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Register a new userPrecision calculation of hyperfine structure and the Zemach radii of $^{6,7}$Li$^+$ ions
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The hyperfine structures of the $2,^3!S_1$ states of the $^6$Li$^+$ and $^7$Li$^+$ ions are investigated theoretically to extract the Zemach radii of the $^6$Li and $^7$Li nuclei by comparing with precision measurements. The obtained Zemach radii are larger than the previous values of Puchalski and Pachucki [href{https://link.aps.org/doi/10.1103/PhysRevLett.111.243001}{Phys. Rev. Lett. {bf 111}, 243001 (2013)}] and disagree with them by about 1.5 and 2.2 standard deviations for $^6$Li and $^7$Li, respectively. Furthermore, our Zemach radius of $^6$Li differs significantly from the nuclear physics value, derived from the nuclear charge and magnetic radii [href{https://link.aps.org/doi/10.1103/PhysRevA.78.012513}{Phys. Rev. A {bf 78}, 012513 (2008)}], by more than 6 sigma, indicating an anomalous nuclear structure for $^6$Li. The conclusion that the Zemach radius of $^7$Li is about 40% larger than that of $^6$Li is confirmed. The obtained Zemach radii are used to calculate the hyperfine splittings of the $2,^3!P_J$ states of $^{6,7}$Li$^+$, where an order of magnitude improvement over the previous theory has been achieved for $^7$Li$^+$.
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We present benchmark calculations of Zemach moments and radii of 2,3H and 3,4He using various few-body methods. Zemach moments are required to interpret muonic atom data measured by the CREMA collaboration at the Paul Scherrer Institute. Conversely, radii extracted from spectroscopic measurements can be compared with ab initio computations, posing stringent constraints on the nuclear model. For a given few-body method, different numerical procedures can be applied to compute these quantities. A detailed analysis of the numerical uncertainties entering the total theoretical error is presented. Uncertainties from the few-body method and the calculational procedure are found to be smaller than the dependencies on the dynamical modeling and the single nucleon inputs, which are found to be <= 2%. When relativistic corrections and two-body currents are accounted for, the calculated moments and radii are in very good agreement with the available experimental data.
A complete effective Hamiltonian for relativistic corrections at orders $malpha^6$ and $malpha^6(m/M)$ in a one-electron molecular system is derived from the NRQED Lagrangian. It includes spin-independent corrections to the energy levels and spin-spin scalar interactions contributing to the hyperfine splitting, both of which had been studied previously. In addition, corrections to electron spin-orbit and spin-spin tensor interactions are newly obtained. This allows improving the hyperfine structure theory in the hydrogen molecular ions. Improved values of the spin-orbit hyperfine coefficient are calculated for a few transitions of current experimental interest.
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