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Register a new userEnhanced critical temperatures in the strongly overdoped iron-based superconductors AFe$_2$As$_2$ (A = K, Cs, Rb) observed by point contacts
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A remarkable several times increase (up to 10 K) of the superconducting critical temperature Tc has been observed in point contacts created on the base of single crystals AFe$_2$As$_2$ (A = K, Cs, Rb). Possible reasons for such a Tc increase in point contacts are briefly discussed on a qualitative level. Among them, it is most likely attributed to interfacial carrier doping and/or uniaxial non-homogeneous pressure arising when the contact is created.
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The magnetic properties of iron-based superconductors $A$Fe$_2$As$_2$ ($A=$K, Cs, and Rb), which are characterized by the V-shaped dependence of the critical temperature ($T_{rm c}$) on pressure ($P$) were studied by means of the muon spin rotation/relaxation technique. In all three systems studied the magnetism was found to appear for pressures slightly below the critical one ($P_{rm c}$), i.e. at pressure where $T_{rm c}(P)$ changes the slope. Rather than competing, magnetism and superconductivity in $A$Fe$_2$As$_2$ are coexisting at $Pgtrsim P_{rm c}$ pressure region. Our results support the scenario of a transition from one pairing state to another, with different symmetries on either side of $P_{rm c}$.
We discuss the results of $^{75}$As Nuclear Quadrupole Resonance (NQR) and muon spin relaxation measurements in AFe$_2$As$_2$ (A= Cs, Rb) iron-based superconductors. We demonstrate that the crossover detected in the nuclear spin-lattice relaxation rate $1/T_1$ (around 150 K in RbFe$_2$As$_2$ and around 75 K in CsFe$_2$As$_2$), from a high temperature nearly localized to a low temperature delocalized behaviour, is associated with the onset of an inhomogeneous local charge distribution causing the broadening or even the splitting of the NQR spectra as well as an increase in the muon spin relaxation rate. We argue that this crossover, occurring at temperatures well above the phase transition to the nematic long-range order, is associated with a charge disproportionation at the Fe sites induced by competing Hunds and Coulomb couplings. In RbFe$_2$As$_2$ around 35 K, far below that crossover temperature, we observe a peak in the NQR $1/T_1$ which is possibly associated with the critical slowing down of electronic nematic fluctuations on approaching the transition to the nematic long-range order.
Unconventional superconductivity from heavy fermion (HF) is always observed in f-electron systems, in which Kondo physics between localized f-electrons and itinerant electrons plays an essential role. Whether HF superconductivity could be achieved in other systems without f electrons, especially for d-electron systems, is still elusive. Here, we experimentally study the origin of d-electron HF behavior in iron-based superconductors (FeSCs) AFe2As2 (A = K, Rb, Cs). Nuclear magnetic resonance on 75As reveals a universal coherent-incoherent crossover with a characteristic temperature T*. Below T*, a so-called Knight shift anomaly is first observed in FeSCs, which exhibits a scaling behavior similar to f-electron HF materials. Furthermore, the scaling rule also regulates the manifestation of magnetic fluctuation. These results undoubtedly support an emergent Kondo scenario for the d-electron HF behavior, which suggests the AFe2As2 (A = K, Rb, Cs) as the first material realization of d-electron HF superconductors.
The origin of diverse nematicity and their order parameters in Fe-based superconductors have been attracting increasing attention. Recently, a new type of nematic order has been discovered in heavily hole-doped ($n_d=5.5$) compound AFe$_2$As$_2$ (A=Cs, Rb). The discovered nematicity has $B_{2g}$ (=$d_{xy}$) symmetry, rotated by $45^circ$ from the $B_{1g}$ (=$d_{x^2-y^2}$) nematicity in usual compounds with $n_dapprox6$. We predict that the nematic bond order, which is the symmetry-breaking of the correlated hopping, is responsible for the $B_{2g}$ nematic order in AFe$_2$As$_2$. The Dirac pockets in AFe$_2$As$_2$ is essential to stabilize the $B_{2g}$ bond order. Both $B_{1g}$ and $B_{2g}$ nematicity in A$_{1-x}$Ba$_x$Fe$_2$As$_2$ are naturally induced by the Aslamazov-Larkin many-body process, which describes the spin-fluctuation-driven charge instability. The present study gives a great hint to control the nature of charge nematicity by modifying the orbital character and the topology of the Fermi surface.
We have synthesized two iron fluo-arsenides $A$Ca$_2$Fe$_4$As$_4$F$_2$ with $A$ = Rb and Cs, analogous to the newly discovered superconductor KCa$_2$Fe$_4$As$_4$F$_2$. The quinary inorganic compounds crystallize in a body-centered tetragonal lattice with space group I4/mmm, which contain double Fe$_2$As$_2$ layers that are separated by insulating Ca$_2$F$_2$ layers. Our electrical and magnetic measurements on the polycrystalline samples demonstrate that the new materials undergo superconducting transitions at Tc = 30.5 K and 28.2 K, respectively, without extrinsic doping. The correlations between Tc and structural parameters are discussed.
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