed quantum information processing, enabling the establishment of entanglement and quantum communication among distant nodes. Fundamentally, networks with independent sources allow for new forms of nonlocality, beyond the paradigmatic Bells theorem. Here we implement the simplest of such networks -- the bilocality scenario -- in an urban network connecting different buildings with a fully scalable and hybrid approach. Two independent sources using different technologies, respectively a quantum dot and a nonlinear crystal, are used to share photonic entangled state among three nodes connected through a 270 m free-space channel and fiber links. By violating a suitable non-linear Bell inequality, we demonstrate the nonlocal behaviour of the correlations among the nodes of the network. Our results pave the way towards the realization of more complex networks and the implementation of quantum communication protocols in an urban environment, leveraging on the capabilities of hybrid photonic technologies.
The generation, manipulation and detection of quantum bits (qubits) encoded on single photons is at the heart of quantum communication and optical quantum information processing. The combination of single-photon sources, passive optical circuits and single-photon detectors enables quantum repeaters and qubit amplifiers, and also forms the basis of all-optical quantum gates and of linear-optics quantum computing. However, the monolithic integration of sources, waveguides and detectors on the same chip, as needed for scaling to meaningful number of qubits, is very challenging, and previous work on quantum photonic circuits has used external sources and detectors. Here we propose an approach to a fully-integrated quantum photonic circuit on a semiconductor chip, and demonstrate a key component of such circuit, a waveguide single-photon detector. Our detectors, based on superconducting nanowires on GaAs ridge waveguides, provide high efficiency (20%) at telecom wavelengths, high timing accuracy (60 ps), response time in the ns range, and are fully compatible with the integration of single-photon sources, passive networks and modulators.
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