No Arabic abstract
This paper represents a theoretical and an experimental study of the spreading dynamics of a liquid droplet, generated by a needle free deposition system called the liquid needle droplet deposition technique. This technique utilizes a continuous liquid jet generated from a pressurized dosing system which generates a liquid drop on a substrate to be characterized by optical contact angle measurements. Although many studies have explored the theoretical modelling of the droplet spreading scenario, a theoretical model representing the spreading dynamics of a droplet, generated by the jet impact and continuous addition of liquid mass, is yet to be addressed. In this study, we developed a theoretical model based on the overall energy balance approach which enables us to study on the physics of variation of droplet spreading under surrounding medium of various viscosities. The numerical solution of the non-linear ordinary differential equation has provided us the opportunity to comment on the variation of droplet spreading, as a function of Weber number ($We$), Reynolds number ($Re$) and Bond number ($Bo$) ranging from 0.5-3, 75-150, and 0.001-0.3, respectively. We have also presented a liquid jet impact model in order to predict the initial droplet diameter as an initial condition for the proposed governing equation. The model has been verified further with the experimental measurements and reasonable agreement has been observed. Experimental observations and theoretical investigations also highlight the precision, repeatability and wide range of the applicability of liquid needle drop deposition technique.
Marangoni instabilities can emerge when a liquid interface is subjected to a concentration or temperature gradient. It is generally believed that for these instabilities bulk effects like buoyancy are negligible as compared to interfacial forces, especially on small scales. Consequently, the effect of a stable stratification on the Marangoni instability has hitherto been ignored. Here we report, for an immiscible drop immersed in a stably stratified ethanol-water mixture, a new type of oscillatory solutal Marangoni instability which is triggered once the stratification has reached a critical value. We experimentally explore the parameter space spanned by the stratification strength and the drop size and theoretically explain the observed crossover from levitating to bouncing by balancing the advection and diffusion around the drop. Finally, the effect of the stable stratification on the Marangoni instability is surprisingly amplified in confined geometries, leading to an earlier onset.
Liquid drops and vibrations are ubiquitous in both everyday life and technology, and their combination can often result in fascinating physical phenomena opening up intriguing opportunities for practical applications in biology, medicine, chemistry and photonics. Here we study, theoretically and experimentally, the response of pancake-shaped liquid drops supported by a solid plate that vertically vibrates at a single, low acoustic range frequency. When the vibration amplitudes are small, the primary response of the drop is harmonic at the frequency of the vibration. However, as the amplitude increases, the half-frequency subharmonic Faraday waves are excited parametrically on the drop surface. We develop a simple hydrodynamic model of a one-dimensional liquid drop to analytically determine the amplitudes of the harmonic and the first superharmonic components of the linear response of the drop. In the nonlinear regime, our numerical analysis reveals an intriguing cascade of instabilities leading to the onset of subharmonic Faraday waves, their modulation instability and chaotic regimes with broadband power spectra. We show that the nonlinear response is highly sensitive to the ratio of the drop size and Faraday wavelength. The primary bifurcation of the harmonic waves is shown to be dominated by a period-doubling bifurcation, when the drop height is comparable with the width of the viscous boundary layer. Experimental results conducted using low-viscosity ethanol and high-viscocity canola oil drops vibrated at 70 Hz are in qualitative agreement with the predictions of our modelling.
The process of drop formation from a nozzle can be seen in many natural systems and engineering applications. Here, we investigate the formation of a liquid droplet from a wettable nozzle. The behavior of a drop is complicated due to an interplay among gravity, capillary rise, viscous drag, and surface tension. In experiments, we observe that drops forming from a wettable nozzle initially climb the outer walls of the nozzle due to surface tension. Then, when the weightof the drops gradually increases, they finally fall due to gravity. By changing the parameters like the nozzle size and fluid flow rate, we have observed that different behaviors of the droplets. Such oscillatory behavior is characterized by a nonlinear equation that consists of capillary rise, viscous drag, and gravity. Two asymptotic solutions in the initial and later stages of drop formation are obtained and show good agreement with experimental observations.
The impact of a liquid drop on a solid surface involves many intertwined physical effects, and is influenced by drop velocity, surface tension, ambient pressure and liquid viscosity, among others. Experiments by Kolinski et al. (2014b) show that the liquid-air interface begins to deviate away from the solid surface even before contact. They found that the lift-off of the interface starts at a critical time that scales with the square root of the kinematic viscosity of the liquid. To understand this, we study the approach of a liquid drop towards a solid surface in the presence of an intervening gas layer. We take a numerical approach to solve the Navier-Stokes equations for the liquid, coupled to the compressible lubrication equations for the gas, in two dimensions. With this approach, we recover the experimentally captured early time effect of liquid viscosity on the drop impact, but our results show that lift-off time and liquid kinematic viscosity have a more complex dependence than the square root scaling relationship. We also predict the effect of interfacial tension at the liquid-gas interface on the drop impact, showing that it mediates the lift-off behavior.
The gasification of multicomponent fuel drops is relevant in various energy-related technologies. An interesting phenomenon associated with this process is the self-induced explosion of the drop, producing a multitude of smaller secondary droplets, which promotes overall fuel atomization and, consequently, improves the combustion efficiency and reduces emissions of liquid-fueled engines. Here, we study a unique explosive gasification process of a tricomponent droplet consisting of water, ethanol, and oil (ouzo), by high-speed monitoring of the entire gasification event taking place in the well-controlled, levitated Leidenfrost state over a superheated plate. It is observed that the preferential evaporation of the most volatile component, ethanol, triggers nucleation of the oil microdroplets/nanodroplets in the remaining drop, which, consequently, becomes an opaque oil-in-water microemulsion. The tiny oil droplets subsequently coalesce into a large one, which, in turn, wraps around the remnant water. Because of the encapsulating oil layer, the droplet can no longer produce enough vapor for its levitation, and, thus, falls and contacts the superheated surface. The direct thermal contact leads to vapor bubble formation inside the drop and consequently drop explosion in the final stage.