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Acoustic frequency combs using gas bubble cluster oscillations in liquids: a proof of concept

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 Added by Ivan Maksymov
 Publication date 2020
  fields Physics
and research's language is English




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We propose a new approach to the generation of acoustic frequency combs (AFC) -- signals with spectra containing equidistant coherent peaks. AFCs are essential for a number of sensing and measurement applications, where the established technology of optical frequency combs suffers from fundamental physical limitations. Our proof-of-principle experiments demonstrate that nonlinear oscillations of a gas bubble cluster in water insonated by a low-pressure single-frequency ultrasound wave produce signals with spectra consisting of equally spaced peaks originating from the interaction of the driving ultrasound wave with the response of the bubble cluster at its natural frequency. The so-generated AFC posses essential characteristics of optical frequency combs and thus, similar to their optical counterparts, can be used to measure various physical, chemical and biological quantities.



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Acoustic frequency combs leverage unique properties of the optical frequency comb technology in high-precision measurements and innovative sensing in optically inaccessible environments such as under water, under ground or inside living organisms. Because acoustic combs with wide spectra would be required for many of these applications but techniques of their generation have not yet been developed, here we propose a new approach to the creation of spectrally-wide acoustic combs using oscillations of polydisperse gas bubble clusters in liquids. By means of numerical simulations we demonstrate that clusters consisting of bubbles with precisely controlled sizes can produce wide acoustic spectra composed of equally-spaced coherent peaks. We show that under typical experimental conditions bubble clusters remain stable over time required for a reliable recording of comb signals. We also demonstrate that the spectral composition of combs can be tuned by adjusting the number and size of bubbles in a cluster.
We present here a comprehensive derivation for the speed of a small bottom-heavy sphere forced by a transverse acoustic field and thereby establish how density inhomogeneities may play a critical role in acoustic propulsion. The sphere is trapped at the pressure node of a standing wave whose wavelength is much larger than the sphere diameter. Due to its inhomogeneous density, the sphere oscillates in translation and rotation relative to the surrounding fluid. The perturbative flows induced by the spheres rotation and translation are shown to generate a rectified inertial flow responsible for a net mean force on the sphere that is able to propel the particle within the zero-pressure plane. To avoid an explicit derivation of the streaming flow, the propulsion speed is computed exactly using a suitable version of the Lorentz reciprocal theorem. The propulsion speed is shown to scale as the inverse of the viscosity, the cube of the amplitude of the acoustic field and is a non trivial function of the acoustic frequency. Interestingly, for some combinations of the constitutive parameters (fluid to solid density ratio, moment of inertia and centroid to center of mass distance), the direction of propulsion is reversed as soon as the frequency of the forcing acoustic field becomes larger than a certain threshold. The results produced by the model are compatible with both the observed phenomenology and the orders of magnitude of the measured velocities.
A lipid coated bubble (LCB) oscillator is a very interesting non-smooth oscillator with many important applications ranging from industry and chemistry to medicine. However, due to the complex behavior of the coating intermixed with the nonlinear behavior of the bubble itself, the dynamics of the LCB are not well understood. In this work, lipid coated Definity microbubbles (MBs) were sonicated with 25 MHz 30 cycle pulses with pressure amplitudes between 70kPa-300kPa. Here, we report higher order subharmonics in the scattered signals of single MBs at low amplitude high frequency ultrasound excitations. Experimental observations reveal the generation of period 2(P2), P3, and two different P4 oscillations at low excitation amplitude. Despite the reduced damping of the uncoated bubble system, such enhanced nonlinear oscillations has not been observed and can not be theoretically explained for the uncoated bubble. To investigate the mechanism of the enhanced nonlinearity, the bifurcation structure of the lipid coated MBs is studied for a wide range of MBs sizes and shell parameters. Consistent with the experimental results, we show that this unique oscillator can exhibit chaotic oscillations and higher order subharmonics at excitation amplitudes considerably below those predicted by the uncoated oscillator. Buckling or rupture of the shell and the dynamic variation of the shell elasticity causes the intensified non-linearity at low excitations. The simulated scattered pressure by single MBs are in good agreement with the experimental signals.
361 - J.D. Carter , A. Govan 2015
In this paper, we derive a viscous generalization of the Dysthe (1979) system from the weakly viscous generalization of the Euler equations introduced by Dias, Dyachenko, and Zakharov (2008). This viscous Dysthe system models the evolution of a weakly viscous, nearly monochromatic wave train on deep water. It contains a term which provides a mechanism for frequency downshifting in the absence of wind and wave breaking. The equation does not preserve the spectral mean. Numerical simulations demonstrate that the spectral mean typically decreases and that the spectral peak decreases for certain initial conditions. The linear stability analysis of the plane-wave solutions of the viscous Dysthe system demonstrates that waves with wave numbers closer to zero decay more slowly than waves with wave numbers further from zero. Comparisons between experimental data and numerical simulations of the NLS, dissipative NLS, Dysthe, and viscous Dysthe systems establish that the viscous Dysthe system accurately models data from experiments in which frequency downshifting was observed and experiments in which frequency downshift was not observed.
Laminar flow over a bubble mattress is expected to experience a significant reduction in friction since the individual surfaces of the bubbles are shear-free. However, if the bubbles are sufficiently curved, their protrusion into the fluid and along the flow direction can lead to an increase in friction as was recently demonstrated experimentally and computationally. We provide in this paper a simple model for this result. We consider a shear flow at low Reynolds number past a two-dimensional array of bubbles, and calculate analytically the effective slip length of the surface as function of the bubble geometry in the dilute limit. Our model is able to reproduce quantitatively the relationship between effective friction and bubble geometry obtained in numerical computations, and in particular: (a) The asymmetry in friction between convex and concave bubbles, and (b) the existence of a geometric transition from reduced to enhanced friction at a critical bubble protrusion angle.
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