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We demonstrate a cryogenic buffer gas-cooled molecular beam source capable of producing bright, continuous beams of cold and slow free radicals via laser ablation over durations of up to 60~seconds. The source design uses a closed liquid helium reservoir as a large thermal mass to minimize heating and ensure reproducible beam properties during operation. Under typical conditions, the source produces beams of our test species SrF, containing $5times10^{12}~$molecules per steradian per second in the $X^{2}Sigma(v=0, N=1)$ state with a rotational temperature of $1.0(2)~$K and a forward velocity of $140~$m/s. The beam properties are robust and unchanged for multiple cell geometries but depend critically on the helium buffer gas flow rate, which must be $geq10~$ standard cubic centimeters per minute to produce bright, continuous beams of molecules for an ablation repetition rate of $55~$Hz.
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Ultracold CH radicals promise a fruitful testbed for probing quantum-state controllable organic chemistry. In this work, we calculate CH vibrational branching ratios (VBRs) and rotational branching ratios (RBRs) with ground state mixing. We subsequently use these values to inform optical cycling proposals and consider two possible radiative cooling schemes using the $X^{2}Pi leftarrow A^{2}Delta$ and $X^{2}Pi leftarrow B^{2}Sigma^{-}$ transitions. As a first step towards laser cooled CH, we characterize the effective buffer gas cooling of this species and produce $sim5times10^{10}$ CH molecules per pulse with a rotational temperature of 2(1) K and a translational temperature of 7(2) K. We also determine the CH-helium collisional cross section to be $2.4(8)times10^{-14}$ cm$^{2}$. This value is crucial to correctly account for collisional broadening and accurately extract the in-cell CH density. These cold CH molecules mark an ideal starting point for future laser cooling and trapping experiments and tests of cold organic chemistry.
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Cold-atom interferometers commonly face systematic effects originating from the coupling between the trajectory of the atomic wave packet and the wave front of the laser beams driving the interferometer. Detrimental for the accuracy and the stability of such inertial sensors, these systematics are particularly enhanced in architectures based on spatially separated laser beams. Here we analyze the effect of a coupling between the relative alignment of two separated laser beams and the trajectory of the atomic wave packet in a four-light-pulse cold-atom gyroscope operated in fountain configuration. We present a method to align the two laser beams at the $0.2 mu$rad level and to determine the optimal mean velocity of the atomic wave packet with an accuracy of $0.2 textrm{mm}cdottextrm{s}^{-1}$. Such fine tuning constrains the associated gyroscope bias to a level of $1times 10^{-10}~textrm{rad}cdottextrm{s}^{-1}$. In addition, we reveal this coupling using the point-source interferometry technique by analyzing single-shot time-of-flight fluorescence traces, which allows us to measure large angular misalignments between the interrogation beams. The alignment method which we present here can be employed in other sensor configurations and is particularly relevant to emerging gravitational wave detector concepts based on cold-atom interferometry.
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