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Acoustic twisted bilayer graphene

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 Added by Harris Pirie
 Publication date 2020
  fields Physics
and research's language is English




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Twisted van der Waals (vdW) heterostructures have recently emerged as an attractive platform to study tunable correlated electron systems. However, the quantum mechanical nature of vdW heterostructures makes their theoretical and experimental exploration laborious and expensive. Here we present a simple platform to mimic the behavior of twisted vdW heterostructures using acoustic metamaterials comprising of interconnected air cavities in a steel plate. Our classical analog of twisted bilayer graphene shows much of the same behavior as its quantum counterpart, including mode localization at a magic angle of about 1.1 degrees. By tuning the thickness of the interlayer membrane, we reach a regime of strong interactions more than three times higher than the feasible range of twisted bilayer graphene under pressure. In this regime, we find the magic angle as high as 6.01 degrees, corresponding to a far denser array of localized modes in real space and further increasing their interaction strength. Our results broaden the capabilities for cross-talk between quantum mechanics and acoustics, as vdW metamaterials can be used both as simplified models for exploring quantum systems and as a means for translating interesting quantum effects into acoustics.



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Using terahertz time-domain spectroscopy, the real part of optical conductivity [$sigma_{1}(omega)$] of twisted bilayer graphene was obtained at different temperatures (10 -- 300 K) in the frequency range 0.3 -- 3 THz. On top of a Drude-like response, we see a strong peak in $sigma_{1} (omega)$ at $sim$2.7 THz. We analyze the overall Drude-like response using a disorder-dependent (unitary scattering) model, then attribute the peak at 2.7 THz to an enhanced density of states at that energy, that is caused by the presence of a van Hove singularity arising from a commensurate twisting of the two graphene layers.
Flatbands with extremely narrow bandwidths on the order of a few mili-electron volts can appear in twisted multilayer graphene systems for appropriate system parameters. Here we investigate the electronic structure of a twisted bi-bilayer graphene, or twisted double bilayer graphene, to find the parameter space where isolated flatbands can emerge as a function of twist angle, vertical pressure, and interlayer potential differences. We find that in twisted bi-bilayer graphene the bandwidth is generally flatter than in twisted bilayer graphene by roughly up to a factor of two in the same parameter space of twist angle $theta$ and interlayer coupling $omega$, making it in principle simpler to tailor narrow bandwidth flatbands. Application of vertical pressure can enhance the first magic angle in minimal models at $theta sim 1.05^{circ}$ to larger values of up to $theta sim 1.5^{circ}$ when $ P sim 2.5$~GPa, where $theta propto omega/ upsilon_{F}$. Narrow bandwidths are expected in bi-bilayers for a continuous range of small twist angles, i.e. without magic angles, when intrinsic bilayer gaps open by electric fields, or due to remote hopping terms. We find that moderate vertical electric fields can contribute in lifting the degeneracy of the low energy flatbands by enhancing the primary gap near the Dirac point and the secondary gap with the higher energy bands. Distinct valley Chern bands are expected near $0^{circ}$ or $180^{circ}$ alignments.
We study the electronic properties of twisted bilayers graphene in the tight-binding approximation. The interlayer hopping amplitude is modeled by a function, which depends not only on the distance between two carbon atoms, but also on the positions of neighboring atoms as well. Using the Lanczos algorithm for the numerical evaluation of eigenvalues of large sparse matrices, we calculate the bilayer single-electron spectrum for commensurate twist angles in the range $1^{circ}lesssimthetalesssim30^{circ}$. We show that at certain angles $theta$ greater than $theta_{c}approx1.89^{circ}$ the electronic spectrum acquires a finite gap, whose value could be as large as $80$ meV. However, in an infinitely large and perfectly clean sample the gap as a function of $theta$ behaves non-monotonously, demonstrating exponentially-large jumps for very small variations of $theta$. This sensitivity to the angle makes it impossible to predict the gap value for a given sample, since in experiment $theta$ is always known with certain error. To establish the connection with experiments, we demonstrate that for a system of finite size $tilde L$ the gap becomes a smooth function of the twist angle. If the sample is infinite, but disorder is present, we expect that the electron mean-free path plays the same role as $tilde L$. In the regime of small angles $theta<theta_c$, the system is a metal with a well-defined Fermi surface which is reduced to Fermi points for some values of $theta$. The density of states in the metallic phase varies smoothly with $theta$.
We present transport measurements of bilayer graphene with 1.38{deg} interlayer twist and apparent additional alignment to its hexagonal boron nitride cladding. As with other devices with twist angles substantially larger than the magic angle of 1.1{deg}, we do not observe correlated insulating states or band reorganization. However, we do observe several highly unusual behaviors in magnetotransport. For a large range of densities around half filling of the moire bands, magnetoresistance is large and quadratic. Over these same densities, the magnetoresistance minima corresponding to gaps between Landau levels split and bend as a function of density and field. We reproduce the same splitting and bending behavior in a simple tight-binding model of Hofstadters butterfly on a square lattice with anisotropic hopping terms. These features appear to be a generic class of experimental manifestations of Hofstadters butterfly and may provide insight into the emergent states of twisted bilayer graphene.
The effects of the long range electrostatic interaction in twisted bilayer graphene are described using the Hartree-Fock approximation. The results show a significant dependence of the band widths and shapes on electron filling, and the existence of broken symmetry phases at many densities, either valley/spin polarized, with broken sublattice symmetry, or both.
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