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Register a new userTerahertz Light Sources by Electronic-Oscillator-Driven Second Harmonic Generation in Extreme-Confinement Cavities
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The majority of sources of coherent optical radiation rely on laser oscillators driven by population inversion. Despite their technological importance in communications, medicine, industry, and other fields, it remains a challenge to access the spectral range of 0.1-10 THz (the terahertz gap), a frequency band for applications ranging from spectroscopy to security and high-speed wireless communications. Here, we propose a way to produce coherent radiation spanning the THz gap by efficient second-harmonic generation (SHG) in low-loss dielectric structures, starting from technologically mature electronic oscillators (EOs) in the ~100 GHz range. To achieve this goal, we introduce hybrid THz-band dielectric cavity designs that combine (1) extreme field concentration in high-quality-factor resonators with (2) nonlinear materials enhanced by phonon resonances. We theoretically predict conversion efficiencies of >$10^3$ %/W and the potential to bridge the THz gap with 1 W of input power. This approach enables efficient, cascaded parametric frequency converters, representing a new generation of light sources extensible into the mid-IR spectrum and beyond.
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Angle-resolved second harmonic generation (SHG) spectra of ZnO microwires show characteristic Fano resonances in the spectral vicinity of exciton-polariton modes. The output SHG spectra after SHG interacting with exciton polariton shows a resonant enhancement peak accompanied by a suppression dip originating from the constructive and destructive interference respectively. It is demonstrated that the Fano line shape, and thus the Fano asymmetry parameter q, can be tuned by the phase-shift of the two channels. The phase-dependent q was calculated and the model describes our experimental results well. In particular, the phase-to-q relation unveil the crucial information about the dynamics of the system, e.g., defining the line shape of output SHG spectra in a superposition of quantum states.
We employ structured light for the second-harmonic generation from subwavelength AlGaAs nanoparticles that support both electric and magnetic multipolar Mie resonances. The vectorial structure of the pump beam allows addressing selectively Mie-resonant modes and control the strength of the generated nonlinear fields. We observe experimentally the enhancement of the second-harmonic generation for the azimuthally polarized vector beams near magnetic dipole resonance, and match our observations with the numerical decomposion of the Mie-type multipoles for the fundamental and generated second-harmonic fields
In second harmonic generation, the phase of the optical field is doubled which has important implication. Here the phase doubling effect is utilized to solve a long-standing challenge in power scaling of single frequency laser. When a (-{pi}/2, {pi}/2) binary phase modulation is applied to a single frequency seed laser to broaden the spectrum and suppress the stimulated Brillouin scattering in high power fiber amplifier, the second harmonic of the phase-modulated laser will return to single frequency, because the (-{pi}/2, {pi}/2) modulation is doubled to (-{pi}, {pi}) for the second harmonic. A compression rate as high as 95% is demonstrated in the experiment limited by the electronic bandwidth of the setup, which can be improved with optimized devices.
Second-order nonlinear effects, such as second-harmonic generation, can be strongly enhanced in nanofabricated photonic materials when both fundamental and harmonic frequencies are spatially and temporally confined. Practically designing low-volume and doubly resonant nanoresonators in conventional semiconductor compounds is challenging owing to their intrinsic refractive index dispersion. In this work we review a recently developed strategy to design doubly resonant nanocavities with low mode volume and large quality factor by localized defects in a photonic crystal structure. We build on this approach by applying an evolutionary optimisation algorithm in connection with Maxwell equations solvers, showing that the proposed design recipe can be applied to any material platform. We explicitly calculate the second-harmonic generation efficiency for doubly resonant photonic crystal cavity designs in typical III-V semiconductor materials, such as GaN and AlGaAs, targeting a fundamental harmonic at telecom wavelengths, and fully accounting for the tensor nature of the respective nonlinear susceptibilities. These results may stimulate the realisation of small footprint photonic nanostructures in leading semiconductor material platforms to achieve unprecedented nonlinear efficiencies.
A scheme for active second harmonics generation is suggested. The system comprises $N$ three-level atoms in ladder configuration, situated into resonant cavity. It is found that the system can lase in either superradiant or subradiant regime, depending on the number of atoms $N$. When N passes some critical value the transition from the super to subradiance occurs in a phase-transition-like manner. Stability study of the steady state supports this conclusion.
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