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Register a new userExtreme Raman red shift: ultrafast multimode non-linear space-time dynamics, pulse compression, and broadly tunable frequency conversion
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Added by
Paolo Antonio Carpeggiani
Publication date
2020
fields
Physics
and research's language is
English
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Ultrashort high-energy pulses at wavelengths longer than 1 $mu$m are nowadays desired for a vast variety of applications in ultrafast and strong-field physics. To date, the main answer to the wavelength tunability for energetic, broadband pulses still relies on optical parametric amplification (OPA), which often requires multiple and complex stages, may feature imperfect beam quality and has limited conversion efficiency into one of the amplified waves. In this work, we present a completely different strategy to realize an energy-efficient and scalable laser frequency shifter. This relies on the continuous red shift provided by stimulated Raman scattering (SRS) over a long propagation distance in nitrogen-filled hollow core fibers (HCF). We show a continuous tunability of the laser wavelength from 1030 nm up to 1730 nm with conversion efficiency higher than 70% and high beam quality. The highly asymmetric spectral broadening, arising from the spatiotemporal nonlinear interplay between high-order modes of the HCF, can be readily employed to generate pulses (~20 fs) significantly shorter than the pump ones (~200 fs) with high beam quality, and the pulse energy can further be scaled up to tens of millijoules. We envision that this technique, coupled with the emerging high-power Yb laser technology, has the potential to answer the increasing demand for energetic multi-TW few-cycle sources tunable in the near-IR.
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Synthetic dimensions in photonic structures provide unique opportunities for actively manipulating light in multiple degrees of freedom. Here, we theoretically explore a dispersive waveguide under the dynamic phase modulation that supports single pulse manipulations in the synthetic (2+1) dimensions. Compared with the counterpart of the conventional (2+1) space-time, we explore temporal diffraction and frequency conversion in a synthetic time-frequency space while the pulse evolves along the spatial dimension. By introducing the effective gauge potential well for photons in the synthetic time-frequency space with the control of the modulation phase, we show that a rich set of pulse propagation behaviors can be achieved, including confined pulse propagation, fast/slow light, and pulse compression. With the additional nonlinear oscillation subject to the effective force along the frequency axis of light, we provide an exotic approach for actively manipulating the single pulse in both temporal and spectral domains, which shows the great promise for applications of the pulse processing and optical communications in integrated photonics.
Visualizing ultrafast dynamics at the atomic scale requires time-resolved pump-probe characterization with femtosecond temporal resolution. For single-shot ultrafast electron diffraction (UED) with fully relativistic electron bunch probes, existing techniques are limited by the achievable electron probe bunch length, charge, and timing jitter. We present the first experimental demonstration of pump-probe UED with THz-driven compression and time-stamping that enable UED probes with unprecedented temporal resolution. This technique utilizes two counter-propagating quasi-single-cycle THz pulses generated from two OH-1 organic crystals coupled into an optimized THz compressor structure. Ultrafast dynamics of photoexcited bismuth films show an improved temporal resolution from 178 fs down to 85 fs when the THz-compressed UED probes are used with no time-stamping correction. Furthermore, we use a novel time-stamping technique to reveal transient oscillations in the dynamical response of THz-excited single-crystal gold films previously inaccessible by standard UED, achieving a time-stamped temporal resolution down to 5 fs.
The 1-10 terahertz (THz) spectral window is emerging as a key region for plenty of applications, requiring not yet available continuous-wave room-temperature THz spectrometers with high spectral purity and ultra-broad tunability. In this regard, the spectral features of stabilized telecom sources can actually be transferred to the THz range by difference frequency generation, considering that the width of the accessible THz spectrum generally scales with the area involved in the nonlinear interaction. For this reason, in this paper we extensively discuss the role of Lithium Niobate (LN) channel waveguides in the experimental accomplishment of a room-temperature continuous wave (CW) spectrometer, with uW-range power levels and a spectral coverage of up to 7.5 THz.To this purpose, and looking for further improvements, a thought characterization of specially-designed LN waveguides is presented, whilst discussing its nonlinear efficiency and its unprecedented capability to handle high optical power (10 7 W/cm 2 ), on the basis of a three-wave-mixing theoretical model.
High-Q microresonator has been suggested a promising platform for optical frequency comb generation, via dissipative soliton formation. To achieve a higher Q and obtain the necessary anomalous dispersion, $Si_3N_4$ microresonators made of multi-mode waveguides were previously implemented. However, coupling between different transverse mode families in the multi-mode waveguides results in periodic disruption of dispersion and quality factor, introducing perturbation to dissipative soliton formation and amplitude modulation to the corresponding spectrum. Careful choice of pump wavelength to avoid the mode crossing region is thus critical in conventional $Si_3N_4$ microresonators. Here, we report a novel design of $Si_3N_4$ microresonator such that single mode operation, high quality factor, and anomalous dispersion are attained simultaneously. The microresonator is consisted of uniform single mode waveguides in the semi-circle region, to eliminate bending induced mode coupling, and adiabatically tapered waveguides in the straight region, to avoid excitation of higher order modes. The intrinsic Q of the microresonator reaches $1.36 times 10^6$ while the GVD remains to be anomalous at $-50 fs^2/mm$. We demonstrate, with this novel microresonator, broadband phase-locked Kerr frequency combs with flat and smooth spectra can be generated by pumping at any resonances in the optical C-band.
Space-time modulated metamaterials support extraordinary rich applications, such as parametric amplification, frequency conversion and non-reciprocal transmission. However, experimental realization of space-time modulation is highly non-trivial, hindering many interesting physics that are theoretically predicted to be experimentally demonstrated. Here, based on the proposed virtualized metamaterials with software-defined impulse response, we experimentally realize non-Hermitian space-time varying metamaterials for efficient and asymmetric frequency conversion by allowing material gain and loss to be tailor-made and balanced in the time domain. In the application of frequency conversion, the combination of space-time varying capability and non-Hermiticity allows us to diminish the main band through gain-loss balance and to increase the efficiency of side band conversion at the same time. In addition, our approach of software-defined metamaterials is flexible to realize the analogy of quantum interference in an acoustic system with design capability. Applying an additional modulation phase delay between different atoms allows to control such interference to get asymmetric amplification in frequency conversion.
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